Kinetic analyses and pyrolytic behavior of Para grass (Urochloa mutica) for its bioenergy potential
•Para grass is a source of low-cost and abundant biomass.•TGA-DSC analyses were performed to understand kinetics of pyrolysis.•Thermodynamics parameters indicate the bioenergy potential of this novel biomass.•The bioenergy potential of the biomass is comparable with established bioenergy crops. The...
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| Published in | Bioresource technology Vol. 224; pp. 708 - 713 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.01.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | •Para grass is a source of low-cost and abundant biomass.•TGA-DSC analyses were performed to understand kinetics of pyrolysis.•Thermodynamics parameters indicate the bioenergy potential of this novel biomass.•The bioenergy potential of the biomass is comparable with established bioenergy crops.
The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation experiments were performed at three different heating rates, 10, 30 and 50°Cmin−1 using simultaneous thermogravimetric-differential scanning calorimetric analyzer, under an inert environment. The kinetic analyses were performed using isoconversional models of Kissenger-Akahira-Sunose (KAS) and Flynn–Wall–Ozawa (FWO). The high heating value was calculated as 15.04MJmol−1. The activation energy (E) values were shown to be ranging from 103 through 233 kJmol−1. Pre-exponential factors (A) indicated the reaction to follow first order kinetics. Gibbs free energy (ΔG) was measured to be ranging from 169 to 173kJmol−1 and 168 to 172kJmol−1, calculated by KAS and FWO methods, respectively. We have shown that Para grass biomass has considerable bioenergy potential comparable to established bioenergy crops such as switchgrass and miscanthus. |
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| AbstractList | The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation experiments were performed at three different heating rates, 10, 30 and 50°Cmin-1 using simultaneous thermogravimetric-differential scanning calorimetric analyzer, under an inert environment. The kinetic analyses were performed using isoconversional models of Kissenger-Akahira-Sunose (KAS) and Flynn-Wall-Ozawa (FWO). The high heating value was calculated as 15.04MJmol-1. The activation energy (E) values were shown to be ranging from 103 through 233 kJmol-1. Pre-exponential factors (A) indicated the reaction to follow first order kinetics. Gibbs free energy (ΔG) was measured to be ranging from 169 to 173kJmol-1 and 168 to 172kJmol-1, calculated by KAS and FWO methods, respectively. We have shown that Para grass biomass has considerable bioenergy potential comparable to established bioenergy crops such as switchgrass and miscanthus. The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation experiments were performed at three different heating rates, 10, 30 and 50°Cmin using simultaneous thermogravimetric-differential scanning calorimetric analyzer, under an inert environment. The kinetic analyses were performed using isoconversional models of Kissenger-Akahira-Sunose (KAS) and Flynn-Wall-Ozawa (FWO). The high heating value was calculated as 15.04MJmol . The activation energy (E) values were shown to be ranging from 103 through 233 kJmol . Pre-exponential factors (A) indicated the reaction to follow first order kinetics. Gibbs free energy (ΔG) was measured to be ranging from 169 to 173kJmol and 168 to 172kJmol , calculated by KAS and FWO methods, respectively. We have shown that Para grass biomass has considerable bioenergy potential comparable to established bioenergy crops such as switchgrass and miscanthus. •Para grass is a source of low-cost and abundant biomass.•TGA-DSC analyses were performed to understand kinetics of pyrolysis.•Thermodynamics parameters indicate the bioenergy potential of this novel biomass.