Inorganic and Layered Perovskites for Optoelectronic Devices

Organic–inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light‐emitting diodes (LEDs), continuous‐wave lasing and ultralow lasing thresh...

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Published inAdvanced materials (Weinheim) Vol. 31; no. 47; pp. e1807095 - n/a
Main Authors Fakharuddin, Azhar, Shabbir, Umair, Qiu, Weiming, Iqbal, Tahir, Sultan, Muhammad, Heremans, Paul, Schmidt‐Mende, Lukas
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.11.2019
Subjects
all‐inorganic perovskites
Cations
Cesium
Current voltage characteristics
Devices
Diodes
Energy conversion efficiency
Excitons
Ion migration
Lasing
layered perovskites
light emission from perovskites
Market entry
Materials science
Morphology
Optoelectronic devices
Organic light emitting diodes
perovskite photonic devices
Perovskites
Photovoltaic cells
Quantum efficiency
stability of inorganic perovskites
Toxicity
layered perovskites
light emission from perovskites
perovskite photonic devices
stability of inorganic perovskites
all-inorganic perovskites
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Abstract Organic–inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light‐emitting diodes (LEDs), continuous‐wave lasing and ultralow lasing thresholds in optically pumped lasers, and detectivity in photodetectors on a par with commercial GaAs rivals are being witnessed, making them the fastest ever emerging material technology. Still, questions on their toxicity and long‐term stability raise concerns toward their market entry. The intrinsic instability in these materials arises due to the organic cation, typically the volatile methylamine (MA), which contributes to hysteresis in the current–voltage characteristics and ion migration. Alternative inorganic substitutes to MA, such as cesium, and large organic cations that lead to a layered structure, enhance structural as well as device operational stability. These perovskites also provide a high exciton binding energy that is a prerequisite to enhance radiative emission yield in LEDs. The incorporation of inorganic and layered perovskites, in the form of polycrystalline films or as single‐crystalline nanostructure morphologies, is now leading to the demonstration of stable devices with excellent performance parameters. Herein, key developments made in various optoelectronic devices using these perovskites are summarized and an outlook toward stable yet efficient devices is presented. Inorganic and layered perovskites have broadened research paradigm for a range of optoelectronic devices. Their unique electronic and photophysical properties show that they are an excellent material, leading forefronts of solar cells, light‐emitting diodes, photodetectors, lasers, and beyond. An overview of key research activities for these devices is provided and challenges for their future research are identified.
AbstractList Organic–inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light‐emitting diodes (LEDs), continuous‐wave lasing and ultralow lasing thresholds in optically pumped lasers, and detectivity in photodetectors on a par with commercial GaAs rivals are being witnessed, making them the fastest ever emerging material technology. Still, questions on their toxicity and long‐term stability raise concerns toward their market entry. The intrinsic instability in these materials arises due to the organic cation, typically the volatile methylamine (MA), which contributes to hysteresis in the current–voltage characteristics and ion migration. Alternative inorganic substitutes to MA, such as cesium, and large organic cations that lead to a layered structure, enhance structural as well as device operational stability. These perovskites also provide a high exciton binding energy that is a prerequisite to enhance radiative emission yield in LEDs. The incorporation of inorganic and layered perovskites, in the form of polycrystalline films or as single‐crystalline nanostructure morphologies, is now leading to the demonstration of stable devices with excellent performance parameters. Herein, key developments made in various optoelectronic devices using these perovskites are summarized and an outlook toward stable yet efficient devices is presented.
