Calcium-rich biochar from crab shell: An unexpected super adsorbent for dye removal
•Calcium-rich biochar (CRB) was directly from crab shell without modification.•CRB showed unprecedented adsorption performance for both cationic and anionic dyes.•CRB could adsorb >10,000 mg/g malachite green.•Congo red adsorption on CRB equilibrated in 2 min with a capacity >20,000 mg/g.•CRB...
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| Published in | Bioresource technology Vol. 267; pp. 510 - 516 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.11.2018
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| Subjects | |
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| Abstract | •Calcium-rich biochar (CRB) was directly from crab shell without modification.•CRB showed unprecedented adsorption performance for both cationic and anionic dyes.•CRB could adsorb >10,000 mg/g malachite green.•Congo red adsorption on CRB equilibrated in 2 min with a capacity >20,000 mg/g.•CRB was a low-cost but excellent dye adsorbent, thus promising in dye removal.
Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here, calcium-rich biochar (CRB) as a low-cost adsorbent was directly prepared from crab shell via a simple pyrolysis process without any modification. Batch adsorption results suggested that CRB was among the dye adsorbents with highest adsorption capacities and fastest adsorption rate. Specifically, it showed high adsorption capacities of 12,502 and 20,317 mg/g for cationic malachite green and anionic Congo red, respectively. The adsorption equilibrium for Congo red onto CRB could be achieved as short as 2 min. Furthermore, the dye adsorption mechanism for CRB, as investigated by zeta potential and FTIR spectra, could be attributed to electrostatic attraction, hydrogen bonding and π-π interaction. Finally, this study suggested that, attributed to its cheap source, simple synthesis process and excellent adsorption performance, CRB was promising in dye removal. |
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| AbstractList | Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here, calcium-rich biochar (CRB) as a low-cost adsorbent was directly prepared from crab shell via a simple pyrolysis process without any modification. Batch adsorption results suggested that CRB was among the dye adsorbents with highest adsorption capacities and fastest adsorption rate. Specifically, it showed high adsorption capacities of 12,502 and 20,317 mg/g for cationic malachite green and anionic Congo red, respectively. The adsorption equilibrium for Congo red onto CRB could be achieved as short as 2 min. Furthermore, the dye adsorption mechanism for CRB, as investigated by zeta potential and FTIR spectra, could be attributed to electrostatic attraction, hydrogen bonding and π-π interaction. Finally, this study suggested that, attributed to its cheap source, simple synthesis process and excellent adsorption performance, CRB was promising in dye removal. •Calcium-rich biochar (CRB) was directly from crab shell without modification.•CRB showed unprecedented adsorption performance for both cationic and anionic dyes.•CRB could adsorb >10,000 mg/g malachite green.•Congo red adsorption on CRB equilibrated in 2 min with a capacity >20,000 mg/g.•CRB was a low-cost but excellent dye adsorbent, thus promising in dye removal. Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here, calcium-rich biochar (CRB) as a low-cost adsorbent was directly prepared from crab shell via a simple pyrolysis process without any modification. Batch adsorption results suggested that CRB was among the dye adsorbents with highest adsorption capacities and fastest adsorption rate. Specifically, it showed high adsorption capacities of 12,502 and 20,317 mg/g for cationic malachite green and anionic Congo red, respectively. The adsorption equilibrium for Congo red onto CRB could be achieved as short as 2 min. Furthermore, the dye adsorption mechanism for CRB, as investigated by zeta potential and FTIR spectra, could be attributed to electrostatic attraction, hydrogen bonding and π-π interaction. Finally, this study suggested that, attributed to its cheap source, simple synthesis process and excellent adsorption performance, CRB was promising in dye removal. Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here, calcium-rich biochar (CRB) as a low-cost adsorbent was directly prepared from crab shell via a simple pyrolysis process without any modification. Batch adsorption results suggested that CRB was among the dye adsorbents with highest adsorption capacities and fastest adsorption rate. Specifically, it showed high adsorption capacities of 12,502 and 20,317 mg/g for cationic malachite green and anionic Congo red, respectively. The adsorption equilibrium for Congo red onto CRB could be achieved as short as 2 min. Furthermore, the dye adsorption mechanism for CRB, as investigated by zeta potential and FTIR spectra, could be attributed to electrostatic attraction, hydrogen bonding and π-π interaction. Finally, this study suggested that, attributed to its cheap source, simple synthesis process and excellent adsorption performance, CRB was promising in dye removal.Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here, calcium-rich biochar (CRB) as a low-cost adsorbent was directly prepared from crab shell via a simple pyrolysis process without any modification. Batch adsorption results suggested that CRB was among the dye adsorbents with highest adsorption capacities and fastest adsorption rate. Specifically, it showed high adsorption capacities of 12,502 and 20,317 mg/g for cationic malachite green and anionic Congo red, respectively. The adsorption equilibrium for Congo red onto CRB could be achieved as short as 2 min. Furthermore, the dye adsorption mechanism for CRB, as investigated by zeta potential and FTIR spectra, could be attributed to electrostatic attraction, hydrogen bonding and π-π interaction. Finally, this study suggested that, attributed to its cheap source, simple synthesis process and excellent adsorption performance, CRB was promising in dye removal. |
| Author | Tan, Furong Zhou, Qin Zhu, Nengmin Zhu, Wenkun He, Mingxiong Dai, Lichun He, Li Hu, Guoquan |
| Author_xml | – sequence: 1 givenname: Lichun surname: Dai fullname: Dai, Lichun email: dailichun@caas.cn organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China – sequence: 2 givenname: Wenkun surname: Zhu fullname: Zhu, Wenkun organization: Sichuan Co-Innovation Center for New Energetic Materials, Southwest University of Science and Technology, Mianyang 621010, China – sequence: 3 givenname: Li surname: He fullname: He, Li organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China – sequence: 4 givenname: Furong surname: Tan fullname: Tan, Furong organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China – sequence: 5 givenname: Nengmin surname: Zhu fullname: Zhu, Nengmin organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China – sequence: 6 givenname: Qin surname: Zhou fullname: Zhou, Qin organization: Key Laboratory of Environmental Nano-Technology and Health Effect, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China – sequence: 7 givenname: Mingxiong surname: He fullname: He, Mingxiong organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China – sequence: 8 givenname: Guoquan surname: Hu fullname: Hu, Guoquan organization: Biogas Institute of Ministry of Agriculture, Chengdu 610041, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30048926$$D View this record in MEDLINE/PubMed |
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| PublicationTitle | Bioresource technology |
| PublicationTitleAlternate | Bioresour Technol |
| PublicationYear | 2018 |
| Publisher | Elsevier Ltd |
| Publisher_xml | – name: Elsevier Ltd |
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| Snippet | •Calcium-rich biochar (CRB) was directly from crab shell without modification.•CRB showed unprecedented adsorption performance for both cationic and anionic... Adsorption is the common-used method to remove dyes from wastewater, and many efforts have been made to develop low-cost but excellent adsorbents. Here,... |
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| SubjectTerms | adsorbents Adsorption Biochar Congo red Crab shell crabs Dye electrostatic interactions Fourier transform infrared spectroscopy hydrogen bonding Malachite green pyrolysis wastewater zeta potential |
| Title | Calcium-rich biochar from crab shell: An unexpected super adsorbent for dye removal |
| URI | https://dx.doi.org/10.1016/j.biortech.2018.07.090 https://www.ncbi.nlm.nih.gov/pubmed/30048926 https://www.proquest.com/docview/2078585295 https://www.proquest.com/docview/2116928756 |
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