Study of the resistances to transfer of gaseous pollutant between material and indoor air
The main parameters which control the emission of volatile organic compounds between wall materials and indoor air were examined. A physically based model considers that the global emission phenomenon results from three elementary physical phenomena: diffusion through the boundary layer separating t...
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Published in | Building and environment Vol. 46; no. 2; pp. 356 - 362 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
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01.02.2011
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Abstract | The main parameters which control the emission of volatile organic compounds between wall materials and indoor air were examined. A physically based model considers that the global emission phenomenon results from three elementary physical phenomena: diffusion through the boundary layer separating the wall from environment, diffusion within the porous network of the materials, and sorption of the gas molecules on the active sites of the materials. The pollutant transfer between porous material and air is therefore subjected to two complementary resistances and we identify first the resistance which controls the transfer. Then, we predict the global emission time constant from the mass transfer coefficient of convection and the thickness of the material. Experimental results from a small scale chamber are compared to predicted values in the case of acetone emission from chipboard in humid air and for high initial acetone concentration. Good agreement is obtained at the beginning of emission but an acetone retention effect by chipboard is observed, showing that it will be necessary to take into account the interactions of water vapor with materials and the pollutants to achieve accurate modeling of the material VOC emission process. |
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AbstractList | The main parameters which control the emission of volatile organic compounds between wall materials and indoor air were examined. A physically based model considers that the global emission phenomenon results from three elementary physical phenomena: diffusion through the boundary layer separating the wall from environment, diffusion within the porous network of the materials, and sorption of the gas molecules on the active sites of the materials. The pollutant transfer between porous material and air is therefore subjected to two complementary resistances and we identify first the resistance which controls the transfer. Then, we predict the global emission time constant from the mass transfer coefficient of convection and the thickness of the material. Experimental results from a small scale chamber are compared to predicted values in the case of acetone emission from chipboard in humid air and for high initial acetone concentration. Good agreement is obtained at the beginning of emission but an acetone retention effect by chipboard is observed, showing that it will be necessary to take into account the interactions of water vapor with materials and the pollutants to achieve accurate modeling of the material VOC emission process. |
Author | Marion, Michaël Tiffonnet, Anne Lise Makhloufi, Rachid Santa-Cruz, Alina |
Author_xml | – sequence: 1 givenname: Michaël surname: Marion fullname: Marion, Michaël email: michael.marion@unicaen.fr organization: IUT Cherbourg-Manche, Département GTE, 120, Rue de l’exode – 50000 Saint-Lô, France – sequence: 2 givenname: Anne Lise surname: Tiffonnet fullname: Tiffonnet, Anne Lise organization: IUT Cherbourg-Manche, Département GTE, 120, Rue de l’exode – 50000 Saint-Lô, France – sequence: 3 givenname: Alina surname: Santa-Cruz fullname: Santa-Cruz, Alina organization: Laboratoire Universitaire des Sciences Appliquées de Cherbourg (LUSAC, EA 4253), Site Universitaire, BP 78– 50130 Octeville, France – sequence: 4 givenname: Rachid surname: Makhloufi fullname: Makhloufi, Rachid organization: Laboratoire Universitaire des Sciences Appliquées de Cherbourg (LUSAC, EA 4253), Site Universitaire, BP 78– 50130 Octeville, France |
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Cites_doi | 10.1016/S0360-1323(97)00060-7 10.1034/j.1600-0668.2003.00208.x 10.1016/S1352-2310(03)00160-2 10.1016/S0360-1323(01)00089-0 10.1111/j.1600-0668.2005.00421.x 10.1016/j.buildenv.2003.10.005 10.1016/0021-9517(86)90176-4 10.3763/aber.2008.0203 10.1016/S0360-1323(03)00064-7 10.1016/j.buildenv.2006.03.003 10.1111/j.1600-0668.1991.04-12.x 10.1016/S0017-9310(03)00352-1 10.1177/1420326X0201100204 10.1016/S0017-9310(03)00012-7 10.1016/j.atmosenv.2006.11.022 10.1016/j.buildenv.2006.10.002 |
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Keywords | Volatile organic compounds Sorption Air quality Mass transfer Theoretical study Indoor pollution Volatile organic compound Pollutant emission Modeling |
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contributor: fullname: Hartley – year: 1995 ident: 10.1016/j.buildenv.2010.07.029_bib20 contributor: fullname: Bejan |
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SubjectTerms | Acetone Air quality Applied sciences Buildings. Public works Diffusion Diffusion layers Emission Engineering Sciences Environmental Sciences Exact sciences and technology Indoor Mass transfer Materials Mathematical models Physics Pollutants Pollution indoor buildings Reactive fluid environment Sorption Volatile organic compounds Walls |
Title | Study of the resistances to transfer of gaseous pollutant between material and indoor air |
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