Mixed-modifier effect in alkaline earth metaphosphate glasses
Modifier-mixing provides a useful tool for tailoring the structural dynamics of oxide glasses. Its physical basis, however, remains subject to intense discussion. Here, we extend our previous consideration of Ca-Mg mixing in alkaline earth metaphosphate glasses [J. Non-Cryst. Solids 468, 74–81 (2017...
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| Published in | Journal of non-crystalline solids Vol. 481; pp. 447 - 456 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2018
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| Online Access | Get full text |
| ISSN | 0022-3093 1873-4812 |
| DOI | 10.1016/j.jnoncrysol.2017.11.041 |
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| Abstract | Modifier-mixing provides a useful tool for tailoring the structural dynamics of oxide glasses. Its physical basis, however, remains subject to intense discussion. Here, we extend our previous consideration of Ca-Mg mixing in alkaline earth metaphosphate glasses [J. Non-Cryst. Solids 468, 74–81 (2017)] across the broader range of alkaline earth species. We report on the effects of divalent modifier mixing for pairs selected from the group of Mg, Ca, Sr and Ba. For this, short-range structural features as obtained from nuclear magnetic resonance, Raman and far-infrared spectroscopy are related to various physical properties, including ionic mobility. Depending primarily on the difference in ion size and bond localization among the modifier cation species, we find different extents of the mixed-modifier effect. This agrees with the dynamic structure model in which the mismatch of cation sites governs non-linear mixing effects. |
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| AbstractList | Modifier-mixing provides a useful tool for tailoring the structural dynamics of oxide glasses. Its physical basis, however, remains subject to intense discussion. Here, we extend our previous consideration of Ca-Mg mixing in alkaline earth metaphosphate glasses [J. Non-Cryst. Solids 468, 74–81 (2017)] across the broader range of alkaline earth species. We report on the effects of divalent modifier mixing for pairs selected from the group of Mg, Ca, Sr and Ba. For this, short-range structural features as obtained from nuclear magnetic resonance, Raman and far-infrared spectroscopy are related to various physical properties, including ionic mobility. Depending primarily on the difference in ion size and bond localization among the modifier cation species, we find different extents of the mixed-modifier effect. This agrees with the dynamic structure model in which the mismatch of cation sites governs non-linear mixing effects. |
| Author | Bragatto, Caio Barca Griebenow, Kristin Kamitsos, Efstratios I. Wondraczek, Lothar |
| Author_xml | – sequence: 1 givenname: Kristin surname: Griebenow fullname: Griebenow, Kristin organization: Otto Schott Institute of Materials Research, University of Jena, Fraunhoferstr. 6, 07743 Jena, Germany – sequence: 2 givenname: Caio Barca surname: Bragatto fullname: Bragatto, Caio Barca organization: Otto Schott Institute of Materials Research, University of Jena, Fraunhoferstr. 6, 07743 Jena, Germany – sequence: 3 givenname: Efstratios I. surname: Kamitsos fullname: Kamitsos, Efstratios I. organization: Theoretical & Physical Chemistry Institute, National Hellenic Research Foundation, 48 Vassileos Constantinou Avenue, 11635, Athens, Greece – sequence: 4 givenname: Lothar orcidid: 0000-0002-0747-3076 surname: Wondraczek fullname: Wondraczek, Lothar email: lothar.wondraczek@uni-jena.de organization: Otto Schott Institute of Materials Research, University of Jena, Fraunhoferstr. 6, 07743 Jena, Germany |
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