Taming a Functional Group: Creating Air-Stable, Chiral Primary Phosphanes
No rings of fire! Enantiopure primary phosphanes have been developed which are remarkably stable to air oxidation in both solid and solution states (see example). This new class of stable ligand synthon appears to owe its stability to conjugation in their aryl backbones with the extended π ring syst...
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| Published in | Angewandte Chemie International Edition Vol. 45; no. 43; pp. 7248 - 7251 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
06.11.2006
WILEY‐VCH Verlag Wiley |
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| Online Access | Get full text |
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| Abstract | No rings of fire! Enantiopure primary phosphanes have been developed which are remarkably stable to air oxidation in both solid and solution states (see example). This new class of stable ligand synthon appears to owe its stability to conjugation in their aryl backbones with the extended π ring system. Even one extra ring is good enough. |
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| AbstractList | No rings of fire! Enantiopure primary phosphanes have been developed which are remarkably stable to air oxidation in both solid and solution states (see example). This new class of stable ligand synthon appears to owe its stability to conjugation in their aryl backbones with the extended π ring system. Even one extra ring is good enough. |
| Author | Gilheany, Declan G. Higham, Lee J. Hiney, Rachel M. Müller-Bunz, Helge |
| Author_xml | – sequence: 1 givenname: Rachel M. surname: Hiney fullname: Hiney, Rachel M. organization: School of Chemistry and Chemical Biology, Centre for Synthesis and Chemical Biology, Conway Institute for Biomolecular and Biomedical Research, University College Dublin, Belfield, Dublin 4, Ireland, Fax: (+353) 1-716-2127 – sequence: 2 givenname: Lee J. surname: Higham fullname: Higham, Lee J. email: lee.higham@ucd.ie organization: School of Chemistry and Chemical Biology, Centre for Synthesis and Chemical Biology, Conway Institute for Biomolecular and Biomedical Research, University College Dublin, Belfield, Dublin 4, Ireland, Fax: (+353) 1-716-2127 – sequence: 3 givenname: Helge surname: Müller-Bunz fullname: Müller-Bunz, Helge organization: School of Chemistry and Chemical Biology, Centre for Synthesis and Chemical Biology, Conway Institute for Biomolecular and Biomedical Research, University College Dublin, Belfield, Dublin 4, Ireland, Fax: (+353) 1-716-2127 – sequence: 4 givenname: Declan G. surname: Gilheany fullname: Gilheany, Declan G. email: declan.gilheany@ucd.ie organization: School of Chemistry and Chemical Biology, Centre for Synthesis and Chemical Biology, Conway Institute for Biomolecular and Biomedical Research, University College Dublin, Belfield, Dublin 4, Ireland, Fax: (+353) 1-716-2127 |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/17022105$$D View this record in MEDLINE/PubMed |
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| Keywords | DESIGN ASYMMETRIC-SYNTHESIS HYDROGENATION OXIDE electrochemistry CRYSTAL asymmetric catalysis air stability phosphanes PRIMARY PHOSPHINES conjugation LIGANDS CHEMISTRY BOND |
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| Notes | Irish Research Council for Science, Engineering, and Technology (IRCSET) ark:/67375/WNG-8P471296-8 EU - No. HMPD-CT-2000-00053 ArticleID:ANIE200602143 We thank the Irish Research Council for Science, Engineering, and Technology (IRCSET) for a scholarship for R.M.H. and the EU for a Marie Curie Host Development Fellowship (HMPD-CT-2000-00053) for L.J.H. We also thank Prof. R. O'Neill for electrochemistry advice and apparatus as well as Dr. G. Docherty (Rhodia) for discussions on phenylphosphane. istex:62194D1A3E0F0723FC6FF37D7988C4262EE29759 We thank the Irish Research Council for Science, Engineering, and Technology (IRCSET) for a scholarship for R.M.H. and the EU for a Marie Curie Host Development Fellowship (HMPD‐CT‐2000‐00053) for L.J.H. We also thank Prof. R. O'Neill for electrochemistry advice and apparatus as well as Dr. G. Docherty (Rhodia) for discussions on phenylphosphane. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| Snippet | No rings of fire! Enantiopure primary phosphanes have been developed which are remarkably stable to air oxidation in both solid and solution states (see... |
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| SubjectTerms | Air air stability asymmetric catalysis Chemistry Chemistry, Multidisciplinary conjugation Crystallography, X-Ray electrochemistry Models, Molecular Molecular Structure Oxidation-Reduction phosphanes Phosphines - chemical synthesis Phosphines - chemistry Physical Sciences Science & Technology Stereoisomerism |
| Title | Taming a Functional Group: Creating Air-Stable, Chiral Primary Phosphanes |
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