Quantifying water transport in anion exchange membrane fuel cells

Sufficient water transport through the membrane is necessary for a well-performing anion exchange membrane fuel cell (AEMFC). In this study, the water flux through a membrane electrode assembly (MEA), using a Tokuyama A201 membrane, is quantified using humidity sensors at the in- and outlet on both...

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Published inInternational journal of hydrogen energy Vol. 44; no. 10; pp. 4930 - 4939
Main Authors Eriksson, Björn, Grimler, Henrik, Carlson, Annika, Ekström, Henrik, Wreland Lindström, Rakel, Lindbergh, Göran, Lagergren, Carina
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 22.02.2019
Subjects
Anion exchange membrane fuel cell
Fuel cells
Relative humidity sensor
Water transport model
Anion exchange membrane fuel cell
Relative humidity sensor
Water transport model
Fuel cells
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Abstract Sufficient water transport through the membrane is necessary for a well-performing anion exchange membrane fuel cell (AEMFC). In this study, the water flux through a membrane electrode assembly (MEA), using a Tokuyama A201 membrane, is quantified using humidity sensors at the in- and outlet on both sides of the MEA. Experiments performed in humidified inert gas at both sides of the MEA or with liquid water at one side shows that the aggregation state of water has a large impact on the transport properties. The water fluxes are shown to be approximately three times larger for a membrane in contact with liquid water compared to vaporous. Further, the flux during fuel cell operation is investigated and shows that the transport rate of water in the membrane is affected by an applied current. The water vapor content increases on both the anode and cathode side of the AEMFC for all investigated current densities. Through modeling, an apparent water drag coefficient is determined to −0.64, indicating that the current-induced transport of water occurs in the opposite direction to the transport of hydroxide ions. These results implicate that flooding, on one or both electrodes, is a larger concern than dry-out in an AEMFC. [Display omitted] •Experimental determination of AEMFC transport coefficients in cells.•Partial pressure of water is the main driving force for diffusion.•Both anode and cathode increase in water content during operation.
AbstractList Sufficient water transport through the membrane is necessary for a well-performing anion exchange membrane fuel cell (AEMFC). In this study, the water flux through a membrane electrode assembly (MEA), using a Tokuyama A201 membrane, is quantified using humidity sensors at the in- and outlet on both sides of the MEA. Experiments performed in humidified inert gas at both sides of the MEA or with liquid water at one side shows that the aggregation state of water has a large impact on the transport properties. The water fluxes are shown to be approximately three times larger for a membrane in contact with liquid water compared to vaporous. Further, the flux during fuel cell operation is investigated and shows that the transport rate of water in the membrane is affected by an applied current. The water vapor content increases on both the anode and cathode side of the AEMFC for all investigated current densities. Through modeling, an apparent water drag coefficient is determined to −0.64, indicating that the current-induced transport of water occurs in the opposite direction to the transport of hydroxide ions. These results implicate that flooding, on one or both electrodes, is a larger concern than dry-out in an AEMFC. [Display omitted] •Experimental determination of AEMFC transport coefficients in cells.•Partial pressure of water is the main driving force for diffusion.•Both anode and cathode increase in water content during operation.
Sufficient water transport through the membrane is necessary for a well-performing anion exchange membrane fuel cell (AEMFC). In this study, the water flux through a membrane electrode assembly (MEA), using a Tokuyama A201 membrane, is quantified using humidity sensors at the in- and outlet on both sides of the MEA. Experiments performed in humidified inert gas at both sides of the MEA or with liquid water at one side shows that the aggregation state of water has a large impact on the transport properties. The water fluxes are shown to be approximately three times larger for a membrane in contact with liquid water compared to vaporous. Further, the flux during fuel cell operation is investigated and shows that the transport rate of water in the membrane is affected by an applied current. The water vapor content increases on both the anode and cathode side of the AEMFC for all investigated current densities. Through modeling, an apparent water drag coefficient is determined to −0.64, indicating that the current-induced transport of water occurs in the opposite direction to the transport of hydroxide ions. These results implicate that flooding, on one or both electrodes, is a larger concern than dry-out in an AEMFC.
Author Ekström, Henrik
Wreland Lindström, Rakel
Eriksson, Björn
Carlson, Annika
Grimler, Henrik
Lindbergh, Göran
Lagergren, Carina
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Keywords Anion exchange membrane fuel cell
Relative humidity sensor
Water transport model
Fuel cells
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Snippet Sufficient water transport through the membrane is necessary for a well-performing anion exchange membrane fuel cell (AEMFC). In this study, the water flux...
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SubjectTerms Anion exchange membrane fuel cell
Fuel cells
Relative humidity sensor
Water transport model
Title Quantifying water transport in anion exchange membrane fuel cells
URI https://dx.doi.org/10.1016/j.ijhydene.2018.12.185
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