Mesoscopic study of cylindrical phases of poly(styrene)-poly(isoprene) copolymer: Order–order phase transitions by temperature control

Phase transitions of cylindrical structures of poly(styrene)–poly(isoprene) copolymer (PS–PI) toward spherical and gyroid structures were explored using DPD simulations and a coarse-grained model. Cylindrical phases were first obtained within a composition interval (“predominance region”) 0.2<fPS...

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Published in	Polymer (Guilford) Vol. 50; no. 19; pp. 4596 - 4601
Main Authors	Rodríguez-Hidalgo, María-del-Rosario, Soto-Figueroa, César, Martínez-Magadán, José-Manuel, Luís-Vicente
Format	Journal Article
Language	English
Published	Kidlington Elsevier Ltd 10.09.2009 Elsevier
Subjects	Applied sciences Block polymers Cylindrical structures Exact sciences and technology Order–order phase transitions Organic polymers Physicochemistry of polymers Properties and characterization Structure, morphology and analysis Cylindrical structures Block polymers Order–order phase transitions Computer simulation Isoprene copolymer Diblock copolymer Temperature effect Theoretical study Composition effect Order-order phase transitions Phase transitions Styrene copolymer
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Abstract	Phase transitions of cylindrical structures of poly(styrene)–poly(isoprene) copolymer (PS–PI) toward spherical and gyroid structures were explored using DPD simulations and a coarse-grained model. Cylindrical phases were first obtained within a composition interval (“predominance region”) 0.2<fPS<0.26 (volume fraction of poly(styrene)). The predominance region of cylindrical structures was then subject to thermal heating cycles. The thermodynamic instabilities of cylindrical microdomains induce anisotropic composition fluctuations and phase transitions. A transition from the cylindrical phase at low composition limit to a spherical arrangement was observed during the thermal heating process. The cylindrical phase at the intermediate and high composition limit within the predominance region exhibits a transition towards a gyroid arrangement. The phase transition control during thermal heating on the cylindrical phases was governed by small variations in composition. The results are consistent with experimental studies. [Display omitted]
AbstractList	Phase transitions of cylindrical structures of poly(styrene)–poly(isoprene) copolymer (PS–PI) toward spherical and gyroid structures were explored using DPD simulations and a coarse-grained model. Cylindrical phases were first obtained within a composition interval (“predominance region”) 0.2<fPS<0.26 (volume fraction of poly(styrene)). The predominance region of cylindrical structures was then subject to thermal heating cycles. The thermodynamic instabilities of cylindrical microdomains induce anisotropic composition fluctuations and phase transitions. A transition from the cylindrical phase at low composition limit to a spherical arrangement was observed during the thermal heating process. The cylindrical phase at the intermediate and high composition limit within the predominance region exhibits a transition towards a gyroid arrangement. The phase transition control during thermal heating on the cylindrical phases was governed by small variations in composition. The results are consistent with experimental studies. [Display omitted] Phase transitions of cylindrical structures of poly(styrene)-poly(isoprene) copolymer (PS-PI) toward spherical and gyroid structures were explored using DPD simulations and a coarse-grained model. Cylindrical phases were first obtained within a composition interval (''predominance region'') 0.2 < f(P(S < 0.26 (volume fraction of poly(styrene)). The predominance region of cylindrical structures was then subject to thermal heating cycles. The thermodynamic instabilities of cylindrical microdomains induce anisotropic composition fluctuations and phase transitions. A transition from the cylindrical phase at low composition limit to a spherical arrangement was observed during the thermal heating process. The cylindrical phase at the intermediate and high composition limit within the predominance region exhibits a transition towards a gyroid arrangement. The phase transition control during thermal heating on the cylindrical phases was governed by small variations in composition. The results are consistent with experimental studies.
Author	Rodríguez-Hidalgo, María-del-Rosario Luís-Vicente Soto-Figueroa, César Martínez-Magadán, José-Manuel
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Snippet	Phase transitions of cylindrical structures of poly(styrene)–poly(isoprene) copolymer (PS–PI) toward spherical and gyroid structures were explored using DPD... Phase transitions of cylindrical structures of poly(styrene)-poly(isoprene) copolymer (PS-PI) toward spherical and gyroid structures were explored using DPD...
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SubjectTerms	Applied sciences Block polymers Cylindrical structures Exact sciences and technology Order–order phase transitions Organic polymers Physicochemistry of polymers Properties and characterization Structure, morphology and analysis
Title	Mesoscopic study of cylindrical phases of poly(styrene)-poly(isoprene) copolymer: Order–order phase transitions by temperature control
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