Cr(VI) removal from aqueous solution using biochar modified with Mg/Al-layered double hydroxide intercalated with ethylenediaminetetraacetic acid
•Biochar loaded with nanoparticles was prepared for Cr(VI) adsorption.•EDTA intercalated LDH significantly improved sorption capacity of Cr(VI).•Adsorption process obeys chemisorption and monolayer adsorption. In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) inter...
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| Published in | Bioresource technology Vol. 276; pp. 127 - 132 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.03.2019
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 0960-8524 1873-2976 1873-2976 |
| DOI | 10.1016/j.biortech.2018.12.114 |
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| Abstract | •Biochar loaded with nanoparticles was prepared for Cr(VI) adsorption.•EDTA intercalated LDH significantly improved sorption capacity of Cr(VI).•Adsorption process obeys chemisorption and monolayer adsorption.
In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr2O72− and OH– increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater. |
|---|---|
| AbstractList | In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr
O
and OH
increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater. •Biochar loaded with nanoparticles was prepared for Cr(VI) adsorption.•EDTA intercalated LDH significantly improved sorption capacity of Cr(VI).•Adsorption process obeys chemisorption and monolayer adsorption. In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr2O72− and OH– increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater. In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr2O72− and OH– increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater. In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr2O72- and OH- increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater.In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain a novel nano-adsorbent (BC@EDTA-LDH), and BC@EDTA-LDH was used to remove hexavalent chromium (Cr(VI)) in aqueous solutions. The results showed that the interaction between LDH and Cr(VI) on biochar played a dominant part in adsorption. The LDH of Cr(VI) intercalation was successfully reconstructed after adsorption. Fourier transform infrared spectra and X-ray diffraction results confirmed the reconstruction of Mg/Al-LDH. LDH had sustained release effect on the solution. As the pH values increased, the electrostatic repulsion between Cr2O72- and OH- increased, and there existed competition for adsorption sites. The maximum adsorption capacity of Cr(VI) was 38 mg/g. The data was well-fitted with pseudo second-order model and Langmuir-Freundlich model. BC@EDTA-LDH showed a high adsorption capacity and was potentially suitable for removing heavy metals in wastewater. |
| Author | Huang, Danlian Zeng, Guangming Guo, Xueying Luo, Hao Zhang, Chen Deng, Rui Wang, Rongzhong Liu, Caihong Xue, Wenjing Zhang, Qing |
| Author_xml | – sequence: 1 givenname: Danlian surname: Huang fullname: Huang, Danlian email: huangdanlian@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 2 givenname: Caihong surname: Liu fullname: Liu, Caihong organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 3 givenname: Chen orcidid: 0000-0002-3579-6980 surname: Zhang fullname: Zhang, Chen organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 4 givenname: Rui surname: Deng fullname: Deng, Rui organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 5 givenname: Rongzhong surname: Wang fullname: Wang, Rongzhong organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 6 givenname: Wenjing surname: Xue fullname: Xue, Wenjing organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 7 givenname: Hao surname: Luo fullname: Luo, Hao organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 8 givenname: Guangming surname: Zeng fullname: Zeng, Guangming organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 9 givenname: Qing surname: Zhang fullname: Zhang, Qing organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 10 givenname: Xueying surname: Guo fullname: Guo, Xueying organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30616211$$D View this record in MEDLINE/PubMed |
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| Keywords | Cr(VI) Adsorption Biochar Layered double hydroxides |
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| Snippet | •Biochar loaded with nanoparticles was prepared for Cr(VI) adsorption.•EDTA intercalated LDH significantly improved sorption capacity of Cr(VI).•Adsorption... In this study, the bamboo biomass loaded with ethylenediaminetetraacetic acid (EDTA) intercalated Mg/Al-layered double hydroxides (LDH) was calcined to obtain... |
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| SubjectTerms | Adsorption aqueous solutions bamboos Biochar biomass chromium Cr(VI) EDTA (chelating agent) electrostatic interactions Fourier transform infrared spectroscopy heavy metals hydroxides Layered double hydroxides wastewater X-ray diffraction |
| Title | Cr(VI) removal from aqueous solution using biochar modified with Mg/Al-layered double hydroxide intercalated with ethylenediaminetetraacetic acid |
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