Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension
Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating particles (INPs) increasing rapidly with decreasing temperature. Here, molecular-dynamics simulations of heterogeneous ice nucleation demonstrate...
Saved in:
Published in | Atmospheric chemistry and physics Vol. 23; no. 18; pp. 10625 - 10642 |
---|---|
Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Katlenburg-Lindau
Copernicus GmbH
26.09.2023
Copernicus Publications |
Subjects | |
Online Access | Get full text |
Cover
Loading…
Abstract | Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating particles (INPs) increasing rapidly with decreasing temperature. Here, molecular-dynamics simulations of heterogeneous ice nucleation demonstrate that the ice nucleation rate is also sensitive to pressure and that negative pressure within supercooled water shifts freezing temperatures to higher temperatures. Negative pressure, or tension, occurs naturally in water capillary bridges and pores and can also result from water agitation. Capillary bridge simulations presented in this study confirm that negative Laplace pressure within the water increases heterogeneous-freezing temperatures. The increase in freezing temperatures with negative pressure is approximately linear within the atmospherically relevant range of 1 to -1000 atm. An equation describing the slope depends on the latent heat of freezing and the molar volume difference between liquid water and ice. Results indicate that negative pressures of -500 atm, which correspond to nanometer-scale water surface curvatures, lead to a roughly 4 K increase in heterogeneous-freezing temperatures. In mixed-phase clouds, this would result in an increase of approximately 1 order of magnitude in active INP concentrations. The findings presented here indicate that any process leading to negative pressure in supercooled water may play a role in ice formation, consistent with experimental evidence of enhanced ice nucleation due to surface geometry or mechanical agitation of water droplets. This points towards the potential for dynamic processes such as contact nucleation and droplet collision or breakup to increase ice nucleation rates through pressure perturbations. |
---|---|
AbstractList | Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating particles (INPs) increasing rapidly with decreasing temperature. Here, molecular-dynamics simulations of heterogeneous ice nucleation demonstrate that the ice nucleation rate is also sensitive to pressure and that negative pressure within supercooled water shifts freezing temperatures to higher temperatures. Negative pressure, or tension, occurs naturally in water capillary bridges and pores and can also result from water agitation. Capillary bridge simulations presented in this study confirm that negative Laplace pressure within the water increases heterogeneous-freezing temperatures. The increase in freezing temperatures with negative pressure is approximately linear within the atmospherically relevant range of 1 to -1000 atm. An equation describing the slope depends