Surface and Interface Engineering of Zn Anodes in Aqueous Rechargeable Zn‐Ion Batteries

Rechargeable zinc‐ion batteries (ZIBs) have shown great potential as an alternative to lithium‐ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco‐friendliness, and high capacity. However, on the other hand, the Zn anode also suff...

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Published inSmall (Weinheim an der Bergstrasse, Germany) Vol. 18; no. 21; pp. e2200006 - n/a
Main Authors Zheng, Jiaxian, Huang, Zihao, Ming, Fangwang, Zeng, Ye, Wei, Binbin, Jiang, Qiu, Qi, Zhengbing, Wang, Zhoucheng, Liang, Hanfeng
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.05.2022
Subjects
Anodes
Anodic protection
interface engineering
Interfacial properties
Lithium-ion batteries
Nanotechnology
protective coating
Rechargeable batteries
support materials
surface engineering
Zinc
zinc‐ion batteries
surface engineering
support materials
zinc-ion batteries
protective coating
interface engineering
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Abstract Rechargeable zinc‐ion batteries (ZIBs) have shown great potential as an alternative to lithium‐ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco‐friendliness, and high capacity. However, on the other hand, the Zn anode also suffers from many issues, including dendritic growth, corrosion, and passivation. These issues are largely related to the surface and interface properties of the Zn anode. Many efforts have therefore been devoted to the modification of the Zn anode, aiming to eliminate the above‐mentioned problems. This review gives a comprehensive summary on the mechanism behind these issues as well as the recent progress on Zn anode modification with focus on the strategies of surface and interface engineering, covering the design and application of both the Zn anode supports and surface protective layers, along with abundant examples. In addition, the promising research directions and perspective on these strategies are also presented. Zn anodes in aqueous Zn‐ion batteries suffer from dendritic growth, corrosion, and passivation issues. A comprehensive review of the recent progress in Zn anode modification with focus on the design and application of both Zn anode supports and surface protective layers is presented. Additionally, promising research directions are also suggested to promote the development of highly reversible Zn anodes.
AbstractList Rechargeable zinc‐ion batteries (ZIBs) have shown great potential as an alternative to lithium‐ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco‐friendliness, and high capacity. However, on the other hand, the Zn anode also suffers from many issues, including dendritic growth, corrosion, and passivation. These issues are largely related to the surface and interface properties of the Zn anode. Many efforts have therefore been devoted to the modification of the Zn anode, aiming to eliminate the above‐mentioned problems. This review gives a comprehensive summary on the mechanism behind these issues as well as the recent progress on Zn anode modification with focus on the strategies of surface and interface engineering, covering the design and application of both the Zn anode supports and surface protective layers, along with abundant examples. In addition, the promising research directions and perspective on these strategies are also presented. Zn anodes in aqueous Zn‐ion batteries suffer from dendritic growth, corrosion, and passivation issues. A comprehensive review of the recent progress in Zn anode modification with focus on the design and application of both Zn anode supports and surface protective layers is presented. Additionally, promising research directions are also suggested to promote the development of highly reversible Zn anodes.
Rechargeable zinc-ion batteries (ZIBs) have shown great potential as an alternative to lithium-ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco-friendliness, and high capacity. However, on the other hand, the Zn anode also suffers from many issues, including dendritic growth, corrosion, and passivation. These issues are largely related to the surface and interface properties of the Zn anode. Many efforts have therefore been devoted to the modification of the Zn anode, aiming to eliminate the above-mentioned problems. This review gives a comprehensive summary on the mechanism behind these issues as well as the recent progress on Zn anode modification with focus on the strategies of surface and interface engineering, covering the design and application of both the Zn anode supports and surface protective layers, along with abundant examples. In addition, the promising research directions and perspective on these strategies are also presented.Rechargeable zinc-ion batteries (ZIBs) have shown great potential as an alternative to lithium-ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco-friendliness, and high capacity. However, on the other hand, the Zn anode also suffers from many issues, including dendritic growth, corrosion, and passivation. These issues are largely related to the surface and interface properties of the Zn anode. Many efforts have therefore been devoted to the modification of the Zn anode, aiming to eliminate the above-mentioned problems. This review gives a comprehensive summary on the mechanism behind these issues as well as the recent progress on Zn anode modification with focus on the strategies of surface and interface engineering, covering the design and application of both the Zn anode supports and surface protective layers, along with abundant examples. In addition, the promising research directions and perspective on these strategies are also presented.
