Ink-jet printing of organic semiconductor for fabricating organic thin-film transistors: Film uniformity control by ink composition
We have investigated the influence of solvent chemistry on ink-jet printed semiconductor patterns. Our research focuses on improving the uniformity of an ink-jet printed single dot semiconductor by adjusting the solvent mixture combination. Use of a solvent mixture with one solvent of a lower boilin...
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Published in | Synthetic metals Vol. 159; no. 13; pp. 1381 - 1385 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Amsterdam
Elsevier B.V
01.07.2009
Elsevier |
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Abstract | We have investigated the influence of solvent chemistry on ink-jet printed semiconductor patterns. Our research focuses on improving the uniformity of an ink-jet printed single dot semiconductor by adjusting the solvent mixture combination. Use of a solvent mixture with one solvent of a lower boiling point and a higher solubility with respect to the semiconductor molecules and another of a higher boiling point and a lower solubility allows us to produce a uniform single dot pattern by ink-jet printing. It was observed that the film uniformity of the semiconductor layer plays an important role in determining the electrical parameters of the transistor. In comparison with uncontrolled ink composition, the OTFT fabricated from the well-controlled ink exhibited better device performance, including a carrier mobility of 8.5
×
10
−3
cm
2
V
−1
s
−1 in the saturation regime, an on/off current ratio of 10
3, and a threshold voltage of 0.39
V with subthreshold slopes of 0.95
V
dec
−1. |
---|---|
AbstractList | We have investigated the influence of solvent chemistry on ink-jet printed semiconductor patterns. Our research focuses on improving the uniformity of an ink-jet printed single dot semiconductor by adjusting the solvent mixture combination. Use of a solvent mixture with one solvent of a lower boiling point and a higher solubility with respect to the semiconductor molecules and another of a higher boiling point and a lower solubility allows us to produce a uniform single dot pattern by ink-jet printing. It was observed that the film uniformity of the semiconductor layer plays an important role in determining the electrical parameters of the transistor. In comparison with uncontrolled ink composition, the OTFT fabricated from the well-controlled ink exhibited better device performance, including a carrier mobility of 8.5
×
10
−3
cm
2
V
−1
s
−1 in the saturation regime, an on/off current ratio of 10
3, and a threshold voltage of 0.39
V with subthreshold slopes of 0.95
V
dec
−1. We have investigated the influence of solvent chemistry on ink-jet printed semiconductor patterns. Our research focuses on improving the uniformity of an ink-jet printed single dot semiconductor by adjusting the solvent mixture combination. Use of a solvent mixture with one solvent of a lower boiling point and a higher solubility with respect to the semiconductor molecules and another of a higher boiling point and a lower solubility allows us to produce a uniform single dot pattern by ink-jet printing. It was observed that the film uniformity of the semiconductor layer plays an important role in determining the electrical parameters of the transistor. In comparison with uncontrolled ink composition, the OTFT fabricated from the well-controlled ink exhibited better device performance, including a carrier mobility of 8.5x10(-(3cm(2)V(-(1s(-(1 in the saturation regime, an on/off current ratio of 10(3), and a threshold voltage of 0.39V with subthreshold slopes of 0.95Vdec(-(1. |
Author | Jeong, Sunho Kim, Dongjo Song, Jun Kwang Lee, Seong Hui Moon, Jooho |
Author_xml | – sequence: 1 givenname: Dongjo surname: Kim fullname: Kim, Dongjo organization: Department of Materials Science and Engineering, Yonsei University, 134 Shinchon-dong Seodaemun-gu, Seoul 120-749, Republic of Korea – sequence: 2 givenname: Sunho surname: Jeong fullname: Jeong, Sunho organization: Department of Materials Science and Engineering, Yonsei University, 134 Shinchon-dong Seodaemun-gu, Seoul 120-749, Republic of Korea – sequence: 3 givenname: Seong Hui surname: Lee fullname: Lee, Seong Hui organization: Department of Materials Science and Engineering, Yonsei University, 134 Shinchon-dong Seodaemun-gu, Seoul 120-749, Republic of Korea – sequence: 4 givenname: Jooho surname: Moon fullname: Moon, Jooho email: jmoon@yonsei.ac.kr organization: Department of Materials Science and Engineering, Yonsei University, 134 Shinchon-dong Seodaemun-gu, Seoul 120-749, Republic of Korea – sequence: 5 givenname: Jun Kwang surname: Song fullname: Song, Jun Kwang organization: Material Testing Team, Korea Testing Laboratory, 222-13 Guro-dong, Guro-gu, Seoul 152-718, Republic of Korea |
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CitedBy_id | crossref_primary_10_1021_jp200972y crossref_primary_10_1108_PRT_05_2019_0043 crossref_primary_10_1016_j_synthmet_2011_08_004 crossref_primary_10_1088_2058_8585_aa8ac3 crossref_primary_10_1002_marc_201900569 crossref_primary_10_3139_146_110260 crossref_primary_10_1002_adma_201001697 crossref_primary_10_1007_s10853_012_6923_z crossref_primary_10_7567_JJAP_52_031601 crossref_primary_10_1143_JJAP_49_05EB06 crossref_primary_10_1039_C5TC02737C crossref_primary_10_1016_j_solener_2010_03_016 |
Cites_doi | 10.1016/S0379-6779(03)00186-3 10.1021/la053450j 10.1002/1521-4095(20020116)14:2<99::AID-ADMA99>3.0.CO;2-9 10.1002/marc.200500493 10.1063/1.2140586 10.1016/j.susc.2005.08.007 10.1021/cm970627p 10.1016/S0040-6090(02)01295-6 10.1021/jp0118322 10.1016/j.synthmet.2004.08.010 10.1021/la049469o 10.1002/adma.200401672 10.1039/b407478e 10.1038/39827 10.1016/S0167-9317(04)00225-4 10.1063/1.2437684 10.1149/1.2783765 10.1063/1.2424671 10.1002/adma.200400690 10.1063/1.1944224 10.1002/adma.200300385 10.1126/science.290.5499.2123 |
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Keywords | 68.55.am Ink-jet printing Organic thin-film transistor Ink 61.25.he 72.80.Le Organic semiconductor Solvent effect Voltage current curve Surface topography Oligomer Experimental study Property processing relationship Structure processing relationship Conjugated polymer Mixed solvent Tetramer Silicon Thiophene polymer Thin film transistor Ink jet printing Growth from solution |
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Snippet | We have investigated the influence of solvent chemistry on ink-jet printed semiconductor patterns. Our research focuses on improving the uniformity of an... |
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SubjectTerms | Application fields Applied sciences Electronics Exact sciences and technology Ink Ink-jet printing Organic semiconductor Organic thin-film transistor Polymer industry, paints, wood Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices Technology of polymers Transistors |
Title | Ink-jet printing of organic semiconductor for fabricating organic thin-film transistors: Film uniformity control by ink composition |
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