on the latent heat of freezing and the molar volume difference between liquid water and ice. Results indicate that negative pressures of -500 atm, which correspond to nanometer-scale water surface curvatures, lead to a roughly 4 K increase in heterogeneous-freezing temperatures. In mixed-phase clouds, this would result in an increase of approximately 1 order of magnitude in active INP concentrations. The findings presented here indicate that any process leading to negative pressure in supercooled water may play a role in ice formation, consistent with experimental evidence of enhanced ice nucleation due to surface geometry or mechanical agitation of water droplets. This points towards the potential for dynamic processes such as contact nucleation and droplet collision or breakup to increase ice nucleation rates through pressure perturbations. Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating particles (INPs) increasing rapidly with decreasing temperature. Here, molecular-dynamics simulations of heterogeneous ice nucleation demonstrate that the ice nucleation rate is also sensitive to pressure and that negative pressure within supercooled water shifts freezing temperatures to higher temperatures. Negative pressure, or tension, occurs naturally in water capillary bridges and pores and can also result from water agitation. Capillary bridge simulations presented in this study confirm that negative Laplace pressure within the water increases heterogeneous-freezing temperatures. The increase in freezing temperatures with negative pressure is approximately linear within the atmospherically relevant range of 1 to −1000 atm. An equation describing the slope depends on the latent heat of freezing and the molar volume difference between liquid water and ice. Results indicate that negative pressures of −500 atm, which correspond to nanometer-scale water surface curvatures, lead to a roughly 4 K increase in heterogeneous-freezing temperatures. In mixed-phase clouds, this would result in an increase of approximately 1 order of magnitude in active INP concentrations. The findings presented here indicate that any process leading to negative pressure in supercooled water may play a role in ice formation, consistent with experimental evidence of enhanced ice nucleation due to surface geometry or mechanical agitation of water droplets. This points towards the potential for dynamic processes such as contact nucleation and droplet collision or breakup to increase ice nucleation rates through pressure perturbations. Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating particles (INPs) increasing rapidly with decreasing temperature. Here, molecular-dynamics simulations of heterogeneous ice nucleation demonstrate that the ice nucleation rate is also sensitive to pressure and that negative pressure within supercooled water shifts freezing temperatures to higher temperatures. Negative pressure, or tension, occurs naturally in water capillary bridges and pores and can also result from water agitation. Capillary bridge simulations presented in this study confirm that negative