Rechargeable zinc-ion batteries (ZIBs) have shown great potential as an alternative to lithium-ion batteries. The ZIBs utilize Zn metal as the anode, which possesses many advantages such as low cost, high safety, eco-friendliness, and high capacity. However, on the other hand, the Zn anode also suffers from many issues, including dendritic growth, corrosion, and passivation. These issues are largely related to the surface and interface properties of the Zn anode. Many efforts have therefore been devoted to the modification of the Zn anode, aiming to eliminate the above-mentioned problems. This review gives a comprehensive summary on the mechanism behind these issues as well as the recent progress on Zn anode modification with focus on the strategies of surface and interface engineering, covering the design and application of both the Zn anode supports and surface protective layers, along with abundant examples. In addition, the promising research directions and perspective on these strategies are also presented.
Author Zheng, Jiaxian
Ming, Fangwang
Zeng, Ye
Jiang, Qiu
Huang, Zihao
Wei, Binbin
Qi, Zhengbing
Wang, Zhoucheng
Liang, Hanfeng
Author_xml – sequence: 1
  givenname: Jiaxian
  surname: Zheng
  fullname: Zheng, Jiaxian
  organization: Xiamen University
– sequence: 2
  givenname: Zihao
  surname: Huang
  fullname: Huang, Zihao
  organization: Xiamen University
– sequence: 3
  givenname: Fangwang
  surname: Ming
  fullname: Ming, Fangwang
  organization: King Abdullah University of Science and Technology (KAUST)
– sequence: 4
  givenname: Ye
  surname: Zeng
  fullname: Zeng, Ye
  organization: Xiamen University
– sequence: 5
  givenname: Binbin
  surname: Wei
  fullname: Wei, Binbin
  organization: Tsinghua University
– sequence: 6
  givenname: Qiu
  surname: Jiang
  fullname: Jiang, Qiu
  email: jiangqiu@uestc.edu.cn
  organization: University of Electronic Science and Technology of China
– sequence: 7
  givenname: Zhengbing
  surname: Qi
  fullname: Qi, Zhengbing
  email: zbqi@xmut.edu.cn
  organization: Xiamen University of Technology
– sequence: 8
  givenname: Zhoucheng
  surname: Wang
  fullname: Wang, Zhoucheng
  organization: Xiamen University
– sequence: 9
  givenname: Hanfeng
  orcidid: 0000-0002-1778-3975
  surname: Liang
  fullname: Liang, Hanfeng
  email: hfliang@xmu.edu.cn
  organization: Xiamen University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35261146$$D View this record in MEDLINE/PubMed
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Keywords surface engineering
support materials
zinc-ion batteries
protective coating
interface engineering
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Snippet Rechargeable zinc‐ion batteries (ZIBs) have shown great potential as an alternative to lithium‐ion batteries. The ZIBs utilize Zn metal as the anode, which...
Rechargeable zinc-ion batteries (ZIBs) have shown great potential as an alternative to lithium-ion batteries. The ZIBs utilize Zn metal as the anode, which...
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SubjectTerms Anodes
Anodic protection
interface engineering
Interfacial properties
Lithium-ion batteries
Nanotechnology
protective coating
Rechargeable batteries
support materials
surface engineering
Zinc
zinc‐ion batteries
Title Surface and Interface Engineering of Zn Anodes in Aqueous Rechargeable Zn‐Ion Batteries
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fsmll.202200006
https://www.ncbi.nlm.nih.gov/pubmed/35261146
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