Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides
Iron-based superconductors all share the same building blocks. So why do local magnetic properties vary from one compound to another? A new theoretical model explains the variation in physical properties and links it to the structural differences, providing a description for a wide range of material...
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| Published in | Nature materials Vol. 10; no. 12; pp. 932 - 935 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.12.2011
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Iron-based superconductors all share the same building blocks. So why do local magnetic properties vary from one compound to another? A new theoretical model explains the variation in physical properties and links it to the structural differences, providing a description for a wide range of materials.
The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity
1
. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (
T
c
). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available
2
. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments
3
. |
|---|---|
| AbstractList | Iron-based superconductors all share the same building blocks. So why do local magnetic properties vary from one compound to another? A new theoretical model explains the variation in physical properties and links it to the structural differences, providing a description for a wide range of materials.
The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity
1
. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (
T
c
). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available
2
. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments
3
. The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (T(c)). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments. [PUBLICATION ABSTRACT] The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (T(c)). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments.The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (T(c)). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments. The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (T sub(c)). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments. The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all share the same basic building blocks, but there is significant variation in their physical properties, such as magnetic ordered moments, effective masses, superconducting gaps and transition temperature (T(c)). Many theoretical techniques have been applied to individual compounds but no consistent description of the microscopic origin of these variations is available. Here we carry out a comparative theoretical study of a large number of iron-based compounds in both their magnetic and paramagnetic states. Taking into account correlation effects and realistic band structures, we describe well the trends in all of the physical properties such as the ordered moments, effective masses and Fermi surfaces across all families of iron compounds, and find them to be in good agreement with experiments. We trace variation in physical properties to variations in the key structural parameters, rather than changes in the screening of the Coulomb interactions. Our results also provide a natural explanation of the strongly Fermi-surface-dependent superconducting gaps observed in experiments. |
| Author | Kotliar, G. Haule, K. Yin, Z. P. |
| Author_xml | – sequence: 1 givenname: Z. P. surname: Yin fullname: Yin, Z. P. email: yinzping@physics.rutgers.edu organization: Department of Physics and Astronomy, Rutgers University, Department of Physics and Astronomy, Stony Brook University – sequence: 2 givenname: K. surname: Haule fullname: Haule, K. organization: Department of Physics and Astronomy, Rutgers University – sequence: 3 givenname: G. surname: Kotliar fullname: Kotliar, G. organization: Department of Physics and Astronomy, Rutgers University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/21927004$$D View this record in MEDLINE/PubMed |
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| Copyright | Springer Nature Limited 2011 Copyright Nature Publishing Group Dec 2011 |
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| Snippet | Iron-based superconductors all share the same building blocks. So why do local magnetic properties vary from one compound to another? A new theoretical model... The iron pnictide and chalcogenide compounds are a subject of intensive investigations owing to their surprisingly high temperature superconductivity. They all... |
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| SubjectTerms | 639/301/119/997 639/638/298/924 Band structure of solids Biomaterials Chalcogenides Chemistry and Materials Science Condensed Matter Physics Gaps High temperature Iron Iron compounds Kinetics letter Materials Science Nanotechnology Optical and Electronic Materials Physical properties Superconductivity Superconductors Transition temperature Transition temperatures |
| Title | Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides |
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