Magnetic resonance imaging techniques for lithium-ion batteries: Principles and applications

Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overvie...

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Published inMagnetic resonance letters Vol. 4; no. 2; p. 200113
Main Authors Lin, Hongxin, Jin, Yanting, Tao, Mingming, Zhou, Yingao, Shan, Peizhao, Zhao, Danhui, Yang, Yong
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.05.2024
KeAi Communications Co. Ltd
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Abstract Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs. [Display omitted]
AbstractList Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs.
Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs. [Display omitted]
ArticleNumber 200113
Author Zhao, Danhui
Tao, Mingming
Jin, Yanting
Lin, Hongxin
Shan, Peizhao
Zhou, Yingao
Yang, Yong
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Issue 2
Keywords Lithium-ion batteries
Electrodes
Magnetic resonance imaging (MRI)
Electrolytes
Commercial batteries
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Snippet Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive,...
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SubjectTerms Commercial batteries
Electrodes
Electrolytes
Lithium-ion batteries
Magnetic resonance imaging (MRI)
Title Magnetic resonance imaging techniques for lithium-ion batteries: Principles and applications
URI https://dx.doi.org/10.1016/j.mrl.2024.200113
https://doaj.org/article/7d78687c1f764a98a88f3a0960855de2
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