Perovskite LaNiO3/Ag3PO4 heterojunction photocatalyst for the degradation of dyes

Pristine lanthanum nickelate (LaNiO 3 ), silver phosphate (Ag 3 PO 4 ) and perovskite lanthanum nickelate silver phosphate composites (LaNiO 3 /Ag 3 PO 4 ) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO 3 in Ag 3 PO 4 . The ph...

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Published inFrontiers in chemistry Vol. 10; p. 969698
Main Authors Ameen, Shahzad, Murtaza, Maida, Arshad, Muhammad, Alhodaib, Aiyeshah, Waseem, Amir
Format Journal Article
LanguageEnglish
Published Frontiers Media S.A 08.12.2022
Subjects
Chemistry
dyes
lanthanum nickelate
photocatalysis
silver phosphate
water pollution
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Abstract Pristine lanthanum nickelate (LaNiO 3 ), silver phosphate (Ag 3 PO 4 ) and perovskite lanthanum nickelate silver phosphate composites (LaNiO 3 /Ag 3 PO 4 ) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO 3 in Ag 3 PO 4 . The physical properties of as-prepared samples were studied by powder X-ray diffraction (pXRD), Fourier-transform infrared (FT-IR), Scanning electron microscopy (SEM) and Energy-dispersive X-ray (EDX). Among all synthesized photocatalysts, 5%LaNiO 3 /Ag 3 PO 4 composite has been proved to be an excellent visible light photocatalyst for the degradation of dyes i.e., rhodamine B (RhB) and methyl orange (MO). The photocatalytic activity and stability of Ag 3 PO 4 were also enhanced by introducing LaNiO 3 in Ag 3 PO 4 heterojunction formation. Complete photodegradation of 50 mg/L of RhB and MO solutions using 25 mg of 5%LaNiO 3 /Ag 3 PO 4 photocatalyst was observed in just 20 min. Photodegradation of RhB and MO using 5%LaNiO 3 /Ag 3 PO 4 catalyst follows first-order kinetics with rate constants of 0.213 and 0.1804 min −1 , respectively. Perovskite LaNiO 3 /Ag 3 PO 4 photocatalyst showed the highest stability up to five cycles. The photodegradation mechanism suggests that the holes ( h + ) and superoxide anion radicals O 2   • − plays a main role in the dye degradation of RhB and MO.
AbstractList Pristine lanthanum nickelate (LaNiO3), silver phosphate (Ag3PO4) and perovskite lanthanum nickelate silver phosphate composites (LaNiO3/Ag3PO4) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO3 in Ag3PO4. The physical properties of as-prepared samples were studied by powder X-ray diffraction (pXRD), Fourier-transform infrared (FT-IR), Scanning electron microscopy (SEM) and Energy-dispersive X-ray (EDX). Among all synthesized photocatalysts, 5%LaNiO3/Ag3PO4 composite has been proved to be an excellent visible light photocatalyst for the degradation of dyes i.e., rhodamine B (RhB) and methyl orange (MO). The photocatalytic activity and stability of Ag3PO4 were also enhanced by introducing LaNiO3 in Ag3PO4 heterojunction formation. Complete photodegradation of 50 mg/L of RhB and MO solutions using 25 mg of 5%LaNiO3/Ag3PO4 photocatalyst was observed in just 20 min. Photodegradation of RhB and MO using 5%LaNiO3/Ag3PO4 catalyst follows first-order kinetics with rate constants of 0.213 and 0.1804 min−1, respectively. Perovskite LaNiO3/Ag3PO4 photocatalyst showed the highest stability up to five cycles. The photodegradation mechanism suggests that the holes (h+) and superoxide anion radicals O2 •− plays a main role in the dye degradation of RhB and MO.