Laplace pressure within the water increases heterogeneous-freezing temperatures. The increase in freezing temperatures with negative pressure is approximately linear within the atmospherically relevant range of 1 to − 1000 atm. An equation describing the slope depends on the latent heat of freezing and the molar volume difference between liquid water and ice. Results indicate that negative pressures of − 500 atm, which correspond to nanometer-scale water surface curvatures, lead to a roughly 4 K increase in heterogeneous-freezing temperatures. In mixed-phase clouds, this would result in an increase of approximately 1 order of magnitude in active INP concentrations. The findings presented here indicate that any process leading to negative pressure in supercooled water may play a role in ice formation, consistent with experimental evidence of enhanced ice nucleation due to surface geometry or mechanical agitation of water droplets. This points towards the potential for dynamic processes such as contact nucleation and droplet collision or breakup to increase ice nucleation rates through pressure perturbations. |
Audience | Academic |
Author | Cantrell, Will Nakamura, Issei Li, Tianshu Shaw, Raymond A Rosky, Elise |
Author_xml | – sequence: 1 fullname: Rosky, Elise – sequence: 2 fullname: Cantrell, Will – sequence: 3 fullname: Li, Tianshu – sequence: 4 fullname: Nakamura, Issei – sequence: 5 fullname: Shaw, Raymond A |
BookMark | eNptkl2L1DAUhous4O7qD_Au4JUXXZPTJmkvl8WPgRXBj-uQJqedDG0yJqmrF_53MzOiDkggCYfnfXMOea-qCx88VtVzRm8469tX2uxraGpGBfAaKDSPqksmOlrLBtqLf-5PqquUdpQCp6y9rH6-DzOaddaRJLeUM7vgE4n4DfVM8lZnssWMMUzoMayJOIPEr2bGI0mCMWtM5IC5aYuRZFz2GHVeIxbYkwdd1GT1tuxG791cnvpRKJ-K_Gn1eNRzwme_z-vqy5vXn-_e1fcf3m7ubu9r0zY81z1yAN7jYIdRCotA20ZC343WIu2EsF0_ik4bgKalgo7amJHLIkEYRCtkc11tTr426J3aR7eUJlTQTh0LIU5Kx-zKVErzjlurrRw60zJmh6FlQgAwMJoywYrXi5PXPoavK6asdmGNvrSvoBMdByFp_5eadDF1fgw5arO4ZNStFEJIzuSBuvkPVZbFxZnyw6Mr9TPByzNBYTJ-z5NeU1KbTx_PWXZiTQwpRRz_DM6oOoRGldAoaNQxNOoQmuYXZG63Fw |
Cites_doi | 10.1021/jp805227c 10.1038/213384a0 10.1175/BAMS-86-6-795 10.1038/ncomms2918 10.1890/05-1879 10.1175/1520-0450(1983)022<1964:CVIFOF>2.0.CO;2 10.1063/1.4919714 10.1175/1520-0450(1969)008<0994:FOSWDD>2.0.CO;2 10.1073/pnas.1913855117 10.1021/acs.jpclett.5b01531 10.1063/1.4938749 10.1021/acs.jpcc.5b09740 10.5194/acp-20-9419-2020 10.1002/qj.49711749710 10.1175/JAS-D-17-0112.1 10.1002/grl.50700 10.5194/acp-20-3209-2020 10.1038/nature07226 10.1038/nmat2508 10.1016/j.cplett.2021.139289 10.1021/acsnano.9b01014 10.1016/j.cplett.2013.07.085 10.1038/s41598-017-16787-3 10.1017/CBO9780511976377 10.1016/j.est.2022.104755 10.5194/acp-11-8767-2011 10.1021/jp071957s 10.1016/S0169-8095(01)00132-6 10.1103/PhysRevLett.117.135702 10.5194/acp-21-18519-2021 10.1002/qj.49709942111 10.1088/0965-0393/18/1/015012 10.1039/C4CP03948C 10.1073/pnas.0910818107 10.1063/5.0049031 10.1039/c1cp22167a 10.1126/science.155.3768.1413 10.1063/5.0140814 10.5194/acp-23-1579-2023 10.1103/PhysRevB.31.5262 10.1021/acs.jpclett.8b02244 10.5194/acp-14-2071-2014 10.1103/PhysRevE.97.023103 10.1063/1.4953854 10.1038/srep02031 10.1021/jacs.5b08748 