Efficient bifunctional piezocatalysis of Au/BiVO4 for simultaneous removal of 4-chlorophenol and Cr(VI) in water
[Display omitted] •The piezoelectric effect of Au/BiVO4 is characterized by PFM measurements.•Au/BiVO4 is used as a bifunctional piezocatalyst for removal of pollutants in water.•Simultaneous removal of 4-chlorophenol and Cr(VI) is achieved by piezocatalysis.•H2O2 and OH induced mechanism on Au/BiVO...
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| Published in | Applied catalysis. B, Environmental Vol. 259; p. 118084 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
15.12.2019
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•The piezoelectric effect of Au/BiVO4 is characterized by PFM measurements.•Au/BiVO4 is used as a bifunctional piezocatalyst for removal of pollutants in water.•Simultaneous removal of 4-chlorophenol and Cr(VI) is achieved by piezocatalysis.•H2O2 and OH induced mechanism on Au/BiVO4 piezocatalysis is proposed.
Piezocatalysis induced by polarization of piezoelectric materials is considered as an emerging technology in environmental cleanup. In this work, a piezoelectric material, Au nanoparticles modified BiVO4 (Au/BiVO4) is synthesized and its piezoelectric response is observed by piezo-response force microscopy. Au/BiVO4 is used as a bifunctional piezocatalyst for simultaneous removal of 4-chlorophenol (4-CP) and hexavalent chromium (Cr(VI)) upon ultrasonic vibration, with 91% and 83% of removal efficiency in 120 min, respectively. The piezocatalytic performance of Au/BiVO4 increases with the increase of ultrasonic power and the decrease of pH. The main active species for 4-CP oxidation and Cr(VI) reduction are determined to beOH and H2O2, respectively, since a significant formation rate ofOH is estimated by a probe method, and a high amount of H2O2 accumulation is directly detected. This study provides understanding on the piezocatalysis mechanism and brings new insights for development of piezocatalysis for multifunctional environmental applications. |
|---|---|
| AbstractList | [Display omitted]
•The piezoelectric effect of Au/BiVO4 is characterized by PFM measurements.•Au/BiVO4 is used as a bifunctional piezocatalyst for removal of pollutants in water.•Simultaneous removal of 4-chlorophenol and Cr(VI) is achieved by piezocatalysis.•H2O2 and OH induced mechanism on Au/BiVO4 piezocatalysis is proposed.
Piezocatalysis induced by polarization of piezoelectric materials is considered as an emerging technology in environmental cleanup. In this work, a piezoelectric material, Au nanoparticles modified BiVO4 (Au/BiVO4) is synthesized and its piezoelectric response is observed by piezo-response force microscopy. Au/BiVO4 is used as a bifunctional piezocatalyst for simultaneous removal of 4-chlorophenol (4-CP) and hexavalent chromium (Cr(VI)) upon ultrasonic vibration, with 91% and 83% of removal efficiency in 120 min, respectively. The piezocatalytic performance of Au/BiVO4 increases with the increase of ultrasonic power and the decrease of pH. The main active species for 4-CP oxidation and Cr(VI) reduction are determined to beOH and H2O2, respectively, since a significant formation rate ofOH is estimated by a probe method, and a high amount of H2O2 accumulation is directly detected. This study provides understanding on the piezocatalysis mechanism and brings new insights for development of piezocatalysis for multifunctional environmental applications. Piezocatalysis induced by polarization of piezoelectric materials is considered as an emerging technology in environmental cleanup. In this work, a piezoelectric material, Au nanoparticles modified BiVO4 (Au/BiVO4) is synthesized and its piezoelectric response is observed by piezo-response force microscopy. Au/BiVO4 is used as a bifunctional piezocatalyst for simultaneous removal of 4-chlorophenol (4-CP) and hexavalent chromium (Cr(VI)) upon ultrasonic vibration, with 91% and 83% of removal efficiency in 120 min, respectively. The piezocatalytic performance of Au/BiVO4 increases with the increase of ultrasonic power and the decrease of pH. The main active species for 4-CP oxidation and Cr(VI) reduction are determined to be•OH and H2O2, respectively, since a significant formation rate of•OH is estimated by a probe method, and a high amount of H2O2 accumulation is directly detected. This study provides understanding on the piezocatalysis mechanism and brings new insights for development of piezocatalysis for multifunctional environmental applications. |
| ArticleNumber | 118084 |
| Author | Wei, Yan Zhang, Yiwen Geng, Wei Su, Hanrui Long, Mingce |
| Author_xml | – sequence: 1 givenname: Yan surname: Wei fullname: Wei, Yan – sequence: 2 givenname: Yiwen surname: Zhang fullname: Zhang, Yiwen – sequence: 3 givenname: Wei surname: Geng fullname: Geng, Wei – sequence: 4 givenname: Hanrui surname: Su fullname: Su, Hanrui – sequence: 5 givenname: Mingce orcidid: 0000-0002-5168-8330 surname: Long fullname: Long, Mingce email: long_mc@sjtu.edu.cn |
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•The piezoelectric effect of Au/BiVO4 is characterized by PFM measurements.•Au/BiVO4 is used as a bifunctional piezocatalyst for removal of... Piezocatalysis induced by polarization of piezoelectric materials is considered as an emerging technology in environmental cleanup. In this work, a... |
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| SubjectTerms | Bifunctional catalysis Bismuth oxides Chlorophenol Chromium Environmental cleanup Gold Gold modified bismuth vanadate Hexavalent chromium Hydrogen peroxide Nanoparticles New technology Oxidation Piezocatalytic effect Piezoelectricity Ultrasonic vibration Vanadates |
| Title | Efficient bifunctional piezocatalysis of Au/BiVO4 for simultaneous removal of 4-chlorophenol and Cr(VI) in water |
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