Metal-organic framework-based foams for efficient microplastics removal
Microplastics are a worldwide problem that poses a giant threat to organisms in the ecosystem and even to human health. The removal of microplastics is a severe challenge that needs to be solved urgently. Herein, a series of zirconium metal-organic framework-based foam materials with interpenetrated...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 8; no. 29; pp. 14644 - 14652 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
28.07.2020
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Microplastics are a worldwide problem that poses a giant threat to organisms in the ecosystem and even to human health. The removal of microplastics is a severe challenge that needs to be solved urgently. Herein, a series of zirconium metal-organic framework-based foam materials with interpenetrated pores, high MOF uniformity and excellent durability have been successfully fabricated and applied in simulated microplastics removal in water or seawater conditions. They can be applied to various types and concentrations of microplastics suspensions. It is worth noting that the best of them, UiO-66-OH@MF-3, can efficiently remove microplastics with an efficiency of up to 95.5 ± 1.2% and can maintain high performance in recycling and large-quantity filtration experiments. Besides, we proposed an automatic filtration system powered by sunlight and accomplished it on the lab-scale. The high performances of these foam materials combined with the new concept of automatic filtration systems might shed some light on the development of novel techniques for microplastics removal.
Zirconium metal-organic frameworks based foam materials have been successfully fabricated and applied in microplastic removal with high efficiency. |
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| AbstractList | Microplastics are a worldwide problem that poses a giant threat to organisms in the ecosystem and even to human health. The removal of microplastics is a severe challenge that needs to be solved urgently. Herein, a series of zirconium metal–organic framework-based foam materials with interpenetrated pores, high MOF uniformity and excellent durability have been successfully fabricated and applied in simulated microplastics removal in water or seawater conditions. They can be applied to various types and concentrations of microplastics suspensions. It is worth noting that the best of them, UiO-66-OH@MF-3, can efficiently remove microplastics with an efficiency of up to 95.5 ± 1.2% and can maintain high performance in recycling and large-quantity filtration experiments. Besides, we proposed an automatic filtration system powered by sunlight and accomplished it on the lab-scale. The high performances of these foam materials combined with the new concept of automatic filtration systems might shed some light on the development of novel techniques for microplastics removal. Microplastics are a worldwide problem that poses a giant threat to organisms in the ecosystem and even to human health. The removal of microplastics is a severe challenge that needs to be solved urgently. Herein, a series of zirconium metal-organic framework-based foam materials with interpenetrated pores, high MOF uniformity and excellent durability have been successfully fabricated and applied in simulated microplastics removal in water or seawater conditions. They can be applied to various types and concentrations of microplastics suspensions. It is worth noting that the best of them, UiO-66-OH@MF-3, can efficiently remove microplastics with an efficiency of up to 95.5 ± 1.2% and can maintain high performance in recycling and large-quantity filtration experiments. Besides, we proposed an automatic filtration system powered by sunlight and accomplished it on the lab-scale. The high performances of these foam materials combined with the new concept of automatic filtration systems might shed some light on the development of novel techniques for microplastics removal. Zirconium metal-organic frameworks based foam materials have been successfully fabricated and applied in microplastic removal with high efficiency. |
| Author | Miao, Chang Lan, Ya-Qian Chen, Yifa Wang, Yi-Rong Chen, Yong-Jun Li, Shun-Li Yang, Ru-Xin Wang, Jian-Hui Gao, Guang-Kuo Zhu, Hong-Jing |
| AuthorAffiliation | Nanjing Normal University Changzhou Institute of Innovation & Development Jiangsu Key Laboratory of New Power Batteries School of Chemistry and Materials Science Jiangsu Collaborative Innovation Centre of Biomedical Functional Materials |
| AuthorAffiliation_xml | – name: School of Chemistry and Materials Science – name: Jiangsu Collaborative Innovation Centre of Biomedical Functional Materials – name: Changzhou Institute of Innovation & Development – name: Nanjing Normal University – name: Jiangsu Key Laboratory of New Power Batteries |
| Author_xml | – sequence: 1 givenname: Yong-Jun surname: Chen fullname: Chen, Yong-Jun – sequence: 2 givenname: Yifa surname: Chen fullname: Chen, Yifa – sequence: 3 givenname: Chang surname: Miao fullname: Miao, Chang – sequence: 4 givenname: Yi-Rong surname: Wang fullname: Wang, Yi-Rong – sequence: 5 givenname: Guang-Kuo surname: Gao fullname: Gao, Guang-Kuo – sequence: 6 givenname: Ru-Xin surname: Yang fullname: Yang, Ru-Xin – sequence: 7 givenname: Hong-Jing surname: Zhu fullname: Zhu, Hong-Jing – sequence: 8 givenname: Jian-Hui surname: Wang fullname: Wang, Jian-Hui – sequence: 9 givenname: Shun-Li surname: Li fullname: Li, Shun-Li – sequence: 10 givenname: Ya-Qian surname: Lan fullname: Lan, Ya-Qian |
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| Title | Metal-organic framework-based foams for efficient microplastics removal |
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