Phosphate adsorption on metal oxides and metal hydroxides: A comparative review
Phosphorus removal from wastewater is important for eutrophication control of water bodies. Metal oxides and metal hydroxides have always been developed and investigated for phosphorus removal, because of their abundance, low cost, environmental friendliness, and chemically stability. This paper pre...
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| Published in | Environmental reviews Vol. 24; no. 3; pp. 319 - 332 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
NRC Research Press
2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Phosphorus removal from wastewater is important for eutrophication control of water bodies. Metal oxides and metal hydroxides have always been developed and investigated for phosphorus removal, because of their abundance, low cost, environmental friendliness, and chemically stability. This paper presents a comparative review of the literature on the preparation methods, adsorption behaviors, adsorption mechanisms, and the regeneration of metal (hydr)oxides (e.g., Fe, Zn, Al, etc.) with regard to phosphate removal. The contrasting results showed that metal hydroxides could offer an effective and economic alternative to metal oxides, because of their cost–benefit synthesis methods, higher adsorption capacities, and shorter adsorption equilibrium times. However, the specific surface area of metal oxides is larger than that of metal hydroxides because of the calcination process. Metal oxides with a higher pH at the zero point of charge have wider optimal adsorption pH ranges than metal hydroxides because of their surface precipitation in alkaline solutions. The regeneration of metal oxides using acids, bases, and salts and that of metal hydroxides using acids and bases has been critically examined. Further research on uniform metal (hydr)oxides with small particle size, high stabilities, low cost, and that are easily regenerated with promising desorbents are proposed. In addition, quantitative mechanism study and application in continuous-mode column trials are also suggested. |
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| AbstractList | Phosphorus removal from wastewater is important for eutrophication control of water bodies. Metal oxides and metal hydroxides have always been developed and investigated for phosphorus removal, because of their abundance, low cost, environmental friendliness, and chemically stability. This paper presents a comparative review of the literature on the preparation methods, adsorption behaviors, adsorption mechanisms, and the regeneration of metal (hydr)oxides (e.g., Fe, Zn, Al, etc.) with regard to phosphate removal. The contrasting results showed that metal hydroxides could offer an effective and economic alternative to metal oxides, because of their cost–benefit synthesis methods, higher adsorption capacities, and shorter adsorption equilibrium times. However, the specific surface area of metal oxides is larger than that of metal hydroxides because of the calcination process. Metal oxides with a higher pH at the zero point of charge have wider optimal adsorption pH ranges than metal hydroxides because of their surface precipitation in alkaline solutions. The regeneration of metal oxides using acids, bases, and salts and that of metal hydroxides using acids and bases has been critically examined. Further research on uniform metal (hydr)oxides with small particle size, high stabilities, low cost, and that are easily regenerated with promising desorbents are proposed. In addition, quantitative mechanism study and application in continuous-mode column trials are also suggested. Phosphorus removal from wastewater is important for eutrophication control of water bodies. Metal oxides and metal hydroxides have always been developed and investigated for phosphorus removal, because of their abundance, low cost, environmental friendliness, and chemically stability. This paper presents a comparative review of the literature on the preparation methods, adsorption behaviors, adsorption mechanisms, and the regeneration of metal (hydr)oxides (e.g., Fe, Zn, Al, etc.) with regard to phosphate removal. The contrasting results showed that metal hydroxides could offer an effective and economic alternative to metal oxides, because of their cost-benefit synthesis methods, higher adsorption capacities, and shorter adsorption equilibrium times. However, the specific surface area of metal oxides is larger than that of metal hydroxides because of the calcination process. Metal oxides with a higher pH at the zero point of charge have wider optimal adsorption pH ranges than metal hydroxides because of their surface precipitation in alkaline solutions. The regeneration of metal oxides using acids, bases, and salts and that of metal hydroxides using acids and bases has been critically examined. Further research on uniform metal (hydr)oxides with small particle size, high stabilities, low cost, and that are easily regenerated with promising desorbents are proposed. In addition, quantitative mechanism study and application in continuous-mode column trials are also suggested.Original Abstract: L'elimination du phosphore des eaux usees est une maniere importante de controler