Structural Engineering toward Gold Nanocluster Catalysis
Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A nanocluster consists of a metal core and a surface ligand shell, and both the core and shell have significant effects on the catalytic properties...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 51; pp. e202209725 - n/a |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
19.12.2022
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A nanocluster consists of a metal core and a surface ligand shell, and both the core and shell have significant effects on the catalytic properties. Thanks to their precise structures, the active metal site of the clusters can be readily identified and the effects of ligands on catalysis can be disclosed. In this Minireview, we summarize recent advances in catalytic research of gold nanoclusters, emphasizing four strategies for constructing open metal sites, including by post‐treatment, the bulky ligands strategy, the surface geometric mismatch method, and heteroatom doping procedures. We also discuss the effects of ligands on the catalytic activity, selectivity, and stability of gold cluster catalysts. Finally, we present future challenges relating to gold cluster catalysis.
Structurally well‐defined gold nanoclusters are promising catalysts, and their molecular nature facilitates the design and controlled synthesis of cluster catalysts. This Minireview summarizes the strategies for constructing active sites and the effects of the ligands on cluster catalysis. The challenges and key future issues regarding catalytic applications of gold nanoclusters are discussed. |
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| AbstractList | Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A nanocluster consists of a metal core and a surface ligand shell, and both the core and shell have significant effects on the catalytic properties. Thanks to their precise structures, the active metal site of the clusters can be readily identified and the effects of ligands on catalysis can be disclosed. In this Minireview, we summarize recent advances in catalytic research of gold nanoclusters, emphasizing four strategies for constructing open metal sites, including by post‐treatment, the bulky ligands strategy, the surface geometric mismatch method, and heteroatom doping procedures. We also discuss the effects of ligands on the catalytic activity, selectivity, and stability of gold cluster catalysts. Finally, we present future challenges relating to gold cluster catalysis.
Structurally well‐defined gold nanoclusters are promising catalysts, and their molecular nature facilitates the design and controlled synthesis of cluster catalysts. This Minireview summarizes the strategies for constructing active sites and the effects of the ligands on cluster catalysis. The challenges and key future issues regarding catalytic applications of gold nanoclusters are discussed. Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A nanocluster consists of a metal core and a surface ligand shell, and both the core and shell have significant effects on the catalytic properties. Thanks to their precise structures, the active metal site of the clusters can be readily identified and the effects of ligands on catalysis can be disclosed. In this Minireview, we summarize recent advances in catalytic research of gold nanoclusters, emphasizing four strategies for constructing open metal sites, including by post‐treatment, the bulky ligands strategy, the surface geometric mismatch method, and heteroatom doping procedures. We also discuss the effects of ligands on the catalytic activity, selectivity, and stability of gold cluster catalysts. Finally, we present future challenges relating to gold cluster catalysis. Abstract Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A nanocluster consists of a metal core and a surface ligand shell, and both the core and shell have significant effects on the catalytic properties. Thanks to their precise structures, the active metal site of the clusters can be readily identified and the effects of ligands on catalysis can be disclosed. In this Minireview, we summarize recent advances in catalytic research of gold nanoclusters, emphasizing four strategies for constructing open metal sites, including by post‐treatment, the bulky ligands strategy, the surface geometric mismatch method, and heteroatom doping procedures. We also discuss the effects of ligands on the catalytic activity, selectivity, and stability of gold cluster catalysts. Finally, we present future challenges relating to gold cluster catalysis. |
| Author | Li, Jiao‐Jiao Guan, Zong‐Jie Wang, Quan‐Ming Hu, Feng |
| Author_xml | – sequence: 1 givenname: Zong‐Jie orcidid: 0000-0001-8977-0850 surname: Guan fullname: Guan, Zong‐Jie organization: Hunan University – sequence: 2 givenname: Jiao‐Jiao surname: Li fullname: Li, Jiao‐Jiao organization: Tsinghua University – sequence: 3 givenname: Feng surname: Hu fullname: Hu, Feng organization: Tsinghua University – sequence: 4 givenname: Quan‐Ming orcidid: 0000-0002-3764-6409 surname: Wang fullname: Wang, Quan‐Ming email: qmwang@tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36169269$$D View this record in MEDLINE/PubMed |
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| Keywords | Ligand Effects Active Sites Gold Catalysis Nanoclusters |
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| Snippet | Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold catalysts. A... Abstract Atomically precise gold nanoclusters provide great opportunities to explore the relationship between the structure and properties of nanogold... |
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| SubjectTerms | Active Sites Catalysis Catalysts Catalytic activity Clusters Gold Ligand Effects Ligands Nanoclusters Reviews Selectivity Structural engineering |
| Title | Structural Engineering toward Gold Nanocluster Catalysis |
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