Expanding the Scope of Polymerization‐Induced Self‐Assembly: Recent Advances and New Horizons
Over the past decade or so, polymerization‐induced self‐assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well‐defined linear block cop...
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| Published in | Macromolecular rapid communications. Vol. 42; no. 23; pp. e2100498 - n/a |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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01.12.2021
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| Abstract | Over the past decade or so, polymerization‐induced self‐assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well‐defined linear block copolymers by using linear macromolecular chain transfer agents (macro‐CTAs) with high chain transfer constants. In this review, a recent process is highlighted from an unusual angle that has expanded the scope of PISA including i) synthesis of block copolymers with nonlinear architectures (e.g., star block copolymer, branched block copolymer) by PISA, ii) in situ synthesis of blends of polymers by PISA, and iii) utilization of macro‐CTAs with low chain transfer constants in PISA. By highlighting these important examples, new insights into the research of PISA and future impact these methods will have on polymer and colloid synthesis are provided.
Different from traditional polymerization‐induced self‐assembly (PISA) that focuses on the preparation of linear block copolymer nano‐objects using macromolecular chain transfer agents with high chain transfer constants, this review summarizes recent advances of PISA, which focuses on in situ synthesis of nonlinear architectures, blends of polymers, and utilization of poor polymerization control. |
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| AbstractList | Over the past decade or so, polymerization-induced self-assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well-defined linear block copolymers by using linear macromolecular chain transfer agents (macro-CTAs) with high chain transfer constants. In this review, a recent process is highlighted from an unusual angle that has expanded the scope of PISA including i) synthesis of block copolymers with nonlinear architectures (e.g., star block copolymer, branched block copolymer) by PISA, ii) in situ synthesis of blends of polymers by PISA, and iii) utilization of macro-CTAs with low chain transfer constants in PISA. By highlighting these important examples, new insights into the research of PISA and future impact these methods will have on polymer and colloid synthesis are provided.Over the past decade or so, polymerization-induced self-assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well-defined linear block copolymers by using linear macromolecular chain transfer agents (macro-CTAs) with high chain transfer constants. In this review, a recent process is highlighted from an unusual angle that has expanded the scope of PISA including i) synthesis of block copolymers with nonlinear architectures (e.g., star block copolymer, branched block copolymer) by PISA, ii) in situ synthesis of blends of polymers by PISA, and iii) utilization of macro-CTAs with low chain transfer constants in PISA. By highlighting these important examples, new insights into the research of PISA and future impact these methods will have on polymer and colloid synthesis are provided. Over the past decade or so, polymerization-induced self-assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well-defined linear block copolymers by using linear macromolecular chain transfer agents (macro-CTAs) with high chain transfer constants. In this review, a recent process is highlighted from an unusual angle that has expanded the scope of PISA including i) synthesis of block copolymers with nonlinear architectures (e.g., star block copolymer, branched block copolymer) by PISA, ii) in situ synthesis of blends of polymers by PISA, and iii) utilization of macro-CTAs with low chain transfer constants in PISA. By highlighting these important examples, new insights into the research of PISA and future impact these methods will have on polymer and colloid synthesis are provided. Over the past decade or so, polymerization‐induced self‐assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer nanoparticles with a diverse set of morphologies. Much of the PISA literature has focused on the preparation of well‐defined linear block copolymers by using linear macromolecular chain transfer agents (macro‐CTAs) with high chain transfer constants. In this review, a recent process is highlighted from an unusual angle that has expanded the scope of PISA including i) synthesis of block copolymers with nonlinear architectures (e.g., star block copolymer, branched block copolymer) by PISA, ii) in situ synthesis of blends of polymers by PISA, and iii) utilization of macro‐CTAs with low chain transfer constants in PISA. By highlighting these important examples, new insights into the research of PISA and future impact these methods will have on polymer and colloid synthesis are provided. Different from traditional polymerization‐induced self‐assembly (PISA) that focuses on the preparation of linear block copolymer nano‐objects using macromolecular chain transfer agents with high chain transfer constants, this review summarizes recent advances of PISA, which focuses on in situ synthesis of nonlinear architectures, blends of polymers, and utilization of poor polymerization control. |
| Author | Tan, Yingxin Cao, Junpeng Tan, Jianbo Chen, Ying Zhang, Li |
| Author_xml | – sequence: 1 givenname: Junpeng surname: Cao fullname: Cao, Junpeng organization: Guangdong University of Technology – sequence: 2 givenname: Yingxin surname: Tan fullname: Tan, Yingxin organization: Guangdong University of Technology – sequence: 3 givenname: Ying surname: Chen fullname: Chen, Ying organization: Guangdong Provincial Key Laboratory of Functional Soft Condensed Matter – sequence: 4 givenname: Li surname: Zhang fullname: Zhang, Li organization: Guangdong Provincial Key Laboratory of Functional Soft Condensed Matter – sequence: 5 givenname: Jianbo orcidid: 0000-0002-5635-7178 surname: Tan fullname: Tan, Jianbo email: tanjianbo@gdut.edu.cn organization: Guangdong Provincial Key Laboratory of Functional Soft Condensed Matter |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34418199$$D View this record in MEDLINE/PubMed |
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| Snippet | Over the past decade or so, polymerization‐induced self‐assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer... Over the past decade or so, polymerization-induced self-assembly (PISA) has become a versatile method for rational preparation of concentrated block copolymer... |
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| SubjectTerms | Assembly blends of polymers Block copolymers Chain transfer Chemical synthesis Copolymers Macromolecular Substances Macromolecules Molecular chains Nanoparticles nonlinear architecture Polymer blends Polymerization polymerization‐induced self‐assembly Polymers poor polymerization control |
| Title | Expanding the Scope of Polymerization‐Induced Self‐Assembly: Recent Advances and New Horizons |
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