Mechanically robust honeycomb graphene aerogel multifunctional polymer composites
This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)–polydimethylsiloxane (PDMS) composites (GAPC) with outstanding mechanical, electrical and thermal properties. GAPC was fabricated by impregnating 3D GA frameworks with PDMS via ice-bath-assisted in...
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| Published in | Carbon (New York) Vol. 93; pp. 659 - 670 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.11.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)–polydimethylsiloxane (PDMS) composites (GAPC) with outstanding mechanical, electrical and thermal properties. GAPC was fabricated by impregnating 3D GA frameworks with PDMS via ice-bath-assisted infiltration and vacuum curing processes. Because of the well-interconnected 3D GA frameworks, GAPC exhibits extremely large deformability (compressive strain=80% and tensile strain=90%), high electrical and thermal conductivities (1S/cm and 0.68W/(mK), respectively), a stable piezo-resistance effect, rapid electric Joule heating performance ((dT/dt)max>3°C/s under a heating power of 12W/cm3), and high hydrophobicity (contact angle=135°). Furthermore, GAPC exhibits a negative temperature coefficient of expansion with decreased electrical resistivity over a broad temperature range, indicating a typical semiconducting behavior and a dual two-dimensional/3D hopping conduction mechanism. |
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| AbstractList | This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)–polydimethylsiloxane (PDMS) composites (GAPC) with outstanding mechanical, electrical and thermal properties. GAPC was fabricated by impregnating 3D GA frameworks with PDMS via ice-bath-assisted infiltration and vacuum curing processes. Because of the well-interconnected 3D GA frameworks, GAPC exhibits extremely large deformability (compressive strain=80% and tensile strain=90%), high electrical and thermal conductivities (1S/cm and 0.68W/(mK), respectively), a stable piezo-resistance effect, rapid electric Joule heating performance ((dT/dt)max>3°C/s under a heating power of 12W/cm3), and high hydrophobicity (contact angle=135°). Furthermore, GAPC exhibits a negative temperature coefficient of expansion with decreased electrical resistivity over a broad temperature range, indicating a typical semiconducting behavior and a dual two-dimensional/3D hopping conduction mechanism. This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)-polydimethylsiloxane (PDMS) composites (GAPC) with outstanding mechanical, electrical and thermal properties. GAPC was fabricated by impregnating 3D GA frameworks with PDMS via ice-bath-assisted infiltration and vacuum curing processes. Because of the well-interconnected 3D GA frameworks, GAPC exhibits extremely large deformability (compressive strain = 80% and tensile strain = 90%), high electrical and thermal conductivities (1 S/cm and 0.68 W/(m K), respectively), a stable piezo-resistance effect, rapid electric Joule heating performance ((dT/dt) sub(max) > 3 [degrees]C/s under a heating power of 12 W/cm super(3)), and high hydrophobicity (contact angle = 135[degrees]). Furthermore, GAPC exhibits a negative temperature coefficient of expansion with decreased electrical resistivity over a broad temperature range, indicating a typical semiconducting behavior and a dual two-dimensional/3D hopping conduction mechanism. |
| Author | Li, Hui Zhang, Qiangqiang Xiong, Guoping Fisher, Timothy S. Xu, Xiang Hu, Han |
| Author_xml | – sequence: 1 givenname: Qiangqiang surname: Zhang fullname: Zhang, Qiangqiang organization: Key Lab of Structures Dynamic Behavior and Control (Harbin Institute of Technology), Ministry of Education, Harbin 150090, PR China – sequence: 2 givenname: Xiang surname: Xu fullname: Xu, Xiang organization: Key Lab of Structures Dynamic Behavior and Control (Harbin Institute of Technology), Ministry of Education, Harbin 150090, PR China – sequence: 3 givenname: Hui surname: Li fullname: Li, Hui email: lihui@hit.edu.cn organization: Key Lab of Structures Dynamic Behavior and Control (Harbin Institute of Technology), Ministry of Education, Harbin 150090, PR China – sequence: 4 givenname: Guoping surname: Xiong fullname: Xiong, Guoping organization: School of Mechanical Engineering, Purdue University, West Lafayette, IN 47907, USA – sequence: 5 givenname: Han surname: Hu fullname: Hu, Han organization: Liaoning Key Lab for Energy Materials and Chemical Engineering, State Key Lab of Fine Chemicals, Dalian University of Technology, Dalian 116024, PR China – sequence: 6 givenname: Timothy S. surname: Fisher fullname: Fisher, Timothy S. organization: School of Mechanical Engineering, Purdue University, West Lafayette, IN 47907, USA |
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| Snippet | This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)–polydimethylsiloxane (PDMS) composites (GAPC) with... This work reports the fabrication and characterization of three-dimensional (3D) graphene aerogel (GA)-polydimethylsiloxane (PDMS) composites (GAPC) with... |
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| SubjectTerms | Aerogels Carbon Contact angle electrical resistance Graphene heat hydrophobicity polymers Silicone resins Strain temperature Thermal properties Three dimensional |
| Title | Mechanically robust honeycomb graphene aerogel multifunctional polymer composites |
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