•The bioenergy potential of the biomass is comparable with established bioenergy crops. The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation experiments were performed at three different heating rates, 10, 30 and 50°Cmin−1 using simultaneous thermogravimetric-differential scanning calorimetric analyzer, under an inert environment. The kinetic analyses were performed using isoconversional models of Kissenger-Akahira-Sunose (KAS) and Flynn–Wall–Ozawa (FWO). The high heating value was calculated as 15.04MJmol−1. The activation energy (E) values were shown to be ranging from 103 through 233 kJmol−1. Pre-exponential factors (A) indicated the reaction to follow first order kinetics. Gibbs free energy (ΔG) was measured to be ranging from 169 to 173kJmol−1 and 168 to 172kJmol−1, calculated by KAS and FWO methods, respectively. We have shown that Para grass biomass has considerable bioenergy potential comparable to established bioenergy crops such as switchgrass and miscanthus. The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation experiments were performed at three different heating rates, 10, 30 and 50°Cmin⁻¹ using simultaneous thermogravimetric-differential scanning calorimetric analyzer, under an inert environment. The kinetic analyses were performed using isoconversional models of Kissenger-Akahira-Sunose (KAS) and Flynn–Wall–Ozawa (FWO). The high heating value was calculated as 15.04MJmol⁻¹. The activation energy (E) values were shown to be ranging from 103 through 233 kJmol⁻¹. Pre-exponential factors (A) indicated the reaction to follow first order kinetics. Gibbs free energy (ΔG) was measured to be ranging from 169 to 173kJmol⁻¹ and 168 to 172kJmol⁻¹, calculated by KAS and FWO methods, respectively. We have shown that Para grass biomass has considerable bioenergy potential comparable to established bioenergy crops such as switchgrass and miscanthus. |
| Author | Ye, Guangbin Qadir, Ghulam Al Ayed, Omar S. Arbi Nehdi, Imededdine Ahmad, Muhammad Sajjad Ibrahim, Muhammad Rashid, Umer Luo, Huibo Mehmood, Muhammad Aamer |
| Author_xml | – sequence: 1 givenname: Muhammad Sajjad surname: Ahmad fullname: Ahmad, Muhammad Sajjad organization: Bioenergy Research Centre, Department of Bioinformatics & Biotechnology, Government College University Faisalabad, Faisalabad 38000, Pakistan – sequence: 2 givenname: Muhammad Aamer surname: Mehmood fullname: Mehmood, Muhammad Aamer email: draamer@gcuf.edu.pk organization: Bioenergy Research Centre, Department of Bioinformatics & Biotechnology, Government College University Faisalabad, Faisalabad 38000, Pakistan – sequence: 3 givenname: Omar S. surname: Al Ayed fullname: Al Ayed, Omar S. organization: Department of Chemical Engineering, Al-Balqa’a Applied University, Amman, Jordan – sequence: 4 givenname: Guangbin surname: Ye fullname: Ye, Guangbin organization: College of Bioengineering, Sichuan University of Science and Engineering, Zigong 643000, People’s Republic of China – sequence: 5 givenname: Huibo surname: Luo fullname: Luo, Huibo organization: College of Bioengineering, Sichuan University of Science and Engineering, Zigong 643000, People’s Republic of China – sequence: 6 givenname: Muhammad surname: Ibrahim fullname: Ibrahim, Muhammad organization: Department of Environmental Sciences & Engineering, Government College University Faisalabad, Faisalabad 38000, Pakistan – sequence: 7 givenname: Umer surname: Rashid fullname: Rashid, Umer organization: Institute of Advanced Technology, Universiti Putra Malaysia, 43400 UPM Serdang, Selangor, Malaysia – sequence: 8 givenname: Imededdine surname: Arbi Nehdi fullname: Arbi Nehdi, Imededdine organization: Chemistry Department, College of Science, King Saud University, Riyadh 1145, Saudi Arabia – sequence: 9 givenname: Ghulam surname: Qadir fullname: Qadir, Ghulam organization: Soil Salinity Research Institute, Pindi Bhattian, Pakistan |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27838316$$D View this record in MEDLINE/PubMed |
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| Snippet | •Para grass is a source of low-cost and abundant biomass.•TGA-DSC analyses were performed to understand kinetics of pyrolysis.•Thermodynamics parameters... The biomass of Urochloa mutica was subjected to thermal degradation analyses to understand its pyrolytic behavior for bioenergy production. Thermal degradation... |
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| SubjectTerms | activation energy Bioenergy Biofuels Biomass calorimetry Gibbs free energy Heating Kinetics Low cost biomass Models, Theoretical Panicum virgatum Poaceae - chemistry Pyrolysis technology TGA-DSC analyses thermal degradation Thermodynamics Thermogravimetry Urochloa mutica |
| Title | Kinetic analyses and pyrolytic behavior of Para grass (Urochloa mutica) for its bioenergy potential |
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