Organic–inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light‐emitting diodes (LEDs), continuous‐wave lasing and ultralow lasing thresholds in optically pumped lasers, and detectivity in photodetectors on a par with commercial GaAs rivals are being witnessed, making them the fastest ever emerging material technology. Still, questions on their toxicity and long‐term stability raise concerns toward their market entry. The intrinsic instability in these materials arises due to the organic cation, typically the volatile methylamine (MA), which contributes to hysteresis in the current–voltage characteristics and ion migration. Alternative inorganic substitutes to MA, such as cesium, and large organic cations that lead to a layered structure, enhance structural as well as device operational stability. These perovskites also provide a high exciton binding energy that is a prerequisite to enhance radiative emission yield in LEDs. The incorporation of inorganic and layered perovskites, in the form of polycrystalline films or as single‐crystalline nanostructure morphologies, is now leading to the demonstration of stable devices with excellent performance parameters. Herein, key developments made in various optoelectronic devices using these perovskites are summarized and an outlook toward stable yet efficient devices is presented. Inorganic and layered perovskites have broadened research paradigm for a range of optoelectronic devices. Their unique electronic and photophysical properties show that they are an excellent material, leading forefronts of solar cells, light‐emitting diodes, photodetectors, lasers, and beyond. An overview of key research activities for these devices is provided and challenges for their future research are identified.
Organic-inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light-emitting diodes (LEDs), continuous-wave lasing and ultralow lasing thresholds in optically pumped lasers, and detectivity in photodetectors on a par with commercial GaAs rivals are being witnessed, making them the fastest ever emerging material technology. Still, questions on their toxicity and long-term stability raise concerns toward their market entry. The intrinsic instability in these materials arises due to the organic cation, typically the volatile methylamine (MA), which contributes to hysteresis in the current-voltage characteristics and ion migration. Alternative inorganic substitutes to MA, such as cesium, and large organic cations that lead to a layered structure, enhance structural as well as device operational stability. These perovskites also provide a high exciton binding energy that is a prerequisite to enhance radiative emission yield in LEDs. The incorporation of inorganic and layered perovskites, in the form of polycrystalline films or as single-crystalline nanostructure morphologies, is now leading to the demonstration of stable devices with excellent performance parameters. Herein, key developments made in various optoelectronic devices using these perovskites are summarized and an outlook toward stable yet efficient devices is presented.Organic-inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in photovoltaic devices, external quantum efficiency >21% in light-emitting diodes (LEDs), continuous-wave lasing and ultralow lasing thresholds in optically pumped lasers, and detectivity in photodetectors on a par with commercial GaAs rivals are being witnessed, making them the fastest ever emerging material technology. Still, questions on their toxicity and long-term stability raise concerns toward their market entry. The intrinsic instability in these materials arises due to the organic cation, typically the volatile methylamine (MA), which contributes to hysteresis in the current-voltage characteristics and ion migration. Alternative inorganic substitutes to MA, such as cesium, and large organic cations that lead to a layered structure, enhance structural as well as device operational stability. These perovskites also provide a high exciton binding energy that is a prerequisite to enhance radiative emission yield in LEDs. The incorporation of inorganic and layered perovskites, in the form of polycrystalline films or as single-crystalline nanostructure morphologies, is now leading to the demonstration of stable devices with excellent performance parameters. Herein, key developments made in various optoelectronic devices using these perovskites are summarized and an outlook toward stable yet efficient devices is presented.