l'eutrophisation des plans d'eau. Les oxydes metalliques et les hydroxydes metalliques ont toujours ete developpes et examines aux fins de l'elimination du phosphore, en raison de leur abondance, leur cout minime, leur respect de l'environnement et leur stabilite chimique. Cet article presente une revue comparative des litteratures sur les methodes de preparation, les comportements d'adsorption, les mecanismes d'adsorption et la regeneration des hydr(oxydes) metalliques (p. ex., Fe, Zn et Al) en ce qui concerne l'elimination du phosphate. Les differences de resultats ont montre que les hydroxydes metalliques peuvent offrir une alternative efficace et economique aux oxydes metalliques, en raison de leurs methodes de synthese a cout avantageux, leurs fortes capacites d'adsorption et leur temps d'atteinte d'equilibre d'adsorption plus court. Cependant, la surface specifique des oxydes metalliques est plus grande que celle des hydroxydes metalliques en raison du procede de calcination. Les oxydes metalliques ayant un pH au point de charge nulle plus eleve ont une gamme de pH plus large pour l'adsorption optimale qu'en ont les hydroxydes en raison de leur precipitation de surface dans les solutions alcalines. La regeneration des oxydes metalliques au moyen d'acides, de bases et de sels et celle des hydroxydes au moyen d'acides et de bases ont fait l'objet d'examens critiques. On propose de plus amples recherches sur les (hydr)oxydes metalliques uniformes ayant une petite dimension de la particule, une haute stabilite, un cout avantageux et etant facilement regeneres a l'aide de desorbants prometteurs. De plus, on suggere aussi une etude quantitative des mecanismes et l'application d'essais de colonne en mode continue (<< continuous-mode column trials >>). [Traduit par la Redaction] |
| Abstract_FL | L’élimination du phosphore des eaux usées est une manière importante de contrôler l’eutrophisation des plans d’eau. Les oxydes métalliques et les hydroxydes métalliques ont toujours été développés et examinés aux fins de l’élimination du phosphore, en raison de leur abondance, leur coût minime, leur respect de l’environnement et leur stabilité chimique. Cet article présente une revue comparative des littératures sur les méthodes de préparation, les comportements d’adsorption, les mécanismes d’adsorption et la régénération des hydr(oxydes) métalliques (p. ex., Fe, Zn et Al) en ce qui concerne l’élimination du phosphate. Les différences de résultats ont montré que les hydroxydes métalliques peuvent offrir une alternative efficace et économique aux oxydes métalliques, en raison de leurs méthodes de synthèse à coût avantageux, leurs fortes capacités d’adsorption et leur temps d’atteinte d’équilibre d’adsorption plus court. Cependant, la surface spécifique des oxydes métalliques est plus grande que celle des hydroxydes métalliques en raison du procédé de calcination. Les oxydes métalliques ayant un pH au point de charge nulle plus élevé ont une gamme de pH plus large pour l’adsorption optimale qu’en ont les hydroxydes en raison de leur précipitation de surface dans les solutions alcalines. La régénération des oxydes métalliques au moyen d’acides, de bases et de sels et celle des hydroxydes au moyen d’acides et de bases ont fait l’objet d’examens critiques. On propose de plus amples recherches sur les (hydr)oxydes métalliques uniformes ayant une petite dimension de la particule, une haute stabilité, un coût avantageux et étant facilement régénérés à l’aide de désorbants prometteurs. De plus, on suggère aussi une étude quantitative des mécanismes et l’application d’essais de colonne en mode continue (« continuous-mode column trials »). [Traduit par la Rédaction] |
| Author | Mengxue Li Yunfeng Xu Guangren Qian Jianyong Liu |
| Author_xml | – sequence: 1 givenname: Mengxue surname: Li fullname: Li, Mengxue organization: School of Environmental and Chemical Engineering, Shanghai University, 333 Nanchen Road, Shanghai 200444, P.R. China – sequence: 2 givenname: Jianyong surname: Liu fullname: Liu, Jianyong organization: School of Environmental and Chemical Engineering, Shanghai University, 333 Nanchen Road, Shanghai 200444, P.R. China – sequence: 3 givenname: Yunfeng surname: Xu fullname: Xu, Yunfeng organization: School of Environmental and Chemical Engineering, Shanghai University, 333 Nanchen Road, Shanghai 200444, P.R. China – sequence: 4 givenname: Guangren surname: Qian fullname: Qian, Guangren organization: School of Environmental and Chemical Engineering, Shanghai University, 333 Nanchen Road, Shanghai 200444, P.R. China |
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| Snippet | Phosphorus removal from wastewater is important for eutrophication control of water bodies. Metal oxides and metal hydroxides have always been developed and... |
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| SubjectTerms | acids adsorption adsorption du phosphate aluminum chemical bases eutrophication hydroxides hydroxydes métalliques iron metal hydroxides metal oxides oxides oxydes métalliques particle size phosphate adsorption phosphates phosphorus surface area surface water wastewater zinc |
| Title | Phosphate adsorption on metal oxides and metal hydroxides: A comparative review |
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