Fe‐CoP Electrocatalyst Derived from a Bimetallic Prussian Blue Analogue for Large‐Current‐Density Oxygen Evolution and Overall Water Splitting
Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non‐noble metal catalyst by direct...
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| Published in | Advanced science Vol. 5; no. 10; pp. 1800949 - n/a |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
John Wiley and Sons Inc
01.10.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non‐noble metal catalyst by directly growing a Co‐Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe‐doped CoP (Fe‐CoP) electrocatalyst. The Fe‐CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm−2 current densities in 1.0 m KOH solution. In addition, the Fe‐CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm−2 current density in alkaline solution. Thus, the Fe‐CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm−2 current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO2‐Pt/C‐based electrolyzer.
A gentle and practical pathway is reported to fabricate efficient, non‐noble metal catalyst by directly growing a bimetallic prussian blue analogue 3D conductive substrate, phosphorized into a 3D bifunctional hierarchical‐pore Fe‐CoP electrocatalyst. The as‐obtained Fe‐CoP can drive large‐current‐density oxygen evolution and efficiently catalyze overall water splitting. |
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| AbstractList | Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non‐noble metal catalyst by directly growing a Co‐Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe‐doped CoP (Fe‐CoP) electrocatalyst. The Fe‐CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm
−2
current densities in 1.0
m
KOH solution. In addition, the Fe‐CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm
−2
current density in alkaline solution. Thus, the Fe‐CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm
−2
current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO
2
‐Pt/C‐based electrolyzer. Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non-noble metal catalyst by directly growing a Co-Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe-doped CoP (Fe-CoP) electrocatalyst. The Fe-CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm current densities in 1.0 m KOH solution. In addition, the Fe-CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm current density in alkaline solution. Thus, the Fe-CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO -Pt/C-based electrolyzer. Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non-noble metal catalyst by directly growing a Co-Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe-doped CoP (Fe-CoP) electrocatalyst. The Fe-CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm-2 current densities in 1.0 m KOH solution. In addition, the Fe-CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm-2 current density in alkaline solution. Thus, the Fe-CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm-2 current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO2-Pt/C-based electrolyzer.Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non-noble metal catalyst by directly growing a Co-Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe-doped CoP (Fe-CoP) electrocatalyst. The Fe-CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm-2 current densities in 1.0 m KOH solution. In addition, the Fe-CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm-2 current density in alkaline solution. Thus, the Fe-CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm-2 current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO2-Pt/C-based electrolyzer. Industrial application of overall water splitting requires developing readily available, highly efficient, and stable oxygen evolution electrocatalysts that can efficiently drive large current density. This study reports a facile and practical method to fabricate a non‐noble metal catalyst by directly growing a Co‐Fe Prussian blue analogue on a 3D porous conductive substrate, which is further phosphorized into a bifunctional Fe‐doped CoP (Fe‐CoP) electrocatalyst. The Fe‐CoP/NF (nickel foam) catalyst shows efficient electrocatalytic activity for oxygen evolution reaction, requiring low overpotentials of 190, 295, and 428 mV to achieve 10, 500, and 1000 mA cm−2 current densities in 1.0 m KOH solution. In addition, the Fe‐CoP/NF can also function as a highly active electrocatalyst for hydrogen evolution reaction with a low overpotential of 78 mV at 10 mA cm−2 current density in alkaline solution. Thus, the Fe‐CoP/NF electrode with meso/macropores can act as both an anode and a cathode to fabricate an electrolyzer for overall water splitting, only requiring a cell voltage of 1.49 V to afford a 10 mA cm−2 current density with remarkable stability. This performance appears to be among the best reported values and is much better than that of the IrO2‐Pt/C‐based electrolyzer. A gentle and practical pathway is reported to fabricate efficient, non‐noble metal catalyst by directly growing a bimetallic prussian blue analogue 3D conductive substrate, phosphorized into a 3D bifunctional hierarchical‐pore Fe‐CoP electrocatalyst. The as‐obtained Fe‐CoP can drive large‐current‐density oxygen evolution and efficiently catalyze overall water splitting. |
| Author | Cao, Li‐Ming Wang, Jia‐Wei Hu, Yu‐Wen Iljin, Andrey Zhang, Zhi‐Ming Tang, Shang‐Feng Lu, Tong‐Bu |
| AuthorAffiliation | 2 Institute for New Energy Materials & Low Carbon Technologies School of Materials Science & Engineering Tianjin University of Technology Tianjin 300384 China 1 MOE Key Laboratory of Bioinorganic and Synthetic Chemistry School of Chemistry Sun Yat‐Sen University Guangzhou 510275 China 3 Institute of Physics National Academy of Sciences of Ukraine Prospect Nauki 46 Kyiv 03028 Ukraine |
| AuthorAffiliation_xml | – name: 3 Institute of Physics National Academy of Sciences of Ukraine Prospect Nauki 46 Kyiv 03028 Ukraine – name: 1 MOE Key Laboratory of Bioinorganic and Synthetic Chemistry School of Chemistry Sun Yat‐Sen University Guangzhou 510275 China – name: 2 Institute for New Energy Materials & Low Carbon Technologies School of Materials Science & Engineering Tianjin University of Technology Tianjin 300384 China |
| Author_xml | – sequence: 1 givenname: Li‐Ming surname: Cao fullname: Cao, Li‐Ming organization: Sun Yat‐Sen University – sequence: 2 givenname: Yu‐Wen surname: Hu fullname: Hu, Yu‐Wen organization: Sun Yat‐Sen University – sequence: 3 givenname: Shang‐Feng surname: Tang fullname: Tang, Shang‐Feng organization: Tianjin University of Technology – sequence: 4 givenname: Andrey surname: Iljin fullname: Iljin, Andrey organization: National Academy of Sciences of Ukraine – sequence: 5 givenname: Jia‐Wei surname: Wang fullname: Wang, Jia‐Wei organization: Sun Yat‐Sen University – sequence: 6 givenname: Zhi‐Ming orcidid: 0000-0003-3116-756X surname: Zhang fullname: Zhang, Zhi‐Ming email: zmzhang@email.tjut.edu.cn organization: Tianjin University of Technology – sequence: 7 givenname: Tong‐Bu surname: Lu fullname: Lu, Tong‐Bu email: lutongbu@mail.sysu.edu.cn organization: Tianjin University of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30356966$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | bifunctional electrocatalysts large current density oxygen evolution Prussian blue analogues |
| Title | Fe‐CoP Electrocatalyst Derived from a Bimetallic Prussian Blue Analogue for Large‐Current‐Density Oxygen Evolution and Overall Water Splitting |
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