Strontium isotopes as tracers of water-rocks interactions, mixing processes and residence time indicator of groundwater within the granite-carbonate coastal aquifer of Bonifacio (Corsica, France)
This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonate coastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer of Bonifacio (southern Corsica, France) mainly composed of continental graniti...
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| Published in | The Science of the total environment Vol. 573; pp. 233 - 246 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
15.12.2016
Elsevier |
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| Online Access | Get full text |
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| Abstract | This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonate coastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer of Bonifacio (southern Corsica, France) mainly composed of continental granitic weathering products and marine calcarenite sediments filling a granitic depression. A multi-tracer approach combining physico-chemical parameters, major ions, selected trace elements, stable isotopes of the water molecule and 87Sr/86Sr ratios measurements is undertaken for 20 groundwater samples during the low water period in November 2014. 5 rock samples of the sedimentary deposits and surrounding granites are also analysed. First, the water-rock interactions processes governing the groundwater mineralization are described in order to fix the hydrogeochemical background. Secondly, the flow conditions are refined through the quantification of inter aquifer levels mixing, and thirdly, the kinetics of water-rock interaction based on groundwater residence time from a previous study using CFCs and SF6 are quantified for the two main flow lines. A regional contrast in the groundwater recharge altitude allowed the oxygene-18 to be useful combined with the 87Sr/86Sr ratios to differentiate the groundwater origins and to compute the mixing rates, revealing the real extension of the watershed and the availability of the resource. The results also highlight a very good correlation between the groundwater residence time and the spatial evolution of 87Sr/86Sr ratios, allowing water-rock interaction kinetics to be defined empirically for the two main flow lines through the calcarenites. These results demonstrate the efficiency of strontium isotopes as tracers of water-rock interaction kinetics and by extension their relevance as a proxy of groundwater residence time, fundamental parameter documenting the long term sustainability of the hydrosystem.
[Display omitted]
•Strontium and major ions are used to define groundwater mineralization processes.•Granites and calcarenites are complex sources of Sr2+.•The 87Sr/86Sr vs δ18O approach is relevant to assess groundwater mixings.•The 87Sr/86Sr ratio is suitable to quantify water-rocks interaction kinetics. |
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| AbstractList | This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonate coastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer of Bonifacio (southern Corsica, France) mainly composed of continental granitic weathering products and marine calcarenite sediments filling a granitic depression. A multi-tracer approach combining physico-chemical parameters, major ions, selected trace elements, stable isotopes of the water molecule and 87Sr/86Sr ratios measurements is undertaken for 20 groundwater samples during the low water period in November 2014. 5 rock samples of the sedimentary deposits and surrounding granites are also analysed. First, the water-rock interactions processes governing the groundwater mineralization are described in order to fix the hydrogeochemical background. Secondly, the flow conditions are refined through the quantification of inter aquifer levels mixing, and thirdly, the kinetics of water-rock interaction based on groundwater residence time from a previous study using CFCs and SF6 are quantified for the two main flow lines. A regional contrast in the groundwater recharge altitude allowed the oxygene-18 to be useful combined with the 87Sr/86Sr ratios to differentiate the groundwater origins and to compute the mixing rates, revealing the real extension of the watershed and the availability of the resource. The results also highlight a very good correlation between the groundwater residence time and the spatial evolution of 87Sr/86Sr ratios, allowing water-rock interaction kinetics to be defined empirically for the two main flow lines through the calcarenites. These results demonstrate the efficiency of strontium isotopes as tracers of water-rock interaction kinetics and by extension their relevance as a proxy of groundwater residence time, fundamental parameter documenting the long term sustainability of the hydrosystem. This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonate coastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer of Bonifacio (southern Corsica, France) mainly composed of continental granitic weathering products and marine calcarenite sediments filling a granitic depression. A multi-tracer approach combining physico-chemical parameters, major ions, selected trace elements, stable isotopes of the water molecule and 87Sr/86Sr ratios measurements is undertaken for 20 groundwater samples during the low water period in November 2014. 5 rock samples of the sedimentary deposits and surrounding granites are also analysed. First, the water-rock interactions processes governing the groundwater mineralization are described in order to fix the hydrogeochemical background. Secondly, the flow conditions are refined through the quantification of inter aquifer levels mixing, and thirdly, the kinetics of water-rock interaction based on groundwater residence time from a previous study using CFCs and SF6 are quantified for the two main flow lines. A regional contrast in the groundwater recharge altitude allowed the oxygene-18 to be useful combined with the 87Sr/86Sr ratios to differentiate the groundwater origins and to compute the mixing rates, revealing the real extension of the watershed and the availability of the resource. The results also highlight a very good correlation between the groundwater residence time and the spatial evolution of 87Sr/86Sr ratios, allowing water-rock interaction kinetics to be defined empirically for the two main flow lines through the calcarenites. These results demonstrate the efficiency of strontium isotopes as tracers of water-rock interaction kinetics and by extension their relevance as a proxy of groundwater residence time, fundamental parameter documenting the long term sustainability of the hydrosystem. [Display omitted] •Strontium and major ions are used to define groundwater mineralization processes.