Mn2+ induced significant improvement and robust stability of radioluminescence in Cs3Cu2I5 for high-performance nuclear battery
Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh circumstances without instant energy supply. In spite of the progress of device structure design, the development of scintillators is far behind. Her...
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| Published in | Nature communications Vol. 12; no. 1; p. 3879 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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London
Nature Publishing Group UK
23.06.2021
Nature Publishing Group Nature Portfolio |
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| Abstract | Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh circumstances without instant energy supply. In spite of the progress of device structure design, the development of scintillators is far behind. Here, a Cs
3
Cu
2
I
5
: Mn scintillator showing a high light yield of ~67000 ph MeV
−1
at 564 nm is presented. Doping and intrinsic features endow Cs
3
Cu
2
I
5
: Mn with robust thermal stability and irradiation hardness that 71% or >95% of the initial radioluminescence intensity can be maintained in an ultra-broad temperature range of 77 K-433 K or after a total irradiation dose of 2590 Gy, respectively. These superiorities allow the fabrication of efficient and stable nuclear batteries, which show an output improvement of 237% respect to the photovoltaic device without scintillator. Luminescence mechanisms including self-trapped exciton, energy transfer, and impact excitation are proposed for the anomalous dramatic radioluminescence improvement. This work will open a window for the fields of nuclear battery and radiography.
Fluorescent-type nuclear batteries are a promising semi-permanent power source, but performance is hindered by scintillator development. Here the authors report a scintillator with high light yield and stability, which leads to improved performance. |
|---|---|
| AbstractList | Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh circumstances without instant energy supply. In spite of the progress of device structure design, the development of scintillators is far behind. Here, a Cs
3
Cu
2
I
5
: Mn scintillator showing a high light yield of ~67000 ph MeV
−1
at 564 nm is presented. Doping and intrinsic features endow Cs
3
Cu
2
I
5
: Mn with robust thermal stability and irradiation hardness that 71% or >95% of the initial radioluminescence intensity can be maintained in an ultra-broad temperature range of 77 K-433 K or after a total irradiation dose of 2590 Gy, respectively. These superiorities allow the fabrication of efficient and stable nuclear batteries, which show an output improvement of 237% respect to the photovoltaic device without scintillator. Luminescence mechanisms including self-trapped exciton, energy transfer, and impact excitation are proposed for the anomalous dramatic radioluminescence improvement. This work will open a window for the fields of nuclear battery and radiography.
Fluorescent-type nuclear batteries are a promising semi-permanent power source, but performance is hindered by scintillator development. Here the authors report a scintillator with high light yield and stability, which leads to improved performance. Fluorescent-type nuclear batteries are a promising semi-permanent power source, but performance is hindered by scintillator development. Here the authors report a scintillator with high light yield and stability, which leads to improved performance. Abstract Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh circumstances without instant energy supply. In spite of the progress of device structure design, the development of scintillators is far behind. Here, a Cs 3 Cu 2 I 5 : Mn scintillator showing a high light yield of ~67000 ph MeV −1 at 564 nm is presented. Doping and intrinsic features endow Cs 3 Cu 2 I 5 : Mn with robust thermal stability and irradiation hardness that 71% or >95% of the initial radioluminescence intensity can be maintained in an ultra-broad temperature range of 77 K-433 K or after a total irradiation dose of 2590 Gy, respectively. These superiorities allow the fabrication of efficient and stable nuclear batteries, which show an output improvement of 237% respect to the photovoltaic device without scintillator. Luminescence mechanisms including self-trapped exciton, energy transfer, and impact excitation are proposed for the anomalous dramatic radioluminescence improvement. This work will open a window for the fields of nuclear battery and radiography. Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh circumstances without instant energy supply. In spite of the progress of device structure design, the development of scintillators is far behind. Here, a Cs3Cu2I5: Mn scintillator showing a high light yield of ~67000 ph MeV−1 at 564 nm is presented. Doping and intrinsic features endow Cs3Cu2I5: Mn with robust thermal stability and irradiation hardness that 71% or >95% of the initial radioluminescence intensity can be maintained in an ultra-broad temperature range of 77 K-433 K or after a total irradiation dose of 2590 Gy, respectively. These superiorities allow the fabrication of efficient and stable nuclear batteries, which show an output improvement of 237% respect to the photovoltaic device without scintillator. Luminescence mechanisms including self-trapped exciton, energy transfer, and impact excitation are proposed for the anomalous dramatic radioluminescence improvement. This work will open a window for the fields of nuclear battery and radiography.Fluorescent-type nuclear batteries are a promising semi-permanent power source, but performance is hindered by scintillator development. Here the authors report a scintillator with high light yield and stability, which leads to improved performance. |
| ArticleNumber | 3879 |
| Author | Chen, Xi Chen, Jiaxin Geng, Dongling Jiang, Lianfu Wu, Ye Yang, Dandan Li, Xiaoming Zeng, Haibo Meng, Cuifang |
| Author_xml | – sequence: 1 givenname: Xiaoming surname: Li fullname: Li, Xiaoming organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 2 givenname: Jiaxin surname: Chen fullname: Chen, Jiaxin organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 3 givenname: Dandan surname: Yang fullname: Yang, Dandan organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 4 givenname: Xi orcidid: 0000-0001-6141-7326 surname: Chen fullname: Chen, Xi organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 5 givenname: Dongling surname: Geng fullname: Geng, Dongling organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 6 givenname: Lianfu surname: Jiang fullname: Jiang, Lianfu organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 7 givenname: Ye surname: Wu fullname: Wu, Ye organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 8 givenname: Cuifang surname: Meng fullname: Meng, Cuifang organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology – sequence: 9 givenname: Haibo orcidid: 0000-0002-0260-1059 surname: Zeng fullname: Zeng, Haibo email: zeng.haibo@njust.edu.cn organization: MIIT Key Laboratory of Advanced Display Material and Devices, School of Materials Science and Engineering, Nanjing University of Science and Technology |
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| Snippet | Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh... Abstract Fluorescent type nuclear battery consisting of scintillator and photovoltaic device enables semipermanent power source for devices working under harsh... Fluorescent-type nuclear batteries are a promising semi-permanent power source, but performance is hindered by scintillator development. Here the authors... |
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| SubjectTerms | 140/146 147/135 639/301 639/4077 Efficiency Energy Energy transfer Excitons Fabrication Fluorescence Humanities and Social Sciences Irradiation Light multidisciplinary Optical properties Photovoltaics Radiation Radiation dosage Radiography Robustness Science Science (multidisciplinary) Scintillation counters Thermal stability |
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| Title | Mn2+ induced significant improvement and robust stability of radioluminescence in Cs3Cu2I5 for high-performance nuclear battery |
| URI | https://link.springer.com/article/10.1038/s41467-021-24185-7 https://www.proquest.com/docview/2544321260 https://search.proquest.com/docview/2544882134 https://pubmed.ncbi.nlm.nih.gov/PMC8222237 https://doaj.org/article/9dc4ede3eecd4bb5a2792d1cc0aac8f8 |
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