MXene‐Derived Ferroelectric Crystals
This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO3) ferroelectric crystals is successfully synthesized using 2D Nb2C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Mat...
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| Published in | Advanced materials (Weinheim) Vol. 31; no. 14; pp. e1806860 - n/a |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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05.04.2019
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| Abstract | This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO3) ferroelectric crystals is successfully synthesized using 2D Nb2C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO3 orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO3 crystals exhibit a saturated polarization of ≈21 µC cm−2, a remnant polarization of ≈17 µC cm−2, and a coercive field of ≈50 kV cm−1. This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals.
MXene‐derived high‐aspect‐ratio potassium niobate (KNbO3) single crystals are successfully synthesized using 2D Nb3C MXene and potassium hydroxide (KOH) as the niobium and potassium source, respectively. The well‐defined butterfly loops of the piezoresponse force microscopy amplitude signals and the distinct 180° switching of the phase signals further corroborate the presence of robust ferroelectricity in M‐KNbO3 crystals. |
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| AbstractList | This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO3) ferroelectric crystals is successfully synthesized using 2D Nb2C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO3 orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO3 crystals exhibit a saturated polarization of ≈21 µC cm−2, a remnant polarization of ≈17 µC cm−2, and a coercive field of ≈50 kV cm−1. This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals.
MXene‐derived high‐aspect‐ratio potassium niobate (KNbO3) single crystals are successfully synthesized using 2D Nb3C MXene and potassium hydroxide (KOH) as the niobium and potassium source, respectively. The well‐defined butterfly loops of the piezoresponse force microscopy amplitude signals and the distinct 180° switching of the phase signals further corroborate the presence of robust ferroelectricity in M‐KNbO3 crystals. This study demonstrates the first synthesis of MXene-derived ferroelectric crystals. Specifically, high-aspect-ratio potassium niobate (KNbO ) ferroelectric crystals is successfully synthesized using 2D Nb C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO crystals exhibit a saturated polarization of ≈21 µC cm , a remnant polarization of ≈17 µC cm , and a coercive field of ≈50 kV cm . This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals. This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO3) ferroelectric crystals is successfully synthesized using 2D Nb2C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO3 orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO3 crystals exhibit a saturated polarization of ≈21 µC cm−2, a remnant polarization of ≈17 µC cm−2, and a coercive field of ≈50 kV cm−1. This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals. This study demonstrates the first synthesis of MXene-derived ferroelectric crystals. Specifically, high-aspect-ratio potassium niobate (KNbO3 ) ferroelectric crystals is successfully synthesized using 2D Nb2 C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO3 orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO3 crystals exhibit a saturated polarization of ≈21 µC cm-2 , a remnant polarization of ≈17 µC cm-2 , and a coercive field of ≈50 kV cm-1 . This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals.This study demonstrates the first synthesis of MXene-derived ferroelectric crystals. Specifically, high-aspect-ratio potassium niobate (KNbO3 ) ferroelectric crystals is successfully synthesized using 2D Nb2 C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO3 orthorhombic phase with Amm2 symmetry is obtained. Additionally, ferroelectricity in KNbO3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO3 crystals exhibit a saturated polarization of ≈21 µC cm-2 , a remnant polarization of ≈17 µC cm-2 , and a coercive field of ≈50 kV cm-1 . This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals. This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO 3 ) ferroelectric crystals is successfully synthesized using 2D Nb 2 C, MXene, and potassium hydroxide (KOH) as the niobium and potassium source, respectively. Material analysis confirms that a KNbO 3 orthorhombic phase with Amm 2 symmetry is obtained. Additionally, ferroelectricity in KNbO 3 is confirmed using standard ferroelectric, dielectric, and piezoresponse force microscopy measurements. The KNbO 3 crystals exhibit a saturated polarization of ≈21 µC cm −2 , a remnant polarization of ≈17 µC cm −2 , and a coercive field of ≈50 kV cm −1 . This discovery illustrates that the 2D nature of MXenes can be exploited to grow ferroelectric crystals. |
| Author | Ming, Fangwang Zhang, Junwei Tu, Shaobo Alshareef, Husam N. Zhang, Xixiang |
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| Keywords | MXene-derived MAX phase hydrothermal synthesis single crystal ferroelectricity |
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| Snippet | This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO3) ferroelectric... This study demonstrates the first synthesis of MXene‐derived ferroelectric crystals. Specifically, high‐aspect‐ratio potassium niobate (KNbO 3 ) ferroelectric... This study demonstrates the first synthesis of MXene-derived ferroelectric crystals. Specifically, high-aspect-ratio potassium niobate (KNbO ) ferroelectric... This study demonstrates the first synthesis of MXene-derived ferroelectric crystals. Specifically, high-aspect-ratio potassium niobate (KNbO3 ) ferroelectric... |
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| SubjectTerms | Coercivity Crystal growth Ferroelectric crystals Ferroelectric materials Ferroelectricity hydrothermal synthesis Materials science MAX phase MXenes MXene‐derived Niobium carbide Orthorhombic phase Polarization Potassium Potassium hydroxides Potassium niobates single crystal |
| Title | MXene‐Derived Ferroelectric Crystals |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201806860 https://www.ncbi.nlm.nih.gov/pubmed/30762903 https://www.proquest.com/docview/2201707943 https://www.proquest.com/docview/2202194326 |
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