•Granites and calcarenites are complex sources of Sr2+.•The 87Sr/86Sr vs δ18O approach is relevant to assess groundwater mixings.•The 87Sr/86Sr ratio is suitable to quantify water-rocks interaction kinetics. This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonatecoastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer ofBonifacio (southern Corsica, France) mainly composed of continental granitic weathering products and marinecalcarenite sediments filling a granitic depression. A multi-tracer approach combining physico-chemical parameters,major ions, selected trace elements, stable isotopes of the water molecule and 87Sr/86Sr ratios measurementsis undertaken for 20 groundwater samples during the low water period in November 2014. 5 rocksamples of the sedimentary deposits and surrounding granites are also analysed. First, the water-rock interactionsprocesses governing the groundwater mineralization are described in order to fix the hydrogeochemicalbackground. Secondly, the flow conditions are refined through the quantification of inter aquifer levels mixing,and thirdly, the kinetics of water-rock interaction based on groundwater residence time from a previous studyusing CFCs and SF6 are quantified for the two main flow lines. A regional contrast in the groundwater rechargealtitude allowed the oxygene-18 to be useful combinedwith the 87Sr/86Sr ratios to differentiate the groundwaterorigins and to compute the mixing rates, revealing the real extension of the watershed and the availability of theresource. The results also highlight a very good correlation between the groundwater residence time and the spatial evolution of 87Sr/86Sr ratios, allowingwater-rock interaction kinetics to be defined empirically for the twomain flowlines through the calcarenites. These results demonstrate the efficiency of strontiumisotopes as tracersof water-rock interaction kinetics and by extension their relevance as a proxy of groundwater residence time,fundamental parameter documenting the long term sustainability of the hydrosystem. This study aims at identifying the water-rock interactions and mixing rates within a complex granite-carbonate coastal aquifer under high touristic pressure. Investigations have been carried out within the coastal aquifer of Bonifacio (southern Corsica, France) mainly composed of continental granitic weathering products and marine calcarenite sediments filling a granitic depression. A multi-tracer approach combining physico-chemical parameters, major ions, selected trace elements, stable isotopes of the water molecule and Sr/ Sr ratios measurements is undertaken for 20 groundwater samples during the low water period in November 2014. 5 rock samples of the sedimentary deposits and surrounding granites are also analysed. First, the water-rock interactions processes governing the groundwater mineralization are described in order to fix the hydrogeochemical background. Secondly, the flow conditions are refined through the quantification of inter aquifer levels mixing, and thirdly, the kinetics of water-rock interaction based on groundwater residence time from a previous study using CFCs and SF are quantified for the two main flow lines. A regional contrast in the groundwater recharge altitude allowed the oxygene-18 to be useful combined with the Sr/ Sr ratios to differentiate the groundwater origins and to compute the mixing rates, revealing the real extension of the watershed and the availability of the resource. The results also highlight a very good correlation between the groundwater residence time and the spatial evolution of Sr/ Sr ratios, allowing water-rock interaction kinetics to be defined empirically for the two main flow lines through the calcarenites. These results demonstrate the efficiency of strontium isotopes as tracers of water-rock interaction kinetics and by extension their relevance as a proxy of groundwater residence time, fundamental parameter documenting the long term sustainability of the hydrosystem. |
| Author | Vergnaud-Ayraud, V. Labasque, T. Huneau, F. Aquilina, L. Celle-Jeanton, H. Santoni, S. Garel, E. |
| Author_xml | – sequence: 1 givenname: S. surname: Santoni fullname: Santoni, S. email: santoni7@univ-corse.fr, santonisebastien17@gmail.com organization: Université de Corse Pascal Paoli, Faculté des Sciences et Techniques, Laboratoire d'Hydrogéologie, Campus Grimaldi, BP 52, F-20250 Corte, France – sequence: 2 givenname: F. surname: Huneau fullname: Huneau, F. organization: Université de Corse Pascal Paoli, Faculté des Sciences et Techniques, Laboratoire d'Hydrogéologie, Campus Grimaldi, BP 52, F-20250 Corte, France – sequence: 3 givenname: E. surname: Garel fullname: Garel, E. organization: Université de Corse Pascal Paoli, Faculté des Sciences et Techniques, Laboratoire d'Hydrogéologie, Campus Grimaldi, BP 52, F-20250 Corte, France – sequence: 4 givenname: L. surname: Aquilina fullname: Aquilina, L. organization: OSUR, Géosciences Rennes, UMR 6118, CNRS/Université Rennes-1, F-35042 Rennes, France – sequence: 5 givenname: V. surname: Vergnaud-Ayraud fullname: Vergnaud-Ayraud, V. organization: OSUR, Géosciences Rennes, UMR 6118, CNRS/Université Rennes-1, F-35042 Rennes, France – sequence: 6 givenname: T. surname: Labasque fullname: Labasque, T. organization: OSUR, Géosciences Rennes, UMR 6118, CNRS/Université Rennes-1, F-35042 Rennes, France – sequence: 7 givenname: H. surname: Celle-Jeanton fullname: Celle-Jeanton, H. organization: Université de Bourgogne Franche-Comté, UFR Sciences et Techniques, CNRS UMR 6249 Chrono-Environnement, 16 route de Gray, F-25 030 Besançon Cedex, France |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27565532$$D View this record in MEDLINE/PubMed https://insu.hal.science/insu-01355392$$DView record in HAL |
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| Keywords | Hydrogeochemistry Water-rocks interaction Kinetics Corsica Strontium isotopes |
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| SubjectTerms | Corsica Earth Sciences Geochemistry Hydrogeochemistry Hydrology Kinetics Sciences of the Universe Strontium isotopes Water-rocks interaction |
| Title | Strontium isotopes as tracers of water-rocks interactions, mixing processes and residence time indicator of groundwater within the granite-carbonate coastal aquifer of Bonifacio (Corsica, France) |
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