Author Qiu, Weiming
Heremans, Paul
Iqbal, Tahir
Sultan, Muhammad
Fakharuddin, Azhar
Shabbir, Umair
Schmidt‐Mende, Lukas
Author_xml – sequence: 1
  givenname: Azhar
  surname: Fakharuddin
  fullname: Fakharuddin, Azhar
  email: azhar.fakhar.uddin@imec.be
  organization: University of Konstanz
– sequence: 2
  givenname: Umair
  surname: Shabbir
  fullname: Shabbir, Umair
  organization: University Campus
– sequence: 3
  givenname: Weiming
  surname: Qiu
  fullname: Qiu, Weiming
  email: weiming.qiu@imec.be
  organization: KU Leuven
– sequence: 4
  givenname: Tahir
  surname: Iqbal
  fullname: Iqbal, Tahir
  organization: University of Gujrat
– sequence: 5
  givenname: Muhammad
  surname: Sultan
  fullname: Sultan, Muhammad
  email: sultan@ncp.edu.pk
  organization: University Campus
– sequence: 6
  givenname: Paul
  surname: Heremans
  fullname: Heremans, Paul
  organization: KU Leuven
– sequence: 7
  givenname: Lukas
  orcidid: 0000-0001-6867-443X
  surname: Schmidt‐Mende
  fullname: Schmidt‐Mende, Lukas
  email: lukas.schmidt-mende@uni-konstanz.de
  organization: University of Konstanz
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31012172$$D View this record in MEDLINE/PubMed
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Issue 47
Keywords layered perovskites
light emission from perovskites
perovskite photonic devices
stability of inorganic perovskites
all-inorganic perovskites
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e_1_2_8_235_5
e_1_2_8_235_1
e_1_2_8_258_1
e_1_2_8_235_2
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e_1_2_8_148_1
e_1_2_8_186_1
e_1_2_8_102_2
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e_1_2_8_262_1
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e_1_2_8_285_1
e_1_2_8_24_1
e_1_2_8_47_1
e_1_2_8_224_1
e_1_2_8_201_1
e_1_2_8_247_1
e_1_2_8_3_1
e_1_2_8_153_2
e_1_2_8_130_1
e_1_2_8_153_1
e_1_2_8_209_1
e_1_2_8_130_2
e_1_2_8_191_2
e_1_2_8_138_1
e_1_2_8_62_1
e_1_2_8_85_1
e_1_2_8_115_1
e_1_2_8_176_1
e_1_2_8_199_1
e_1_2_8_251_1
e_1_2_8_297_1
e_1_2_8_274_1
e_1_2_8_13_1
e_1_2_8_36_1
e_1_2_8_59_1
e_1_2_8_190_1
e_1_2_8_213_1
e_1_2_8_259_1
e_1_2_8_236_1
e_1_2_8_187_3
e_1_2_8_141_1
e_1_2_8_164_1
e_1_2_8_97_1
e_1_2_8_149_1
e_1_2_8_51_1
e_1_2_8_74_1
e_1_2_8_103_1
e_1_2_8_126_1
e_1_2_8_187_1
e_1_2_8_187_2
e_1_2_8_240_1
e_1_2_8_263_1
e_1_2_8_286_1
e_1_2_8_308_1
e_1_2_8_69_4
e_1_2_8_23_2
e_1_2_8_69_2
e_1_2_8_46_1
e_1_2_8_69_3
e_1_2_8_69_1
e_1_2_8_180_1
e_1_2_8_202_1
e_1_2_8_225_1
e_1_2_8_248_1
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e_1_2_8_154_1
e_1_2_8_4_1
e_1_2_8_131_1
e_1_2_8_139_2
e_1_2_8_192_1
e_1_2_8_300_1
e_1_2_8_116_1
e_1_2_8_23_1
e_1_2_8_139_1
e_1_2_8_84_2
e_1_2_8_84_1
e_1_2_8_61_1
e_1_2_8_177_1
e_1_2_8_252_1
e_1_2_8_275_1
e_1_2_8_298_1
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e_1_2_8_58_1
e_1_2_8_191_1
e_1_2_8_214_1
e_1_2_8_237_1
e_1_2_8_165_1
e_1_2_8_96_1
e_1_2_8_142_1
e_1_2_8_180_2
e_1_2_8_127_1
e_1_2_8_12_1
e_1_2_8_73_3
e_1_2_8_73_2
e_1_2_8_73_1
e_1_2_8_50_1
e_1_2_8_104_1
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Snippet Organic–inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in...
Organic-inorganic halide perovskites are making breakthroughs in a range of optoelectronic devices. Reports of >23% certified power conversion efficiency in...
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StartPage e1807095
SubjectTerms all‐inorganic perovskites
Cations
Cesium
Current voltage characteristics
Devices
Diodes
Energy conversion efficiency
Excitons
Ion migration
Lasing
layered perovskites
light emission from perovskites
Market entry
Materials science
Morphology
Optoelectronic devices
Organic light emitting diodes
perovskite photonic devices
Perovskites
Photovoltaic cells
Quantum efficiency
stability of inorganic perovskites
Toxicity
Title Inorganic and Layered Perovskites for Optoelectronic Devices
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201807095
https://www.ncbi.nlm.nih.gov/pubmed/31012172
https://www.proquest.com/docview/2315585655
https://www.proquest.com/docview/2213151394
Volume 31
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