Recent advances in application of graphitic carbon nitride-based catalysts for degrading organic contaminants in water through advanced oxidation processes beyond photocatalysis: A critical review
•Recent advances of g-C3N4-based catalysts in AOPs beyond photocatalysis are reviewed.•Catalytic performance and involved mechanism are summarized.•Effect of water chemistry on catalytic performance is discussed.•Reusability and stability in water treatment are mentioned.•Future prospects in real en...
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| Published in | Water research (Oxford) Vol. 184; p. 116200 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.10.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | •Recent advances of g-C3N4-based catalysts in AOPs beyond photocatalysis are reviewed.•Catalytic performance and involved mechanism are summarized.•Effect of water chemistry on catalytic performance is discussed.•Reusability and stability in water treatment are mentioned.•Future prospects in real environmental applications are proposed.
Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic contaminants. Graphitic carbon nitride (g-C3N4)-based catalysts with high performance and cost effectiveness are promising heterogeneous catalysts for AOPs. Most research on g-C3N4-based catalysts focuses on photocatalytic oxidation, but increasingly researchers are paying attention to the application of g-C3N4-based catalysts in other AOPs beyond photocatalysis. This review aims to concisely highlight recent state-of-the-art progress of g-C3N4-based catalysts in AOPs beyond photocatalysis. Emphasis is made on the application of g-C3N4-based catalysts in three classical AOPs including Fenton-based processes, catalytic ozonation and persulfates activation. The catalytic performance and involved mechanism of g-C3N4-based catalysts in these AOPs are discussed in detail. Meanwhile, the effect of water chemistry including pH, water temperature, natural organic matter, inorganic anions and dissolved oxygen on the catalytic performance of g-C3N4-based catalysts are summarized. Moreover, the reusability, stability and toxicity of g-C3N4-based catalysts in water treatment are also mentioned. Lastly, perspectives on the major challenges and opportunities of g-C3N4-based catalysts in these AOPs are proposed for better developments in the future research.
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| AbstractList | Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic contaminants. Graphitic carbon nitride (g-C3N4)-based catalysts with high performance and cost effectiveness are promising heterogeneous catalysts for AOPs. Most research on g-C3N4-based catalysts focuses on photocatalytic oxidation, but increasingly researchers are paying attention to the application of g-C3N4-based catalysts in other AOPs beyond photocatalysis. This review aims to concisely highlight recent state-of-the-art progress of g-C3N4-based catalysts in AOPs beyond photocatalysis. Emphasis is made on the application of g-C3N4-based catalysts in three classical AOPs including Fenton-based processes, catalytic ozonation and persulfates activation. The catalytic performance and involved mechanism of g-C3N4-based catalysts in these AOPs are discussed in detail. Meanwhile, the effect of water chemistry including pH, water temperature, natural organic matter, inorganic anions and dissolved oxygen on the catalytic performance of g-C3N4-based catalysts are summarized. Moreover, the reusability, stability and toxicity of g-C3N4-based catalysts in water treatment are also mentioned. Lastly, perspectives on the major challenges and opportunities of g-C3N4-based catalysts in these AOPs are proposed for better developments in the future research.Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic contaminants. Graphitic carbon nitride (g-C3N4)-based catalysts with high performance and cost effectiveness are promising heterogeneous catalysts for AOPs. Most research on g-C3N4-based catalysts focuses on photocatalytic oxidation, but increasingly researchers are paying attention to the application of g-C3N4-based catalysts in other AOPs beyond photocatalysis. This review aims to concisely highlight recent state-of-the-art progress of g-C3N4-based catalysts in AOPs beyond photocatalysis. Emphasis is made on the application of g-C3N4-based catalysts in three classical AOPs including Fenton-based processes, catalytic ozonation and persulfates activation. The catalytic performance and involved mechanism of g-C3N4-based catalysts in these AOPs are discussed in detail. Meanwhile, the effect of water chemistry including pH, water temperature, natural organic matter, inorganic anions and dissolved oxygen on the catalytic performance of g-C3N4-based catalysts are summarized. Moreover, the reusability, stability and toxicity of g-C3N4-based catalysts in water treatment are also mentioned. Lastly, perspectives on the major challenges and opportunities of g-C3N4-based catalysts in these AOPs are proposed for better developments in the future research. Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic contaminants. Graphitic carbon nitride (g-C₃N₄)-based catalysts with high performance and cost effectiveness are promising heterogeneous catalysts for AOPs. Most research on g-C₃N₄-based catalysts focuses on photocatalytic oxidation, but increasingly researchers are paying attention to the application of g-C₃N₄-based catalysts in other AOPs beyond photocatalysis. This review aims to concisely highlight recent state-of-the-art progress of g-C₃N₄-based catalysts in AOPs beyond photocatalysis. Emphasis is made on the application of g-C₃N₄-based catalysts in three classical AOPs including Fenton-based processes, catalytic ozonation and persulfates activation. The catalytic performance and involved mechanism of g-C₃N₄-based catalysts in these AOPs are discussed in detail. Meanwhile, the effect of water chemistry including pH, water temperature, natural organic matter, inorganic anions and dissolved oxygen on the catalytic performance of g-C₃N₄-based catalysts are summarized. Moreover, the reusability, stability and toxicity of g-C₃N₄-based catalysts in water treatment are also mentioned. Lastly, perspectives on the major challenges and opportunities of g-C₃N₄-based catalysts in these AOPs are proposed for better developments in the future research. •Recent advances of g-C3N4-based catalysts in AOPs beyond photocatalysis are reviewed.•Catalytic performance and involved mechanism are summarized.•Effect of water chemistry on catalytic performance is discussed.•Reusability and stability in water treatment are mentioned.•Future prospects in real environmental applications are proposed. Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic contaminants. Graphitic carbon nitride (g-C3N4)-based catalysts with high performance and cost effectiveness are promising heterogeneous catalysts for AOPs. Most research on g-C3N4-based catalysts focuses on photocatalytic oxidation, but increasingly researchers are paying attention to the application of g-C3N4-based catalysts in other AOPs beyond photocatalysis. This review aims to concisely highlight recent state-of-the-art progress of g-C3N4-based catalysts in AOPs beyond photocatalysis. Emphasis is made on the application of g-C3N4-based catalysts in three classical AOPs including Fenton-based processes, catalytic ozonation and persulfates activation. The catalytic performance and involved mechanism of g-C3N4-based catalysts in these AOPs are discussed in detail. Meanwhile, the effect of water chemistry including pH, water temperature, natural organic matter, inorganic anions and dissolved oxygen on the catalytic performance of g-C3N4-based catalysts are summarized. Moreover, the reusability, stability and toxicity of g-C3N4-based catalysts in water treatment are also mentioned. Lastly, perspectives on the major challenges and opportunities of g-C3N4-based catalysts in these AOPs are proposed for better developments in the future research. [Display omitted] |
| ArticleNumber | 116200 |
| Author | Huang, Danlian Zeng, Guangming Zhang, Chen Song, Biao Guo, Hai Tang, Xiang Wang, Wenjun Yang, Yang Zhou, Chengyun Xiong, Weiping Li, Xiaopei Li, Xin |
| Author_xml | – sequence: 1 givenname: Yang surname: Yang fullname: Yang, Yang organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 2 givenname: Xin surname: Li fullname: Li, Xin organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 3 givenname: Chengyun surname: Zhou fullname: Zhou, Chengyun organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 4 givenname: Weiping surname: Xiong fullname: Xiong, Weiping organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 5 givenname: Guangming orcidid: 0000-0002-4230-7647 surname: Zeng fullname: Zeng, Guangming email: zgming@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 6 givenname: Danlian surname: Huang fullname: Huang, Danlian email: huangdanlian@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 7 givenname: Chen orcidid: 0000-0002-3579-6980 surname: Zhang fullname: Zhang, Chen email: zhangchen@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 8 givenname: Wenjun surname: Wang fullname: Wang, Wenjun organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 9 givenname: Biao surname: Song fullname: Song, Biao organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 10 givenname: Xiang surname: Tang fullname: Tang, Xiang organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 11 givenname: Xiaopei surname: Li fullname: Li, Xiaopei organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China – sequence: 12 givenname: Hai surname: Guo fullname: Guo, Hai organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China |
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| Snippet | •Recent advances of g-C3N4-based catalysts in AOPs beyond photocatalysis are reviewed.•Catalytic performance and involved mechanism are summarized.•Effect of... Advanced oxidation processes (AOPs) have attracted much interest in the field of water treatment owing to their high removal efficiency for refractory organic... |
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| SubjectTerms | Advanced oxidation processes Carbon nitride cost effectiveness Degradation dissolved oxygen graphene hydrochemistry organic matter Organic pollutants oxidation ozonation photocatalysis toxicity water water pollution water temperature Water treatment |
| Title | Recent advances in application of graphitic carbon nitride-based catalysts for degrading organic contaminants in water through advanced oxidation processes beyond photocatalysis: A critical review |
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