10.1021/jp4118375 10.1146/annurev-fluid-030321-103941 10.5194/acp-2022-696 10.1103/PhysRevLett.126.015704 10.1063/1.5145334 10.1126/science.189.4206.880 10.5194/acp-11-8003-2011 10.1021/acs.jpcb.2c06246 10.1103/PhysRevB.28.784 10.1073/pnas.1620999114 10.1021/acs.jpcb.7b11476 10.1021/jp0506336 10.37099/mtu.dc.all-datasets/41 10.1103/PhysRevLett.113.235701 10.1006/jcph.1995.1039 10.5194/acp-22-10099-2022 10.1021/jp9626531 10.1039/c3fd00035d 10.1021/ja411507a 10.3390/atmos11010001 10.1021/jp066080w 10.1029/2004GL020483 10.1021/jacs.0c10663 10.1038/s41467-018-08222-6 10.5194/acp-12-9817-2012 10.1029/2021GL097373 10.1038/35020537 |
ContentType | Journal Article |
Copyright | COPYRIGHT 2023 Copernicus GmbH 2023. This work is published under https://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
Copyright_xml | – notice: COPYRIGHT 2023 Copernicus GmbH – notice: 2023. This work is published under https://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
DBID | AAYXX CITATION ISR 7QH 7TG 7TN 7UA 8FD 8FE 8FG ABUWG AFKRA ARAPS ATCPS AZQEC BENPR BFMQW BGLVJ BHPHI BKSAR C1K CCPQU DWQXO F1W GNUQQ H8D H96 HCIFZ KL. L.G L7M P5Z P62 PATMY PCBAR PIMPY PQEST PQQKQ PQUKI PRINS PYCSY DOA |
DOI | 10.5194/acp-23-10625-2023 |
DatabaseName | CrossRef Gale In Context: Science Aqualine Meteorological & Geoastrophysical Abstracts Oceanic Abstracts Water Resources Abstracts Technology Research Database ProQuest SciTech Collection ProQuest Technology Collection ProQuest Central (Alumni) ProQuest Central Advanced Technologies & Aerospace Database (1962 - current) ProQuest Agricultural & Environmental Science ProQuest Central Essentials AUTh Library subscriptions: ProQuest Central ProQuest Continental Europe Database Technology Collection ProQuest Natural Science Collection ProQuest Earth, Atmospheric & Aquatic Science Environmental Sciences and Pollution Management ProQuest One Community College ProQuest Central ASFA: Aquatic Sciences and Fisheries Abstracts ProQuest Central Student Aerospace Database Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources SciTech Premium Collection (Proquest) (PQ_SDU_P3) Meteorological & Geoastrophysical Abstracts - Academic Aquatic Science & Fisheries Abstracts (ASFA) Professional Advanced Technologies Database with Aerospace ProQuest Advanced Technologies & Aerospace Database ProQuest Advanced Technologies & Aerospace Collection Environmental Science Database ProQuest Earth, Atmospheric & Aquatic Science Database Publicly Available Content Database ProQuest One Academic Eastern Edition (DO NOT USE) ProQuest One Academic ProQuest One Academic UKI Edition ProQuest Central China Environmental Science Collection DOAJ Directory of Open Access Journals |
