The Ising triangular-lattice antiferromagnet neodymium heptatantalate as a quantum spin liquid candidate

Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model, while additional non-commuting exchange terms were proposed to induce its quantum versi...

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Published inNature materials Vol. 21; no. 4; pp. 416 - 422
Main Authors Arh, T., Sana, B., Pregelj, M., Khuntia, P., Jagličić, Z., Le, M. D., Biswas, P. K., Manuel, P., Mangin-Thro, L., Ozarowski, A., Zorko, A.
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 01.04.2022
Nature Publishing Group
Subjects
639/301/119/997
639/766/119/997
Anisotropy
Antiferromagnetism
Biomaterials
Chemistry and Materials Science
Commuting
Condensed Matter Physics
Electron paramagnetic resonance
Electron spin
Ising model
Liquid phases
Liquids
Magnetic anisotropy
Magnetism
Materials Science
Nanotechnology
Neodymium
Neutron scattering
Optical and Electronic Materials
Orbital stability
Rare earth elements
Resonance scattering
Spin liquid
Spin resonance
Spin-orbit interactions
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Abstract Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model, while additional non-commuting exchange terms were proposed to induce its quantum version—a quantum spin liquid. However, these predictions have not yet been confirmed experimentally. Here, we report evidence for such a state in the triangular-lattice antiferromagnet NdTa 7 O 19 . We determine its magnetic ground state, which is characterized by effective spin-1/2 degrees of freedom with Ising-like nearest-neighbour correlations and gives rise to spin excitations persisting down to the lowest accessible temperature of 40 mK. Our study demonstrates the key role of strong spin–orbit coupling in stabilizing spin liquids that result from magnetic anisotropy and highlights the large family of rare-earth (RE) heptatantalates RETa 7 O 19 as a framework for realization of these states, which represent a promising platform for quantum applications. Neutron scattering, electron spin resonance, muon spectroscopy and magnetization measurements are applied to evidence a quantum spin liquid phase in NdTa 7 O 19 .
AbstractList Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model, while additional non-commuting exchange terms were proposed to induce its quantum version—a quantum spin liquid. However, these predictions have not yet been confirmed experimentally. Here, we report evidence for such a state in the triangular-lattice antiferromagnet NdTa 7 O 19 . We determine its magnetic ground state, which is characterized by effective spin-1/2 degrees of freedom with Ising-like nearest-neighbour correlations and gives rise to spin excitations persisting down to the lowest accessible temperature of 40 mK. Our study demonstrates the key role of strong spin–orbit coupling in stabilizing spin liquids that result from magnetic anisotropy and highlights the large family of rare-earth (RE) heptatantalates RETa 7 O 19 as a framework for realization of these states, which represent a promising platform for quantum applications. Neutron scattering, electron spin resonance, muon spectroscopy and magnetization measurements are applied to evidence a quantum spin liquid phase in NdTa 7 O 19 .
Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model, while additional non-commuting exchange terms were proposed to induce its quantum version—a quantum spin liquid. However, these predictions have not yet been confirmed experimentally. Here, we report evidence for such a state in the triangular-lattice antiferromagnet NdTa7O19. We determine its magnetic ground state, which is characterized by effective spin-1/2 degrees of freedom with Ising-like nearest-neighbour correlations and gives rise to spin excitations persisting down to the lowest accessible temperature of 40 mK. Our study demonstrates the key role of strong spin–orbit coupling in stabilizing spin liquids that result from magnetic anisotropy and highlights the large family of rare-earth (RE) heptatantalates RETa7O19 as a framework for realization of these states, which represent a promising platform for quantum applications.Neutron scattering, electron spin resonance, muon spectroscopy and magnetization measurements are applied to evidence a quantum spin liquid phase in NdTa7O19.
Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model, while additional non-commuting exchange terms were proposed to induce its quantum version-a quantum spin liquid. However, these predictions have not yet been confirmed experimentally. Here, we report evidence for such a state in the triangular-lattice antiferromagnet NdTa O . We determine its magnetic ground state, which is characterized by effective spin-1/2 degrees of freedom with Ising-like nearest-neighbour correlations and gives rise to spin excitations persisting down to the lowest accessible temperature of 40 mK. Our study demonstrates the key role of strong spin-orbit coupling in stabilizing spin liquids that result from magnetic anisotropy and highlights the large family of rare-earth (RE) heptatantalates RETa O as a framework for realization of these states, which represent a promising platform for quantum applications.
Author Khuntia, P.
Pregelj, M.
Mangin-Thro, L.
Ozarowski, A.
Jagličić, Z.
Biswas, P. K.
Le, M. D.
Manuel, P.
Zorko, A.
Arh, T.
Sana, B.
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Snippet Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was...
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SubjectTerms 639/301/119/997
639/766/119/997
Anisotropy
Antiferromagnetism
Biomaterials
Chemistry and Materials Science
Commuting
Condensed Matter Physics
Electron paramagnetic resonance
Electron spin
Ising model
Liquid phases
Liquids
Magnetic anisotropy
Magnetism
Materials Science
Nanotechnology
Neodymium
Neutron scattering
Optical and Electronic Materials
Orbital stability
Rare earth elements
Resonance scattering
Spin liquid
Spin resonance
Spin-orbit interactions
Title The Ising triangular-lattice antiferromagnet neodymium heptatantalate as a quantum spin liquid candidate
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https://www.ncbi.nlm.nih.gov/pubmed/34969994
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