Formation of Hexagonally Packed Hollow Hoops and Morphology Transition in RAFT Ethanol Dispersion Polymerization
Similar to the traditional self‐assembly strategy, polymerization induced self‐assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the...
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| Published in | Macromolecular rapid communications. Vol. 36; no. 15; pp. 1428 - 1436 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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Germany
Blackwell Publishing Ltd
01.08.2015
Wiley Subscription Services, Inc |
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| Abstract | Similar to the traditional self‐assembly strategy, polymerization induced self‐assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano‐objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials.
Highly ordered assemblies with a hexagonally packed hollow hoops (HHHs) structure are successfully fabricated through morphology transition from large compound vesicles to HHHs in RAFT dispersion polymerization for the first time. Besides the chain length ratio (R) of hydrophobic to hydrophilic blocks, the chain mobility in the nano‐objects is a determining factor for morphology transition. |
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| AbstractList | Similar to the traditional self-assembly strategy, polymerization induced self-assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano-objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials. Similar to the traditional self‐assembly strategy, polymerization induced self‐assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano‐objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials. Highly ordered assemblies with a hexagonally packed hollow hoops (HHHs) structure are successfully fabricated through morphology transition from large compound vesicles to HHHs in RAFT dispersion polymerization for the first time. Besides the chain length ratio (R) of hydrophobic to hydrophilic blocks, the chain mobility in the nano‐objects is a determining factor for morphology transition. Similar to the traditional self‐assembly strategy, polymerization induced self‐assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio ( R ) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano‐objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials. image Similar to the traditional self-assembly strategy, polymerization induced self-assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano-objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials.Similar to the traditional self-assembly strategy, polymerization induced self-assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano-objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials. Similar to the traditional self-assembly strategy, polymerization induced self-assembly and reorganization (PISR) can produce a myriad of polymeric morphologies through morphology transitions. Besides the chain length ratio (R) of the hydrophobic to the hydrophilic blocks, the chain mobility in the intermediate nano-objects, which is a requisite for morphology transition, is a determining factor in the formation of the final morphology. Although various morphologies have been fabricated, hexagonally packed hollow hoops (HHHs) with highly ordered internal structure have not, to the best of our knowledge, been prepared by PISR. In this article, the fabrication of HHHs through morphology transition from large compound vesicles to HHHs is reported. HHHs with highly regular internal structure may have significance in theoretical research and practical applications of nanomaterials. Highly ordered assemblies with a hexagonally packed hollow hoops (HHHs) structure are successfully fabricated through morphology transition from large compound vesicles to HHHs in RAFT dispersion polymerization for the first time. Besides the chain length ratio (R) of hydrophobic to hydrophilic blocks, the chain mobility in the nano-objects is a determining factor for morphology transition. |
| Author | Pan, Cai-Yuan Zhang, Wen-Jian Hong, Chun-Yan |
| Author_xml | – sequence: 1 givenname: Wen-Jian surname: Zhang fullname: Zhang, Wen-Jian organization: CAS Key Laboratory of Soft Matter Chemistry, Department of Polymer Science and Engineering, University of Science and Technology of China, Anhui, 230026, Hefei, P. R. China – sequence: 2 givenname: Chun-Yan surname: Hong fullname: Hong, Chun-Yan email: hongcy@ustc.edu.cn organization: CAS Key Laboratory of Soft Matter Chemistry, Department of Polymer Science and Engineering, University of Science and Technology of China, Anhui, 230026, Hefei, P. R. China – sequence: 3 givenname: Cai-Yuan surname: Pan fullname: Pan, Cai-Yuan email: hongcy@ustc.edu.cn organization: CAS Key Laboratory of Soft Matter Chemistry, Department of Polymer Science and Engineering, University of Science and Technology of China, Anhui, 230026, Hefei, P. R. China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26032959$$D View this record in MEDLINE/PubMed |
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| Copyright | 2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. Copyright 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Keywords | morphology transition RAFT dispersion polymerization hexagonally packed hollow hoops |
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| Snippet | Similar to the traditional self‐assembly strategy, polymerization induced self‐assembly and reorganization (PISR) can produce a myriad of polymeric... Similar to the traditional self-assembly strategy, polymerization induced self-assembly and reorganization (PISR) can produce a myriad of polymeric... |
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| SubjectTerms | Chain mobility Dispersions Ethanol Ethanol - chemistry Ethyl alcohol Fabrication hexagonally packed hollow hoops Hoops Hydrophobic and Hydrophilic Interactions Morphology morphology transition Nanotechnology Polymerization Polymers - chemistry RAFT dispersion polymerization Rafts Self assembly Vesicles |
| Title | Formation of Hexagonally Packed Hollow Hoops and Morphology Transition in RAFT Ethanol Dispersion Polymerization |
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