In situ growth of porphyrinic metal–organic framework nanocrystals on graphene nanoribbons for the electrocatalytic oxidation of nitrite
Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal–organic framework, MOF-525 , by solvothermally growing MOF-525 in a suspension of well-dispersed GNRs. A nanocomposite, which is composed of the MOF-525 nanocrystals interconnected by numerous one-dimensional G...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 4; no. 27; pp. 10673 - 10682 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2016
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal–organic framework,
MOF-525
, by solvothermally growing
MOF-525
in a suspension of well-dispersed GNRs. A nanocomposite, which is composed of the
MOF-525
nanocrystals interconnected by numerous one-dimensional GNRs, is successfully synthesized. Due to the excellent dispersity, uniform thin films of the
MOF-525
/GNR nanocomposite can be simply deposited on conducting glass substrates by using drop casting. The obtained thin film of the
MOF-525
/GNR nanocomposite is applied for electrochemical nitrite sensors. The
MOF-525
nanocrystals serve as a high-surface-area electrocatalyst toward nitrite and the interconnected GNRs act as conductive bridges to provide facile charge transport. The thin film of the
MOF-525
/GNR nanocomposite thus exhibits a much better electrocatalytic activity for the oxidation of nitrite compared to the pristine
MOF-525
thin film. |
|---|---|
| AbstractList | Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal-organic framework, MOF-525, by solvothermally growing MOF-525 in a suspension of well-dispersed GNRs. A nanocomposite, which is composed of the MOF-525 nanocrystals interconnected by numerous one-dimensional GNRs, is successfully synthesized. Due to the excellent dispersity, uniform thin films of the MOF-525/GNR nanocomposite can be simply deposited on conducting glass substrates by using drop casting. The obtained thin film of the MOF-525/GNR nanocomposite is applied for electrochemical nitrite sensors. The MOF-525 nanocrystals serve as a high-surface-area electrocatalyst toward nitrite and the interconnected GNRs act as conductive bridges to provide facile charge transport. The thin film of the MOF-525/GNR nanocomposite thus exhibits a much better electrocatalytic activity for the oxidation of nitrite compared to the pristine MOF-525 thin film. Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal–organic framework, MOF-525 , by solvothermally growing MOF-525 in a suspension of well-dispersed GNRs. A nanocomposite, which is composed of the MOF-525 nanocrystals interconnected by numerous one-dimensional GNRs, is successfully synthesized. Due to the excellent dispersity, uniform thin films of the MOF-525 /GNR nanocomposite can be simply deposited on conducting glass substrates by using drop casting. The obtained thin film of the MOF-525 /GNR nanocomposite is applied for electrochemical nitrite sensors. The MOF-525 nanocrystals serve as a high-surface-area electrocatalyst toward nitrite and the interconnected GNRs act as conductive bridges to provide facile charge transport. The thin film of the MOF-525 /GNR nanocomposite thus exhibits a much better electrocatalytic activity for the oxidation of nitrite compared to the pristine MOF-525 thin film. |
| Author | Lee, Min-Han Ho, Kuo-Chuan Chiang, Wei-Hung Kung, Chung-Wei Li, Yan-Sheng Wang, Shan-Yu |
| Author_xml | – sequence: 1 givenname: Chung-Wei surname: Kung fullname: Kung, Chung-Wei organization: Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan – sequence: 2 givenname: Yan-Sheng surname: Li fullname: Li, Yan-Sheng organization: Department of Chemical Engineering, National Taiwan University of Science and Technology, Taipei 10617, Taiwan – sequence: 3 givenname: Min-Han surname: Lee fullname: Lee, Min-Han organization: Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan – sequence: 4 givenname: Shan-Yu surname: Wang fullname: Wang, Shan-Yu organization: Department of Chemical Engineering, National Taiwan University of Science and Technology, Taipei 10617, Taiwan – sequence: 5 givenname: Wei-Hung surname: Chiang fullname: Chiang, Wei-Hung organization: Department of Chemical Engineering, National Taiwan University of Science and Technology, Taipei 10617, Taiwan – sequence: 6 givenname: Kuo-Chuan surname: Ho fullname: Ho, Kuo-Chuan organization: Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan, Institute of Polymer Science and Engineering |
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| Snippet | Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal–organic framework,
MOF-525
, by solvothermally growing
MOF-525
in a... Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal-organic framework, MOF-525, by solvothermally growing MOF-525 in a... Graphene nanoribbons (GNRs) are incorporated with the nanocrystals of a porphyrinic metal–organic framework, MOF-525, by solvothermally growing MOF-525 in a... |
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| SubjectTerms | catalysts coordination polymers electrochemistry glass Graphene Metal-organic frameworks Nanocomposites Nanocrystals Nanostructure Nitrites Oxidation Thin films |
| Title | In situ growth of porphyrinic metal–organic framework nanocrystals on graphene nanoribbons for the electrocatalytic oxidation of nitrite |
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