B-doping-induced amorphization of LDH for large-current-density hydrogen evolution reaction
B-doping-induced amorphization of crystalline layered double hydroxide supported on nickel foam could activate it as an extremely efficient HER catalyst, affording large current densities of 500 and 1000 mA cm–2 at overpotentials of only 286 and 381 mV, respectively. [Display omitted] •B-doping-indu...
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| Published in | Applied catalysis. B, Environmental Vol. 261; p. 118240 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
01.02.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | B-doping-induced amorphization of crystalline layered double hydroxide supported on nickel foam could activate it as an extremely efficient HER catalyst, affording large current densities of 500 and 1000 mA cm–2 at overpotentials of only 286 and 381 mV, respectively.
[Display omitted]
•B-doping-induced amorphization of LDH was developed to activate catalytic performance.•Amorphous NiCo LDH/NF catalyst could afford large current densities at very small overpotentials.•The strategy of B-doping-induced amorphization is versatile.
Developing a platinum-free hydrogen evolution reaction (HER) electrocatalyst that can steadily drive a large current density is of great significance in a commercially electrochemical water splitting technology. Herein, we show that the B-doping-induced amorphization of crystalline layered double hydroxide (LDH) activates it as an extremely efficient HER catalyst. The amorphous B-incorporated nickel-cobalt LDH supported on the nickel foam (A-NiCo LDH/NF) can yield large current densities at small overpotentials (100 mA cm–2 at 151 mV, 500 mA cm–2 at 286 mV, and 1000 mA cm–2 at 381 mV) with high durability in alkaline medium even after 72 h, which is even better than commercial platinum. This work may provide a promising way for structure tuning of transition metal LDH to effectively boost HER efficiency towards practical water electrolysis. |
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| AbstractList | Developing a platinum-free hydrogen evolution reaction (HER) electrocatalyst that can steadily drive a large current density is of great significance in a commercially electrochemical water splitting technology. Herein, we show that the B-doping-induced amorphization of crystalline layered double hydroxide (LDH) activates it as an extremely efficient HER catalyst. The amorphous B-incorporated nickel-cobalt LDH supported on the nickel foam (A-NiCo LDH/NF) can yield large current densities at small overpotentials (100 mA cm–2 at 151 mV, 500 mA cm–2 at 286 mV, and 1000 mA cm–2 at 381 mV) with high durability in alkaline medium even after 72 h, which is even better than commercial platinum. This work may provide a promising way for structure tuning of transition metal LDH to effectively boost HER efficiency towards practical water electrolysis. B-doping-induced amorphization of crystalline layered double hydroxide supported on nickel foam could activate it as an extremely efficient HER catalyst, affording large current densities of 500 and 1000 mA cm–2 at overpotentials of only 286 and 381 mV, respectively. [Display omitted] •B-doping-induced amorphization of LDH was developed to activate catalytic performance.•Amorphous NiCo LDH/NF catalyst could afford large current densities at very small overpotentials.•The strategy of B-doping-induced amorphization is versatile. Developing a platinum-free hydrogen evolution reaction (HER) electrocatalyst that can steadily drive a large current density is of great significance in a commercially electrochemical water splitting technology. Herein, we show that the B-doping-induced amorphization of crystalline layered double hydroxide (LDH) activates it as an extremely efficient HER catalyst. The amorphous B-incorporated nickel-cobalt LDH supported on the nickel foam (A-NiCo LDH/NF) can yield large current densities at small overpotentials (100 mA cm–2 at 151 mV, 500 mA cm–2 at 286 mV, and 1000 mA cm–2 at 381 mV) with high durability in alkaline medium even after 72 h, which is even better than commercial platinum. This work may provide a promising way for structure tuning of transition metal LDH to effectively boost HER efficiency towards practical water electrolysis. |
| ArticleNumber | 118240 |
| Author | Chen, Ziliang Guo, Peifang Fei, Ben Yang, Hongyuan Wu, Renbing |
| Author_xml | – sequence: 1 givenname: Hongyuan surname: Yang fullname: Yang, Hongyuan – sequence: 2 givenname: Ziliang orcidid: 0000-0001-5307-7309 surname: Chen fullname: Chen, Ziliang – sequence: 3 givenname: Peifang surname: Guo fullname: Guo, Peifang – sequence: 4 givenname: Ben surname: Fei fullname: Fei, Ben – sequence: 5 givenname: Renbing surname: Wu fullname: Wu, Renbing email: rbwu@fudan.edu.cn |
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| PublicationTitle | Applied catalysis. B, Environmental |
| PublicationYear | 2020 |
| Publisher | Elsevier B.V Elsevier BV |
| Publisher_xml | – name: Elsevier B.V – name: Elsevier BV |
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| Snippet | B-doping-induced amorphization of crystalline layered double hydroxide supported on nickel foam could activate it as an extremely efficient HER catalyst,... Developing a platinum-free hydrogen evolution reaction (HER) electrocatalyst that can steadily drive a large current density is of great significance in a... |
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| SubjectTerms | Amorphization Amorphization of crystalline LDH B-doping Catalysts Cobalt Current density Doping Electrochemistry Electrolysis HER catalyst Hydrogen evolution reactions Hydroxides Large current density Metal foams Nickel Platinum Transition metals Water splitting |
| Title | B-doping-induced amorphization of LDH for large-current-density hydrogen evolution reaction |
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