Magnetic resonance imaging techniques for lithium-ion batteries: Principles and applications
Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overvie...
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Published in | Magnetic resonance letters Vol. 4; no. 2; p. 200113 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
01.05.2024
KeAi Communications Co. Ltd |
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Abstract | Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs.
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AbstractList | Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs. Operando monitoring of internal and local electrochemical processes within lithium-ion batteries (LIBs) is crucial, necessitating a range of non-invasive, real-time imaging characterization techniques including nuclear magnetic resonance (NMR) techniques. This review provides a comprehensive overview of the recent applications and advancements of non-invasive magnetic resonance imaging (MRI) techniques in LIBs. It initially introduces the principles and hardware of MRI, followed by a detailed summary and comparison of MRI techniques used for characterizing liquid/solid electrolytes, electrodes and commercial batteries. This encompasses the determination of electrolytes' transport properties, acquisition of ion distribution profile, and diagnosis of battery defects. By focusing on experimental parameters and optimization strategies, our goal is to explore MRI methods suitable to a variety of research subjects, aiming to enhance imaging quality across diverse scenarios and offer critical physical/chemical insights into the ongoing operation processes of LIBs. [Display omitted] |
ArticleNumber | 200113 |
Author | Zhao, Danhui Tao, Mingming Jin, Yanting Lin, Hongxin Shan, Peizhao Zhou, Yingao Yang, Yong |
Author_xml | – sequence: 1 givenname: Hongxin surname: Lin fullname: Lin, Hongxin organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 2 givenname: Yanting surname: Jin fullname: Jin, Yanting organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 3 givenname: Mingming surname: Tao fullname: Tao, Mingming organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 4 givenname: Yingao surname: Zhou fullname: Zhou, Yingao organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 5 givenname: Peizhao surname: Shan fullname: Shan, Peizhao organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 6 givenname: Danhui surname: Zhao fullname: Zhao, Danhui organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China – sequence: 7 givenname: Yong surname: Yang fullname: Yang, Yong email: yyang@xmu.edu.cn organization: State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials and Department of Chemistry, College of Chemistry and Chemical Engineering, Tan Kah Kee Innovation Laboratory (IKKEM), Xiamen University, Xiamen, 361005, China |
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Keywords | Lithium-ion batteries Electrodes Magnetic resonance imaging (MRI) Electrolytes Commercial batteries |
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