DatabaseTitle | CrossRef Publicly Available Content Database Aquatic Science & Fisheries Abstracts (ASFA) Professional ProQuest Central Student Technology Collection Technology Research Database ProQuest Advanced Technologies & Aerospace Collection ProQuest Central Essentials ProQuest Central (Alumni Edition) SciTech Premium Collection ProQuest One Community College ProQuest Central China Water Resources Abstracts Environmental Sciences and Pollution Management Earth, Atmospheric & Aquatic Science Collection ProQuest Central Aerospace Database Meteorological & Geoastrophysical Abstracts Oceanic Abstracts Natural Science Collection ProQuest Central Korea Agricultural & Environmental Science Collection Advanced Technologies Database with Aerospace Advanced Technologies & Aerospace Collection ProQuest One Academic Eastern Edition Earth, Atmospheric & Aquatic Science Database ProQuest Technology Collection Continental Europe Database ProQuest SciTech Collection Aqualine Environmental Science Collection Advanced Technologies & Aerospace Database Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources ProQuest One Academic UKI Edition ASFA: Aquatic Sciences and Fisheries Abstracts Environmental Science Database ProQuest One Academic Meteorological & Geoastrophysical Abstracts - Academic |
DatabaseTitleList | CrossRef Publicly Available Content Database |
Database_xml | – sequence: 1 dbid: DOA name: Directory of Open Access Journals url: https://www.doaj.org/ sourceTypes: Open Website – sequence: 2 dbid: 8FG name: ProQuest Technology Collection url: https://search.proquest.com/technologycollection1 sourceTypes: Aggregation Database |
DeliveryMethod | fulltext_linktorsrc |
Discipline | Meteorology & Climatology |
EISSN | 1680-7324 |
EndPage | 10642 |
ExternalDocumentID | oai_doaj_org_article_a585ddad7b8c411dbb41662212ca0161 A766675179 10_5194_acp_23_10625_2023 |
GroupedDBID | 23N 2WC 3V. 4P2 5GY 5VS 6J9 7XC 8FE 8FG 8FH 8R4 8R5 AAFWJ AAYXX ABUWG ACGFO ADBBV AENEX AFKRA AFPKN AFRAH AHGZY AIAGR ALMA_UNASSIGNED_HOLDINGS ARAPS ATCPS BBORY BCNDV BENPR BFMQW BGLVJ BHPHI BKSAR BPHCQ CCPQU CITATION D1K E3Z EBS EDH EJD FD6 GROUPED_DOAJ GX1 H13 HCIFZ HH5 IAO IEA ISR ITC K6- KQ8 M~E OK1 P2P P62 PATMY PCBAR PIMPY PQQKQ PROAC PYCSY Q2X RIG RKB RNS TR2 XSB ~02 7QH 7TG 7TN 7UA 8FD AZQEC C1K DWQXO F1W GNUQQ H8D H96 KL. L.G L7M PQEST PQUKI PRINS |
ID | FETCH-LOGICAL-c435t-9e52259ebdbf76de20437298fdde0866d89f68ac2234060faccf57225e2b64673 |
IEDL.DBID | 8FG |
ISSN | 1680-7324 1680-7316 |
IngestDate | Thu Sep 05 15:40:46 EDT 2024 Fri Sep 13 03:37:06 EDT 2024 Thu Feb 22 23:27:05 EST 2024 Thu Nov 09 12:32:16 EST 2023 Sat Sep 28 20:58:03 EDT 2024 Fri Aug 23 01:21:45 EDT 2024 |
IsDoiOpenAccess | true |
IsOpenAccess | true |
IsPeerReviewed | true |
IsScholarly | true |
Issue | 18 |
Language | English |
LinkModel | DirectLink |
MergedId | FETCHMERGED-LOGICAL-c435t-9e52259ebdbf76de20437298fdde0866d89f68ac2234060faccf57225e2b64673 |
ORCID | 0000-0002-3477-4456 0000-0003-0390-2424 |
OpenAccessLink | https://www.proquest.com/docview/2868526709/abstract/?pq-origsite=%requestingapplication% |
PQID | 2868526709 |
PQPubID | 105744 |
PageCount | 18 |
ParticipantIDs | doaj_primary_oai_doaj_org_article_a585ddad7b8c411dbb41662212ca0161 proquest_journals_2868526709 gale_infotracmisc_A766675179 gale_infotracacademiconefile_A766675179 gale_incontextgauss_ISR_A766675179 crossref_primary_10_5194_acp_23_10625_2023 |
PublicationCentury | 2000 |
PublicationDate | 2023-09-26 |
PublicationDateYYYYMMDD | 2023-09-26 |
