Ultrathin two-dimensional layered metal hydroxides: an emerging platform for advanced catalysis, energy conversion and storage
The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered metal hydroxides (LMHs) are increasingly being recognized as an important category in 2D nanomaterials, and the corresponding research has been...
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| Published in | Chemical Society reviews Vol. 45; no. 18; pp. 4873 - 4891 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
England
21.09.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered metal hydroxides (LMHs) are increasingly being recognized as an important category in 2D nanomaterials, and the corresponding research has been experiencing a significant renaissance. Due to the flexible tunability of metal ions, their naturally positively charged plane and 2D anisotropy with nanometre thickness, ultrathin LMHs and their derived hybrids have shown exciting perspectives in many fields, such as catalysis, and energy storage and conversion. As for practical application, ultrathin 2D LMHs have exhibited high performances in electrocatalysis (
e.g.
the hydrogen and oxygen evolution reactions), photocatalysis and supercapacitors. In particular, hybrid materials based on ultrathin LMHs have proven to further improve the catalytic performance by synergistic effects derived from the hybrid interfaces. Nevertheless, studies on ultrathin LMHs are still in the infant stage and lag far behind other important 2D nanomaterials. Hence, it is essential to update the reported work in this emerging research area. In this tutorial review, we aim to summarize recent developments in ultrathin LMHs and their derived hybrids. The quite dispersed literature regarding ultrathin LMH-based materials is classified under the framework of catalysis- and energy-related properties and applications.
The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. |
|---|---|
| AbstractList | The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered metal hydroxides (LMHs) are increasingly being recognized as an important category in 2D nanomaterials, and the corresponding research has been experiencing a significant renaissance. Due to the flexible tunability of metal ions, their naturally positively charged plane and 2D anisotropy with nanometre thickness, ultrathin LMHs and their derived hybrids have shown exciting perspectives in many fields, such as catalysis, and energy storage and conversion. As for practical application, ultrathin 2D LMHs have exhibited high performances in electrocatalysis (e.g. the hydrogen and oxygen evolution reactions), photocatalysis and supercapacitors. In particular, hybrid materials based on ultrathin LMHs have proven to further improve the catalytic performance by synergistic effects derived from the hybrid interfaces. Nevertheless, studies on ultrathin LMHs are still in the infant stage and lag far behind other important 2D nanomaterials. Hence, it is essential to update the reported work in this emerging research area. In this tutorial review, we aim to summarize recent developments in ultrathin LMHs and their derived hybrids. The quite dispersed literature regarding ultrathin LMH-based materials is classified under the framework of catalysis- and energy-related properties and applications. The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered metal hydroxides (LMHs) are increasingly being recognized as an important category in 2D nanomaterials, and the corresponding research has been experiencing a significant renaissance. Due to the flexible tunability of metal ions, their naturally positively charged plane and 2D anisotropy with nanometre thickness, ultrathin LMHs and their derived hybrids have shown exciting perspectives in many fields, such as catalysis, and energy storage and conversion. As for practical application, ultrathin 2D LMHs have exhibited high performances in electrocatalysis ( e.g. the hydrogen and oxygen evolution reactions), photocatalysis and supercapacitors. In particular, hybrid materials based on ultrathin LMHs have proven to further improve the catalytic performance by synergistic effects derived from the hybrid interfaces. Nevertheless, studies on ultrathin LMHs are still in the infant stage and lag far behind other important 2D nanomaterials. Hence, it is essential to update the reported work in this emerging research area. In this tutorial review, we aim to summarize recent developments in ultrathin LMHs and their derived hybrids. The quite dispersed literature regarding ultrathin LMH-based materials is classified under the framework of catalysis- and energy-related properties and applications. The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered metal hydroxides (LMHs) are increasingly being recognized as an important category in 2D nanomaterials, and the corresponding research has been experiencing a significant renaissance. Due to the flexible tunability of metal ions, their naturally positively charged plane and 2D anisotropy with nanometre thickness, ultrathin LMHs and their derived hybrids have shown exciting perspectives in many fields, such as catalysis, and energy storage and conversion. As for practical application, ultrathin 2D LMHs have exhibited high performances in electrocatalysis ( e.g. the hydrogen and oxygen evolution reactions), photocatalysis and supercapacitors. In particular, hybrid materials based on ultrathin LMHs have proven to further improve the catalytic performance by synergistic effects derived from the hybrid interfaces. Nevertheless, studies on ultrathin LMHs are still in the infant stage and lag far behind other important 2D nanomaterials. Hence, it is essential to update the reported work in this emerging research area. In this tutorial review, we aim to summarize recent developments in ultrathin LMHs and their derived hybrids. The quite dispersed literature regarding ultrathin LMH-based materials is classified under the framework of catalysis- and energy-related properties and applications. The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. |
| Author | Tang, Zhiyong Yin, Huajie |
| AuthorAffiliation | National Center for Nanoscience and Technology CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in Nanoscience |
| AuthorAffiliation_xml | – sequence: 0 name: CAS Center for Excellence in Nanoscience – sequence: 0 name: National Center for Nanoscience and Technology – sequence: 0 name: CAS Key Laboratory of Nanosystem and Hierarchical Fabrication |
| Author_xml | – sequence: 1 givenname: Huajie surname: Yin fullname: Yin, Huajie – sequence: 2 givenname: Zhiyong surname: Tang fullname: Tang, Zhiyong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27373467$$D View this record in MEDLINE/PubMed |
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| Notes | Huajie Yin obtained his PhD degree from the National Center for Nanoscience and Technology and Tsinghua University in 2015 under the direction of Prof. Zhiyong Tang. He is now working as a postdoctoral research fellow at Griffith University. His main research interests are focused on two-dimensional materials and related applications in electrocatalysis, energy storage and conversion. Dr Zhiyong Tang obtained his PhD degree from the Chinese Academy of Sciences in 2000 under the direction of Prof. Erkang Wang. After finishing his postdoctoral training at both the Swiss Federal Institute of Technology, Zurich, and the University of Michigan, he returned to China and took a position as a professor at the National Center for Nanoscience and Technology at the end of 2006. His main research interests are focused on the preparation, assembly and application of functional inorganic nanomaterials in the field of energy. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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| Snippet | The unique properties of graphene are triggering a great deal of attention toward the family of ultrathin two-dimensional (2D) structures. Ultrathin layered... |
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| SubjectTerms | anisotropy Catalysis Categories energy conversion Graphene hydrogen hydroxides Infants Metal hydroxides metal ions Nanomaterials Nanostructure oxygen production photocatalysis synergism Two dimensional |
| Title | Ultrathin two-dimensional layered metal hydroxides: an emerging platform for advanced catalysis, energy conversion and storage |
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