Self-Assembled Asymmetric Block Copolymer Membranes: Bridging the Gap from Ultra- to Nanofiltration
The self‐assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra‐ to nanofiltration and decrease the pore size of self‐assembled block copolymer membranes to below 5 nm without post‐...
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| Published in | Angewandte Chemie International Edition Vol. 54; no. 47; pp. 13937 - 13941 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
16.11.2015
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The self‐assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra‐ to nanofiltration and decrease the pore size of self‐assembled block copolymer membranes to below 5 nm without post‐treatment. It is now reported that the self‐assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol−1 in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux.
Blends of two chemically interacting copolymers bridge the gap from ultra‐ (UF) to nanofiltration (NF) as such membranes with pore sizes below 5 nm have been synthesized without post‐treatment. Simulations of the membrane formation process by dissipative particle dynamics were used to explain the dramatic observed pore size reduction combined with an increase in water flux. |
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| AbstractList | The self-assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra- to nanofiltration and decrease the pore size of self-assembled block copolymer membranes to below 5 nm without post-treatment. It is now reported that the self-assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol(-1) in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux.The self-assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra- to nanofiltration and decrease the pore size of self-assembled block copolymer membranes to below 5 nm without post-treatment. It is now reported that the self-assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol(-1) in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux. The self-assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra- to nanofiltration and decrease the pore size of self-assembled block copolymer membranes to below 5nm without post-treatment. It is now reported that the self-assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5nm. The membrane containing an ultraporous, 60nm thin separation layer can fully reject solutes with molecular weights of 600gmol-1 in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux. The self‐assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra‐ to nanofiltration and decrease the pore size of self‐assembled block copolymer membranes to below 5 nm without post‐treatment. It is now reported that the self‐assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol −1 in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux. The self-assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra- to nanofiltration and decrease the pore size of self-assembled block copolymer membranes to below 5 nm without post-treatment. It is now reported that the self-assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol(-1) in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux. The self‐assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to bridge the gap from ultra‐ to nanofiltration and decrease the pore size of self‐assembled block copolymer membranes to below 5 nm without post‐treatment. It is now reported that the self‐assembly of blends of two chemically interacting copolymers can lead to highly porous membranes with pore diameters as small as 1.5 nm. The membrane containing an ultraporous, 60 nm thin separation layer can fully reject solutes with molecular weights of 600 g mol−1 in aqueous solutions with a water flux that is more than one order of magnitude higher than the permeance of commercial nanofiltration membranes. Simulations of the membrane formation process by dissipative particle dynamics (DPD) were used to explain the dramatic observed pore size reduction combined with an increase in water flux. Blends of two chemically interacting copolymers bridge the gap from ultra‐ (UF) to nanofiltration (NF) as such membranes with pore sizes below 5 nm have been synthesized without post‐treatment. Simulations of the membrane formation process by dissipative particle dynamics were used to explain the dramatic observed pore size reduction combined with an increase in water flux. |
| Author | Ma, Zengwei Moreno, Nicolas Yu, Haizhou Nunes, Suzana P. Peinemann, Klaus-Viktor Qiu, Xiaoyan Calo, Victor Manuel |
| Author_xml | – sequence: 1 givenname: Haizhou surname: Yu fullname: Yu, Haizhou organization: Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) – sequence: 2 givenname: Xiaoyan surname: Qiu fullname: Qiu, Xiaoyan organization: Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) – sequence: 3 givenname: Nicolas surname: Moreno fullname: Moreno, Nicolas organization: Biological and Environmental Science and Engineering Division (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) – sequence: 4 givenname: Zengwei surname: Ma fullname: Ma, Zengwei organization: School of Optoelectronic Information, Chongqing University of Technology, Chongqing 40054 (China) – sequence: 5 givenname: Victor Manuel surname: Calo fullname: Calo, Victor Manuel organization: Center for Numerical Porous Media (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) – sequence: 6 givenname: Suzana P. surname: Nunes fullname: Nunes, Suzana P. organization: Biological and Environmental Science and Engineering Division (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) – sequence: 7 givenname: Klaus-Viktor surname: Peinemann fullname: Peinemann, Klaus-Viktor email: klausviktor.peinemann@kaust.edu.sa organization: Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900 (Kingdom of Saudi Arabia) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26388216$$D View this record in MEDLINE/PubMed |
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| Keywords | membranes block copolymers self-assembly nanofiltration |
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| Snippet | The self‐assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to... The self-assembly of block copolymers is an emerging strategy to produce isoporous ultrafiltration membranes. However, thus far, it has not been possible to... |
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| SubjectTerms | block copolymers Copolymers Membranes Nanofiltration Nanotechnology Pore size self-assembly Solutes Ultrafiltration |
| Title | Self-Assembled Asymmetric Block Copolymer Membranes: Bridging the Gap from Ultra- to Nanofiltration |
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