Directional properties of polar paramagnetic molecules subject to congruent electric, magnetic and optical fields

We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarizable) molecule offer possibilities to both amplify and control the directionality of the ensuing molecular states that surpass those available in double-field combination...

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Published inNew journal of physics Vol. 17; no. 4; pp. 45017 - 45042
Main Authors Sharma, Ketan, Friedrich, Bretislav
Format Journal Article
LanguageEnglish
Published Bristol IOP Publishing 24.04.2015
Subjects
Account reviews
alignment and orientation
combined fields
Coupling (molecular)
Crystals
Electric fields
induced-dipole interaction
Magnetic properties
nonresonant laser field
Physics
polarizability
Stark effect
Zeeman effect
Online AccessGet full text
ISSN1367-2630
1367-2630
DOI10.1088/1367-2630/17/4/045017

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Abstract We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarizable) molecule offer possibilities to both amplify and control the directionality of the ensuing molecular states that surpass those available in double-field combinations or in single fields alone. At the core of these triple-field effects is the lifting of the degeneracy of the projection quantum number M by the magnetic field superimposed on the optical field and a subsequent coupling of the members of the 'doubled' (for states with ) tunneling doublets due to the optical field by even a weak electrostatic field.
AbstractList We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarizable) molecule offer possibilities to both amplify and control the directionality of the ensuing molecular states that surpass those available in double-field combinations or in single fields alone. At the core of these triple-field effects is the lifting of the degeneracy of the projection quantum number M by the magnetic field superimposed on the optical field and a subsequent coupling of the members of the ‘doubled’ (for states with $M\ne 0$ ) tunneling doublets due to the optical field by even a weak electrostatic field.
We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarizable) molecule offer possibilities to both amplify and control the directionality of the ensuing molecular states that surpass those available in double-field combinations or in single fields alone. At the core of these triple-field effects is the lifting of the degeneracy of the projection quantum number M by the magnetic field superimposed on the optical field and a subsequent coupling of the members of the 'doubled' (for states with ) tunneling doublets due to the optical field by even a weak electrostatic field.
Author Sharma, Ketan
Friedrich, Bretislav
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  surname: Sharma
  fullname: Sharma, Ketan
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  givenname: Bretislav
  surname: Friedrich
  fullname: Friedrich, Bretislav
  email: bretislav.friedrich@fhi-berlin.mpg.de
  organization: Fritz-Haber-Institut der Max-Planck-Gesellschaft Faradayweg 4-6, D-14195 Berlin, Germany
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Snippet We show that congruent electric, magnetic and non-resonant optical fields acting concurrently on a polar paramagnetic (and polarizable) molecule offer...
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SubjectTerms Account reviews
alignment and orientation
combined fields
Coupling (molecular)
Crystals
Electric fields
induced-dipole interaction
Magnetic properties
nonresonant laser field
Physics
polarizability
Stark effect
Zeeman effect
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Title Directional properties of polar paramagnetic molecules subject to congruent electric, magnetic and optical fields
URI https://iopscience.iop.org/article/10.1088/1367-2630/17/4/045017
https://www.proquest.com/docview/2312940206
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Volume 17
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