3D Continuously Porous Graphene for Energy Applications

Constructing bulk graphene materials with well‐reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures,...

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Published inAdvanced materials (Weinheim) Vol. 34; no. 15; pp. e2108750 - n/a
Main Authors Han, Jiuhui, Johnson, Isaac, Chen, Mingwei
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.04.2022
Subjects
3D graphene
Curvature
Energy conversion
Energy storage
Graphene
Mass transport
Materials science
Microstructure
Minimal surfaces
Thermal conductivity
topological defects
Transport properties
energy conversion
energy storage
topological defects
3D graphene
curvature
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Abstract Constructing bulk graphene materials with well‐reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures, chemistries, and properties for energy storage and conversion are reviewed. Both template‐based and template‐free methods have been developed to synthesize the 3D continuously porous graphene, which typically has the microstructure reminiscent of pseudo‐periodic minimal surfaces. The 3D graphene can well preserve the properties of 2D graphene of being highly conductive, surface abundant, and mechanically robust, together with unique 2D electronic behaviors. Additionally, the bicontinuous porosity and large curvature offer new functionalities, such as rapid mass transport, ample open space, mechanical flexibility, and tunable electric/thermal conductivity. Particularly, the 3D curvature provides a new degree of freedom for tailoring the catalysis and transport properties of graphene. The 3D graphene with those extraordinary properties has shown great promises for a wide range of applications, especially for energy conversion and storage. This article overviews the recent advances made in addressing the challenges of developing 3D continuously porous graphene, the benefits and opportunities of the new materials for energy‐related applications, and the remaining challenges that warrant future study. 3D continuously porous graphene formed by folding a single‐sheet graphene into a 3D porous architecture has well‐retained 2D properties of graphene and novel functionalities from 3D structure, representing a distinct class of graphene materials with numerous unique and extraordinary properties. A comprehensive review of 3D continuously porous graphene and their applications in energy conversion and storage is provided.
AbstractList Constructing bulk graphene materials with well-reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures, chemistries, and properties for energy storage and conversion are reviewed. Both template-based and template-free methods have been developed to synthesize the 3D continuously porous graphene, which typically has the microstructure reminiscent of pseudo-periodic minimal surfaces. The 3D graphene can well preserve the properties of 2D graphene of being highly conductive, surface abundant, and mechanically robust, together with unique 2D electronic behaviors. Additionally, the bicontinuous porosity and large curvature offer new functionalities, such as rapid mass transport, ample open space, mechanical flexibility, and tunable electric/thermal conductivity. Particularly, the 3D curvature provides a new degree of freedom for tailoring the catalysis and transport properties of graphene. The 3D graphene with those extraordinary properties has shown great promises for a wide range of applications, especially for energy conversion and storage. This article overviews the recent advances made in addressing the challenges of developing 3D continuously porous graphene, the benefits and opportunities of the new materials for energy-related applications, and the remaining challenges that warrant future study.Constructing bulk graphene materials with well-reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures, chemistries, and properties for energy storage and conversion are reviewed. Both template-based and template-free methods have been developed to synthesize the 3D continuously porous graphene, which typically has the microstructure reminiscent of pseudo-periodic minimal surfaces. The 3D graphene can well preserve the properties of 2D graphene of being highly conductive, surface abundant, and mechanically robust, together with unique 2D electronic behaviors. Additionally, the bicontinuous porosity and large curvature offer new functionalities, such as rapid mass transport, ample open space, mechanical flexibility, and tunable electric/thermal conductivity. Particularly, the 3D curvature provides a new degree of freedom for tailoring the catalysis and transport properties of graphene. The 3D graphene with those extraordinary properties has shown great promises for a wide range of applications, especially for energy conversion and storage. This article overviews the recent advances made in addressing the challenges of developing 3D continuously porous graphene, the benefits and opportunities of the new materials for energy-related applications, and the remaining challenges that warrant future study.
Constructing bulk graphene materials with well‐reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures, chemistries, and properties for energy storage and conversion are reviewed. Both template‐based and template‐free methods have been developed to synthesize the 3D continuously porous graphene, which typically has the microstructure reminiscent of pseudo‐periodic minimal surfaces. The 3D graphene can well preserve the properties of 2D graphene of being highly conductive, surface abundant, and mechanically robust, together with unique 2D electronic behaviors. Additionally, the bicontinuous porosity and large curvature offer new functionalities, such as rapid mass transport, ample open space, mechanical flexibility, and tunable electric/thermal conductivity. Particularly, the 3D curvature provides a new degree of freedom for tailoring the catalysis and transport properties of graphene. The 3D graphene with those extraordinary properties has shown great promises for a wide range of applications, especially for energy conversion and storage. This article overviews the recent advances made in addressing the challenges of developing 3D continuously porous graphene, the benefits and opportunities of the new materials for energy‐related applications, and the remaining challenges that warrant future study. 3D continuously porous graphene formed by folding a single‐sheet graphene into a 3D porous architecture has well‐retained 2D properties of graphene and novel functionalities from 3D structure, representing a distinct class of graphene materials with numerous unique and extraordinary properties. A comprehensive review of 3D continuously porous graphene and their applications in energy conversion and storage is provided.
Constructing bulk graphene materials with well‐reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In this article, the recent progress in the fabrications and applications of sterically continuous porous graphene with designable microstructures, chemistries, and properties for energy storage and conversion are reviewed. Both template‐based and template‐free methods have been developed to synthesize the 3D continuously porous graphene, which typically has the microstructure reminiscent of pseudo‐periodic minimal surfaces. The 3D graphene can well preserve the properties of 2D graphene of being highly conductive, surface abundant, and mechanically robust, together with unique 2D electronic behaviors. Additionally, the bicontinuous porosity and large curvature offer new functionalities, such as rapid mass transport, ample open space, mechanical flexibility, and tunable electric/thermal conductivity. Particularly, the 3D curvature provides a new degree of freedom for tailoring the catalysis and transport properties of graphene. The 3D graphene with those extraordinary properties has shown great promises for a wide range of applications, especially for energy conversion and storage. This article overviews the recent advances made in addressing the challenges of developing 3D continuously porous graphene, the benefits and opportunities of the new materials for energy‐related applications, and the remaining challenges that warrant future study.
Author Johnson, Isaac
Han, Jiuhui
Chen, Mingwei
Author_xml – sequence: 1
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  surname: Han
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  surname: Chen
  fullname: Chen, Mingwei
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Issue 15
Keywords energy conversion
energy storage
topological defects
3D graphene
curvature
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Snippet Constructing bulk graphene materials with well‐reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In...
Constructing bulk graphene materials with well-reserved 2D properties is essential for device and engineering applications of atomically thick graphene. In...
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SubjectTerms 3D graphene
Curvature
Energy conversion
Energy storage
Graphene
Mass transport
Materials science
Microstructure
Minimal surfaces
Thermal conductivity
topological defects
Transport properties
Title 3D Continuously Porous Graphene for Energy Applications
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202108750
https://www.ncbi.nlm.nih.gov/pubmed/34870863
https://www.proquest.com/docview/2649895712
https://www.proquest.com/docview/2607306678
Volume 34
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