PublicationDate_xml | – month: 09 year: 2023 text: 2023-09-26 day: 26 |
PublicationDecade | 2020 |
PublicationPlace | Katlenburg-Lindau |
PublicationPlace_xml | – name: Katlenburg-Lindau |
PublicationTitle | Atmospheric chemistry and physics |
PublicationYear | 2023 |
Publisher | Copernicus GmbH Copernicus Publications |
Publisher_xml | – name: Copernicus GmbH – name: Copernicus Publications |
References | ref13 ref57 ref12 ref56 ref15 ref59 ref14 ref58 ref53 ref52 ref11 ref55 ref10 ref54 ref17 ref16 ref19 ref18 ref51 ref50 ref46 ref45 ref48 ref47 ref42 ref41 ref44 ref43 ref49 ref8 ref7 ref9 ref4 ref3 ref6 ref5 ref40 ref35 ref34 ref37 ref36 ref31 ref75 ref30 ref74 ref33 ref32 ref2 ref1 ref39 ref38 ref71 ref70 ref73 ref72 ref24 ref68 ref23 ref67 ref26 ref25 ref69 ref20 ref64 ref63 ref22 ref66 ref21 ref65 ref28 ref27 ref29 ref60 ref62 ref61 |
References_xml | – ident: ref48 doi: 10.1021/jp805227c – ident: ref18 doi: 10.1038/213384a0 – ident: ref6 doi: 10.1175/BAMS-86-6-795 – ident: ref40 doi: 10.1038/ncomms2918 – ident: ref28 doi: 10.1890/05-1879 – ident: ref37 doi: 10.1175/1520-0450(1983)022<1964:CVIFOF>2.0.CO;2 – ident: ref11 doi: 10.1063/1.4919714 – ident: ref1 doi: 10.1175/1520-0450(1969)008<0994:FOSWDD>2.0.CO;2 – ident: ref63 doi: 10.1073/pnas.1913855117 – ident: ref52 doi: 10.1021/acs.jpclett.5b01531 – ident: ref72 doi: 10.1063/1.4938749 – ident: ref4 doi: 10.1021/acs.jpcc.5b09740 – ident: ref12 doi: 10.5194/acp-20-9419-2020 – ident: ref59 doi: 10.1002/qj.49711749710 – ident: ref21 doi: 10.1175/JAS-D-17-0112.1 – ident: ref71 doi: 10.1002/grl.50700 – ident: ref2 – ident: ref47 doi: 10.5194/acp-20-3209-2020 – ident: ref70 doi: 10.1038/nature07226 – ident: ref38 doi: 10.1038/nmat2508 – ident: ref61 doi: 10.1016/j.cplett.2021.139289 – ident: ref8 doi: 10.1021/acsnano.9b01014 – ident: ref50 doi: 10.1016/j.cplett.2013.07.085 – ident: ref46 doi: 10.1038/s41598-017-16787-3 – ident: ref35 doi: 10.1017/CBO9780511976377 – ident: ref69 doi: 10.1016/j.est.2022.104755 – ident: ref51 doi: 10.5194/acp-11-8767-2011 – ident: ref22 doi: 10.1021/jp071957s – ident: ref15 doi: 10.1016/S0169-8095(01)00132-6 – ident: ref17 doi: 10.1103/PhysRevLett.117.135702 – ident: ref29 doi: 10.5194/acp-21-18519-2021 – ident: ref53 doi: 10.1002/qj.49709942111 – ident: ref67 doi: 10.1088/0965-0393/18/1/015012 – ident: ref25 doi: 10.1039/C4CP03948C – ident: ref13 doi: 10.1073/pnas.0910818107 – ident: ref16 doi: 10.1063/5.0049031 – ident: ref39 doi: 10.1039/c1cp22167a – ident: ref60 doi: 10.1126/science.155.3768.1413 – ident: ref49 doi: 10.1063/5.0140814 – ident: ref31 doi: 10.5194/acp-23-1579-2023 – ident: ref66 doi: 10.1103/PhysRevB.31.5262 – ident: ref57 doi: 10.1021/acs.jpclett.8b02244 – ident: ref45 doi: 10.5194/acp-14-2071-2014 – ident: ref73 doi: 10.1103/PhysRevE.97.023103 – ident: ref42 doi: 10.1063/1.4953854 – ident: ref41 doi: 10.1038/srep02031 – ident: ref19 doi: 10.1021/jacs.5b08748 – ident: ref43 doi: 10.1021/jp4118375 – ident: ref10 doi: 10.1146/annurev-fluid-030321-103941 – ident: ref20 doi: 10.5194/acp-2022-696 – ident: ref5 doi: 10.1103/PhysRevLett.126.015704 – ident: ref55 doi: 10.1063/1.5145334 – ident: ref30 doi: 10.1126/science.189.4206.880 – ident: ref36 doi: 10.5194/acp-11-8003-2011 – ident: ref14 doi: 10.1021/acs.jpcb.2c06246 – ident: ref65 doi: 10.1103/PhysRevB.28.784 – ident: ref24 doi: 10.1073/pnas.1620999114 – ident: ref58 doi: 10.1021/acs.jpcb.7b11476 – ident: ref64 doi: 10.1021/jp0506336 – ident: ref7 doi: 10.37099/mtu.dc.all-datasets/41 – ident: ref23 doi: 10.1103/PhysRevLett.113.235701 – ident: ref54 doi: 10.1006/jcph.1995.1039 – ident: ref62 doi: 10.5194/acp-22-10099-2022 – ident: ref33 doi: 10.1021/jp9626531 – ident: ref32 doi: 10.1039/c3fd00035d – ident: ref44 doi: 10.1021/ja411507a – ident: ref56 – ident: ref74 doi: 10.3390/atmos11010001 – ident: ref75 doi: 10.1021/jp066080w – ident: ref3 doi: 10.1029/2004GL020483 – ident: ref27 doi: 10.1021/jacs.0c10663 – ident: ref9 doi: 10.1038/s41467-018-08222-6 – ident: ref26 doi: 10.5194/acp-12-9817-2012 – ident: ref68 doi: 10.1029/2021GL097373 – ident: ref34 doi: 10.1038/35020537 |
SSID | ssj0025014 |
Score | 2.4567206 |
Snippet | Heterogeneous ice nucleation is thought to be the primary pathway for the formation of ice in mixed-phase clouds, with the number of active ice-nucleating... |
SourceID | doaj proquest gale crossref |
SourceType | Open Website Aggregation Database |
StartPage | 10625 |
SubjectTerms | Agitation Agreements Analysis Approximation Bridges Capillary pressure Cloud formation Droplets Freezing Freezing temperatures Hypotheses Ice formation Ice nucleation Latent heat Molar volume Molecular dynamics Nucleation Perturbation Pressure Simulation Simulation methods Supercooled water Surface geometry Temperature Tension Water Water droplets Water drops |
SummonAdditionalLinks | – databaseName: DOAJ Directory of Open Access Journals dbid: DOA link: http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwrV3Pa9VAEF5KT16KVovRVhYRC8LS9zbJJu9Yi6UKz4Ntobdlf9qCJo8kj-Kh_3u_2eSJ7yBePCaZ_Nidyew3ycw3jL1zceaDclLIYK0oKL-xxsInCuXyMs59CAUVOC-_qovr4stNefNHqy_KCRvpgceJOzHAs94bX9naFfO5txYQQkl4XGcIriTvOy83wdQUatHfMgq1VD0T1Jtp_J8JtFKcGLcSkvKxgPwFNQ_fWpEScf_f3HNac86fsr0JLPLT8SGfsZ3Q7LNsCZzbdulzOH_Pz37cAXSmrefsYbnpdsv7u59TZ66eE00TrjPcmoHfUv5LC7MJiPk53ARviNI4SfLWuXXXcxJL-R-cmKsm2mUIN_we0LTjVHjWcWdW1LKo-8VTFnzbvGDX55-uzi7E1GBBOKCkQSwC0Fe5CNbbWCkfqE4WYLuO8HkIdZSvF1HVxgFCYN2fReNcLCucEqRV8LD5Adtt2ia8ZLily2cO2CMsCIFFW5amyKOX3kcLiJWxD5tJ1quRR0Mj_iCNaGhEy1wnjWjSSMY-khp-CxIFdtoBw9CTYeh_GUbG3pISNZFcNJRF892s-15_vvymTysEbRWRk2XseBKK7dAZjGIsSsCgiBdrS_JwSxJvods-vLEVPXmBXsta1aUkhrxX_2NEr9kTmh3KVpHqkO0O3TocARIN9k2y_kdyCAlk priority: 102 providerName: Directory of Open Access Journals |
Title | Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension |
URI | https://www.proquest.com/docview/2868526709/abstract/ https://doaj.org/article/a585ddad7b8c411dbb41662212ca0161 |
Volume | 23 |
hasFullText | 1 |
inHoldings | 1 |
isFullTextHit | |
isPrint | |
