Selective anion exchange membranes for high coulombic efficiency vanadium redox flow batteries
A quaternary ammonium functionalized poly(fluorenyl ether) anion exchange membrane (AEM) with extremely low VO2+ permeation was characterized for vanadium redox flow battery (VRFB) application. One hundred percent coulombic efficiency (CE) was achieved for the AEM-based VRFB at all the current densi...
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| Published in | Electrochemistry communications Vol. 26; pp. 37 - 40 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Lausanne
Elsevier B.V
01.01.2013
Amsterdam Elsevier New York, NY |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A quaternary ammonium functionalized poly(fluorenyl ether) anion exchange membrane (AEM) with extremely low VO2+ permeation was characterized for vanadium redox flow battery (VRFB) application. One hundred percent coulombic efficiency (CE) was achieved for the AEM-based VRFB at all the current densities tested. Comparatively, the CE of a N212 membrane-based VRFB was lower than 94% and varied with charge/discharge current density. At current densities lower than 60mAcm−2, the energy effiency of the AEM-based VRFB was higher than that of a device with N212. The cycling performance demonstrated that the AEM-based VRFB was free of capacity fade, which is a consequence of its low VO2+ permeability. These observations are of significant importance for flow batteries that operate intermittently or at moderate current densities.
► Anion exchange membrane blocked the transport of vanadium ions due to the Donnan effect. ► One hundred percent coulombic efficiency of battery was achieved using anion exchange membrane. ► Lower current density gave higher voltage efficiency and energy efficiency. ► No capacity fade for maintenance-free operation |
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| AbstractList | A quaternary ammonium functionalized poly(fluorenyl ether) anion exchange membrane (AEM) with extremely low VO2+ permeation was characterized for vanadium redox flow battery (VRFB) application. One hundred percent coulombic efficiency (CE) was achieved for the AEM-based VRFB at all the current densities tested. Comparatively, the CE of a N212 membrane-based VRFB was lower than 94% and varied with charge/discharge current density. At current densities lower than 60mAcm−2, the energy effiency of the AEM-based VRFB was higher than that of a device with N212. The cycling performance demonstrated that the AEM-based VRFB was free of capacity fade, which is a consequence of its low VO2+ permeability. These observations are of significant importance for flow batteries that operate intermittently or at moderate current densities.
► Anion exchange membrane blocked the transport of vanadium ions due to the Donnan effect. ► One hundred percent coulombic efficiency of battery was achieved using anion exchange membrane. ► Lower current density gave higher voltage efficiency and energy efficiency. ► No capacity fade for maintenance-free operation |
| Author | Kumbur, E. Caglan Agar, Ertan Hickner, Michael A. Chen, Dongyang |
| Author_xml | – sequence: 1 givenname: Dongyang surname: Chen fullname: Chen, Dongyang organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA – sequence: 2 givenname: Michael A. surname: Hickner fullname: Hickner, Michael A. email: hickner@matse.psu.edu organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA – sequence: 3 givenname: Ertan surname: Agar fullname: Agar, Ertan organization: Electrochemical Energy Systems Laboratory, Department of Mechanical Engineering and Mechanics, Drexel University, Philadelphia, PA 19104, USA – sequence: 4 givenname: E. Caglan surname: Kumbur fullname: Kumbur, E. Caglan email: eck32@drexel.edu organization: Electrochemical Energy Systems Laboratory, Department of Mechanical Engineering and Mechanics, Drexel University, Philadelphia, PA 19104, USA |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=26834200$$DView record in Pascal Francis |
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| Keywords | Coulombic efficiency Vanadium redox flow battery Anion exchange membrane Capacity fade Self-discharge Cycling Fluorine containing copolymer Flow battery Vanadium Quaternary ammonium copolymer Ether copolymer Transition metal Secondary cell Cardic copolymer Discharge charge cycle Redox couple Deterioration Current efficiency Capacitance Self discharge Fluorene derivative copolymer Electrical characteristic Functional group |
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| Snippet | A quaternary ammonium functionalized poly(fluorenyl ether) anion exchange membrane (AEM) with extremely low VO2+ permeation was characterized for vanadium... |
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| SubjectTerms | Anion exchange membrane Applied sciences Capacity fade Coulombic efficiency Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Exact sciences and technology Self-discharge Vanadium redox flow battery |
| Title | Selective anion exchange membranes for high coulombic efficiency vanadium redox flow batteries |
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