Pristine lanthanum nickelate (LaNiO3), silver phosphate (Ag3PO4) and perovskite lanthanum nickelate silver phosphate composites (LaNiO3/Ag3PO4) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO3 in Ag3PO4. The physical properties of as-prepared samples were studied by powder X-ray diffraction (pXRD), Fourier-transform infrared (FT-IR), Scanning electron microscopy (SEM) and Energy-dispersive X-ray (EDX). Among all synthesized photocatalysts, 5%LaNiO3/Ag3PO4 composite has been proved to be an excellent visible light photocatalyst for the degradation of dyes i.e., rhodamine B (RhB) and methyl orange (MO). The photocatalytic activity and stability of Ag3PO4 were also enhanced by introducing LaNiO3 in Ag3PO4 heterojunction formation. Complete photodegradation of 50 mg/L of RhB and MO solutions using 25 mg of 5%LaNiO3/Ag3PO4 photocatalyst was observed in just 20 min. Photodegradation of RhB and MO using 5%LaNiO3/Ag3PO4 catalyst follows first-order kinetics with rate constants of 0.213 and 0.1804 min-1, respectively. Perovskite LaNiO3/Ag3PO4 photocatalyst showed the highest stability up to five cycles. The photodegradation mechanism suggests that the holes ( h +) and superoxide anion radicals O 2   • - plays a main role in the dye degradation of RhB and MO.Pristine lanthanum nickelate (LaNiO3), silver phosphate (Ag3PO4) and perovskite lanthanum nickelate silver phosphate composites (LaNiO3/Ag3PO4) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO3 in Ag3PO4. The physical properties of as-prepared samples were studied by powder X-ray diffraction (pXRD), Fourier-transform infrared (FT-IR), Scanning electron microscopy (SEM) and Energy-dispersive X-ray (EDX). Among all synthesized photocatalysts, 5%LaNiO3/Ag3PO4 composite has been proved to be an excellent visible light photocatalyst for the degradation of dyes i.e., rhodamine B (RhB) and methyl orange (MO). The photocatalytic activity and stability of Ag3PO4 were also enhanced by introducing LaNiO3 in Ag3PO4 heterojunction formation. Complete photodegradation of 50 mg/L of RhB and MO solutions using 25 mg of 5%LaNiO3/Ag3PO4 photocatalyst was observed in just 20 min. Photodegradation of RhB and MO using 5%LaNiO3/Ag3PO4 catalyst follows first-order kinetics with rate constants of 0.213 and 0.1804 min-1, respectively. Perovskite LaNiO3/Ag3PO4 photocatalyst showed the highest stability up to five cycles. The photodegradation mechanism suggests that the holes ( h +) and superoxide anion radicals O 2   • - plays a main role in the dye degradation of RhB and MO.
Pristine lanthanum nickelate (LaNiO 3 ), silver phosphate (Ag 3 PO 4 ) and perovskite lanthanum nickelate silver phosphate composites (LaNiO 3 /Ag 3 PO 4 ) were prepared using the facile hydrothermal method. Three composites were synthesized by varying the percentage of LaNiO 3 in Ag 3 PO 4 . The physical properties of as-prepared samples were studied by powder X-ray diffraction (pXRD), Fourier-transform infrared (FT-IR), Scanning electron microscopy (SEM) and Energy-dispersive X-ray (EDX). Among all synthesized photocatalysts, 5%LaNiO 3 /Ag 3 PO 4 composite has been proved to be an excellent visible light photocatalyst for the degradation of dyes i.e., rhodamine B (RhB) and methyl orange (MO). The photocatalytic activity and stability of Ag 3 PO 4 were also enhanced by introducing LaNiO 3 in Ag 3 PO 4 heterojunction formation. Complete photodegradation of 50 mg/L of RhB and MO solutions using 25 mg of 5%LaNiO 3 /Ag 3 PO 4 photocatalyst was observed in just 20 min. Photodegradation of RhB and MO using 5%LaNiO 3 /Ag 3 PO 4 catalyst follows first-order kinetics with rate constants of 0.213 and 0.1804 min −1 , respectively. Perovskite LaNiO 3 /Ag 3 PO 4 photocatalyst showed the highest stability up to five cycles. The photodegradation mechanism suggests that the holes ( h + ) and superoxide anion radicals O 2   • − plays a main role in the dye degradation of RhB and MO.
Author Arshad, Muhammad
Waseem, Amir
Ameen, Shahzad
Alhodaib, Aiyeshah
Murtaza, Maida
AuthorAffiliation 1 Department of Chemistry , Quaid-i-Azam University , Islamabad , Pakistan
3 Department of Physics , College of Science , Qassim University , Buraydah , Saudi Arabia
2 Nanosciences and Technology Department , National Centre for Physics (NCP) , Quaid-i-Azam University (QAU) Campus , Islamabad , Pakistan
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This article was submitted to Photocatalysis and Photochemistry, a section of the journal Frontiers in Chemistry
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Snippet Pristine lanthanum nickelate (LaNiO 3 ), silver phosphate (Ag 3 PO 4 ) and perovskite lanthanum nickelate silver phosphate composites (LaNiO 3 /Ag 3 PO 4 )...
Pristine lanthanum nickelate (LaNiO3), silver phosphate (Ag3PO4) and perovskite lanthanum nickelate silver phosphate composites (LaNiO3/Ag3PO4) were prepared...
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StartPage 969698
SubjectTerms Chemistry
dyes
lanthanum nickelate
photocatalysis
silver phosphate
water pollution
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Title Perovskite LaNiO3/Ag3PO4 heterojunction photocatalyst for the degradation of dyes
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Volume 10
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