CFD model for the simulation of chemical looping combustion

A chemical looping combustion (CLC) system uses a metal oxide solid carrier to combust a source of fuel in isolation from the source of oxygen which produces an exhaust gas of primarily carbon dioxide and water. In this work, a full three-dimensional model of a chemical looping combustion system was...

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Published inPowder technology Vol. 265; pp. 47 - 53
Main Author Parker, James M.
Format Journal Article Conference Proceeding
LanguageEnglish
Published Amsterdam Elsevier B.V 01.10.2014
Elsevier
Subjects
Applied sciences
Chemical engineering
Chemical looping combustion
Computational fluid dynamics
CPFD method
Exact sciences and technology
Fluidization
Hydrodynamics of contact apparatus
Miscellaneous
Reactors
Solid-solid systems
Computational fluid dynamics
CPFD method
Chemical looping combustion
Temperature distribution
Swelling
Carbon dioxide
Hydrodynamics
Combustion
Devolatilization
Fluidization
Modeling
Three dimensional model
Utilities
Coal
Fuel
Exhaust gas
Gasification
Oxidation
Reactor
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Abstract A chemical looping combustion (CLC) system uses a metal oxide solid carrier to combust a source of fuel in isolation from the source of oxygen which produces an exhaust gas of primarily carbon dioxide and water. In this work, a full three-dimensional model of a chemical looping combustion system was developed to simulate the particle–fluid hydrodynamics, thermal characteristics, and reaction efficiency of the CLC system using coal particles as a fuel source. Multiple heterogeneous and homogenous reactions are considered in the CLC model including the oxidation and reduction reactions of the metal oxide carrier and gasification reactions. Within each coal particle, the temperature-dependent devolatilization, moisture release, and particle swelling effects are included. Modeling results showing fluidization regimes, circulation rate, reactor efficiencies, and temperature profiles are presented to demonstrate the utility of the model.
AbstractList A chemical looping combustion (CLC) system uses a metal oxide solid carrier to combust a source of fuel in isolation from the source of oxygen which produces an exhaust gas of primarily carbon dioxide and water. In this work, a full three-dimensional model of a chemical looping combustion system was developed to simulate the particle–fluid hydrodynamics, thermal characteristics, and reaction efficiency of the CLC system using coal particles as a fuel source. Multiple heterogeneous and homogenous reactions are considered in the CLC model including the oxidation and reduction reactions of the metal oxide carrier and gasification reactions. Within each coal particle, the temperature-dependent devolatilization, moisture release, and particle swelling effects are included. Modeling results showing fluidization regimes, circulation rate, reactor efficiencies, and temperature profiles are presented to demonstrate the utility of the model.
Author Parker, James M.
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  givenname: James M.
  surname: Parker
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Keywords Computational fluid dynamics
CPFD method
Chemical looping combustion
Temperature distribution
Swelling
Carbon dioxide
Hydrodynamics
Combustion
Devolatilization
Fluidization
Modeling
Three dimensional model
Utilities
Coal
Fuel
Exhaust gas
Gasification
Oxidation
Reactor
Language English
License CC BY 4.0
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MeetingName Selected Papers from the 2012 NETL Multiphase Flow Workshop
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Snippet A chemical looping combustion (CLC) system uses a metal oxide solid carrier to combust a source of fuel in isolation from the source of oxygen which produces...
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StartPage 47
SubjectTerms Applied sciences
Chemical engineering
Chemical looping combustion
Computational fluid dynamics
CPFD method
Exact sciences and technology
Fluidization
Hydrodynamics of contact apparatus
Miscellaneous
Reactors
Solid-solid systems
Title CFD model for the simulation of chemical looping combustion
URI https://dx.doi.org/10.1016/j.powtec.2014.01.027
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