OPAC (orange peel activated carbon) derived from waste orange peel for the adsorption of chlorophenoxyacetic acid herbicides from water: Adsorption isotherm, kinetic modelling and thermodynamic studies

[Display omitted] •Low-cost carbon – adsorbent was prepared from orange peel waste by simple method.•The synthesised orange peel activated carbon surface area was 592.471 m2 g−1.•Adsorption mechanism and kinetics studies of highly hazardous chlorophenoxy herbicides from aqueous was studied.•Maximum...

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Published in	Bioresource technology Vol. 261; pp. 329 - 341
Main Authors	Pandiarajan, Aarthi, Kamaraj, Ramakrishnan, Vasudevan, Sudharshan, Vasudevan, Subramanyan
Format	Journal Article
Language	English
Published	England Elsevier Ltd 01.08.2018
Subjects	adsorbents Adsorption Carbon Citrus sinensis Herbicide herbicides Herbicides - chemistry Hydrogen-Ion Concentration Isotherm Kinetics Modelling Orange peel activated carbon (OPAC) orange peels pyrolysis sorption isotherms surface area temperature Thermodynamic Thermodynamics wastes Water Water Pollutants, Chemical Water Purification Orange peel activated carbon (OPAC) Adsorption Isotherm Modelling Kinetics Herbicide Thermodynamic
Online Access	Get full text
ISSN	0960-8524 1873-2976 1873-2976
DOI	10.1016/j.biortech.2018.04.005

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Abstract	[Display omitted] •Low-cost carbon – adsorbent was prepared from orange peel waste by simple method.•The synthesised orange peel activated carbon surface area was 592.471 m2 g−1.•Adsorption mechanism and kinetics studies of highly hazardous chlorophenoxy herbicides from aqueous was studied.•Maximum Langmuir capacity of 574.71 mg g−1 was achieved. This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m2 g−1, pore volume and pore diameter of 0.242 cc g−1 and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g−1 was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water.
AbstractList	[Display omitted] •Low-cost carbon – adsorbent was prepared from orange peel waste by simple method.•The synthesised orange peel activated carbon surface area was 592.471 m2 g−1.•Adsorption mechanism and kinetics studies of highly hazardous chlorophenoxy herbicides from aqueous was studied.•Maximum Langmuir capacity of 574.71 mg g−1 was achieved. This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m2 g−1, pore volume and pore diameter of 0.242 cc g−1 and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g−1 was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water. This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m2 g−1, pore volume and pore diameter of 0.242 cc g−1 and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g−1 was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water. This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m2 g-1, pore volume and pore diameter of 0.242 cc g-1 and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g-1 was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water.This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m2 g-1, pore volume and pore diameter of 0.242 cc g-1 and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g-1 was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water. This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application for the adsorption of chlorophenoxyacetic acid herbicides from the water. The OPAC exhibited the surface area of 592.471 m  g , pore volume and pore diameter of 0.242 cc g and 1.301 nm respectively. The adsorption kinetics and thermodynamic equilibrium modelling for all chlorophenoxyacetic acid herbicides were investigated. The various parametric effects such as pH and temperature were evaluated. A pseudo-second-order kinetic model was well fitted for all the herbicides. The Langmuir isotherm was obeyed for all the herbicides and the maximum Langmuir capacity of 574.71 mg g was achieved. The thermodynamic studies revealed that the adsorption increases with increase in temperature. The results shows that the orange peel derived carbon (OPAC) as effective and efficient adsorbent material for the removal of chlorophenoxyacid herbicides from the water.
Author	Vasudevan, Sudharshan Vasudevan, Subramanyan Kamaraj, Ramakrishnan Pandiarajan, Aarthi
Author_xml	– sequence: 1 givenname: Aarthi surname: Pandiarajan fullname: Pandiarajan, Aarthi organization: CSIR-Central Electrochemical Research Institute, Karaikudi 630006, India – sequence: 2 givenname: Ramakrishnan surname: Kamaraj fullname: Kamaraj, Ramakrishnan organization: CSIR-Central Electrochemical Research Institute, Karaikudi 630006, India – sequence: 3 givenname: Sudharshan surname: Vasudevan fullname: Vasudevan, Sudharshan organization: Department of Mechanical Engineering, Thiagarajar College of Engineering, Madurai 625015, India – sequence: 4 givenname: Subramanyan surname: Vasudevan fullname: Vasudevan, Subramanyan email: vasudevan65@gmail.com organization: CSIR-Central Electrochemical Research Institute, Karaikudi 630006, India
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/29677661$$D View this record in MEDLINE/PubMed
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Keywords	Orange peel activated carbon (OPAC) Adsorption Isotherm Modelling Kinetics Herbicide Thermodynamic
Language	English
License	Copyright © 2018 Elsevier Ltd. All rights reserved.
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Snippet	[Display omitted] •Low-cost carbon – adsorbent was prepared from orange peel waste by simple method.•The synthesised orange peel activated carbon surface area... This study presents the orange peel activated carbon (OPAC), derived from biowaste precursor (orange peel) by single step pyrolysis method and its application...
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SubjectTerms	adsorbents Adsorption Carbon Citrus sinensis Herbicide herbicides Herbicides - chemistry Hydrogen-Ion Concentration Isotherm Kinetics Modelling Orange peel activated carbon (OPAC) orange peels pyrolysis sorption isotherms surface area temperature Thermodynamic Thermodynamics wastes Water Water Pollutants, Chemical Water Purification
Title	OPAC (orange peel activated carbon) derived from waste orange peel for the adsorption of chlorophenoxyacetic acid herbicides from water: Adsorption isotherm, kinetic modelling and thermodynamic studies
URI	https://dx.doi.org/10.1016/j.biortech.2018.04.005 https://www.ncbi.nlm.nih.gov/pubmed/29677661 https://www.proquest.com/docview/2028952077 https://www.proquest.com/docview/2237523099
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