link | http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwfV3da9RAEF9q--KL-Imp9VhEFITl7jbJJvckbel5Cle0Wuzbsp9tQbPXJEfxwf_dmb1N5R70KSSZJCQzmf3N7sxvCHlt_MQ6YTjjTmtWYH5jDQMfK4TJSz-1zhVY4Lw8FYvz4tNFebFDFkMtDKZVDj4xOmobDM6Rj3kt6pIj29hYaZwFMP34_eqGYf8oXGdNzTTukb0pcuJhzfj8w13ohatnGHqJesKwV9NmfRPQSzFWZsU45mdBJMCwmfjWCBWJ_P_lruMYNH9IHiTwSA832n5EdlzzmGRLwL2hjdPj9A09_nENIDTuPSG_l0P3W9pd_0ydujqKtE1wn_5K9fQK82ECmJEL646C26ANUhxHSRqMWbcdRbGYD0KRySrRMINwQ28BqrYUC9FaatQKWxi1v2jMig_NU3I-P_l2vGCp4QIzgJp6NnOAxsqZ01b7SliHdbMAvmsPPhBCH2HrmRe1MgApAAdMvDLGlxVc4rgW4HHzZ2S3CY17TuCRJp8YwCJuhojM67JURe4tt9ZrgFwZeTd8ZLna8GpIiEdQIxI0Inkuo0YkaiQjR6iGO0GkxI4HQnsp0x8mFQQ-1ipb6doU06nVGrCm4DA0G4W4NiOvUIkSSS8azKq5VOuukx-_nsnDCoK4CsnKMvI2CfmANqZSkQK8FPJkbUkebEnCX2m2Tw-2IpNX6ORfG97__-kX5D6-N-alcHFAdvt27V4C-On1KNr1iOwdnZx-PsPtfPnl-yhOJfwBa3MJBg |
link.rule.ids | 315,786,790,870,2115,12792,21416,27957,27958,33408,33779,43635,43840,74392,74659 |
linkProvider | ProQuest |
linkToHtml | http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwfV1Nb9QwELWgHOCC-BSB0loIgYRkdddJnOwJtRXLFro9QCv1Ztlju61UkiXJCnHof2fG6y3aAxyTTBI548y8sWfeMPYWwsh5BVJIb60oKL-xRscnCgV5GcbO-4IKnOcnanZWfDkvz9OCW5_SKtc2MRpq1wKtke_JWtWlJLaxj4ufgrpG0e5qaqFxl90rcnSdVCk-_XwbcNGeGQVcqh4J6tC02tVEzFLsGVgISVlZiP8FtRDf8EuRvv9fRjp6nukj9jBBRr6_0vFjdsc3T1g2R7TbdnFRnL_jh9dXCD3j0VN2M1_3vOX91Y_Un6vnRNaEzxkuzcAvKQumxcnjMfLnaCx4Q8TGUZK3AMuu5yQWs0A48Vcl8mUUbvgvBKgdp_KzjoNZUOOi7jePufBt84ydTT-dHs5EarMgALHSICYeMVg58dbZUCnnqVoWIXcd0PJhwKNcPQmqNoBAAr3_KBiAUFZ4i5dWoZ3Nn7Otpm38C4avhHwEiED8hHBYsGVpijw46VywCLQy9mH9kfVixaahMQohjWjUiJa5jhrRpJGMHZAabgWJCDueaLsLnf4rbTDccc64ytZQjMfOWkSYSqJDBkNoNmNvSImaqC4ayqW5MMu-10ffv-n9CkO3iijKMvY-CYV26AyOYlWagIMidqwNye0NSfwXYfPyeq7oZAt6_Xfmvvz_5V12f3Y6P9bHRydfX7EH9A0oM0WqbbY1dEv_GuHPYHfiHP8Du5YEBQ |
linkToPdf | http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwfV3da9RAEF-0BfFFrB8YW9tFREFY7m6TbHJP0q-jVe8o1ULflv1sC232THKID_7vzuztVe5BH5NMEpKZzP4m-9vfEPLO-KF1wnDGndasQH5jDQMfK4TJSz-yzhW4wHk6EycXxefL8jLxn7pEq1zlxJiobTD4j3zAa1GXHNXGBj7RIs6OJp_mPxh2kMKZ1tRO4yHZrApRQoRvHhzPzs7vyy-cQcPyS9RDhv2alnOcgGCKgTJzxpGjBdUAw4bia6NUFPP_V8qO49DkKXmSACTdX3p8izxwzTOSTQH7hjb-Iqfv6eHtDQDRuPWc_J6uOuDS7uYudevqKEo3wXX6a9XTa-TEBAglFxYdhdRBG5Q5jpY0GLNoO4pmkRNCUc0qSTGDcUN_AlxtKS5Ga6lRc2xj1P6ikRkfmhfkYnL8_fCEpaYLzABy6tnYASIrx05b7SthHa6dBQBee8iDUP4IW4-9qJUBWAFYYOiVMb6s4BTHtYCsm78kG01o3CsCtzT50AAecWNEZV6XpSpyb7m1XgPsysjH1UuW86W2hoSaBD0iwSOS5zJ6RKJHMnKAbrg3RFnsuCO0VzJ9ZVJB8WOtspWuTTEaWa0BbwoOw7NRiG0z8hadKFH4osEQulKLrpOn387lfgWFXIWCZRn5kIx86FsFT7FcqAAPhVpZa5Y7a5bwZZr1w6tYkSkzdPJvHL_-_-E98ggCXH49nX3ZJo_xFSBNhYsdstG3C_cGsFCvd1OQ_wFnRgmo |
openUrl | ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Molecular+simulations+reveal+that+heterogeneous+ice+nucleation+occurs+at+higher+temperatures+in+water+under+capillary+tension&rft.jtitle=Atmospheric+chemistry+and+physics&rft.au=Rosky%2C+Elise&rft.au=Cantrell%2C+Will&rft.au=Li%2C+Tianshu&rft.au=Nakamura%2C+Issei&rft.date=2023-09-26&rft.pub=Copernicus+GmbH&rft.issn=1680-7316&rft.volume=23&rft.issue=18&rft.spage=10625&rft_id=info:doi/10.5194%2Facp-23-10625-2023&rft.externalDBID=ISR&rft.externalDocID=A766675179 |
thumbnail_l | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=1680-7324&client=summon |
thumbnail_m | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=1680-7324&client=summon |
thumbnail_s | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=1680-7324&client=summon |