A review of conversion of lignocellulose biomass to liquid transport fuels by integrated refining strategies

Due to the limitations on carbon emissions, many countries are seeking potential clean, renewable and sustainable energy and fuels. Conversion of lignocellulose biomass to liquid fuel is one of the research hotpots because biomass is a renewable and sustainable resource. This paper outlines an attra...

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Published inFuel processing technology Vol. 208; p. 106485
Main Authors Wang, Chenguang, Zhang, Xinghua, Liu, Qiang, Zhang, Qi, Chen, Lungang, Ma, Longlong
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 01.11.2020
Elsevier Science Ltd
Subjects
Alkanes
Aromatic compounds
aromatic hydrocarbons
Aviation fuel
Biomass
Biomass energy production
carbon
catalytic activity
cellulose
Chemical synthesis
Clean energy
Conversion
Depolymerization
Dimers
emissions
fuels
Gasoline
hemicellulose
Hydrocarbons
Hydrodeoxygenation
Lignin
Lignocellulose
Lignocellulosic biomass
Liquid fuels
liquids
Platform molecule
refining
renewable energy sources
State-of-the-art reviews
Depolymerization
Hydrocarbons
Hydrodeoxygenation
Lignocellulosic biomass
Platform molecule
Online AccessGet full text
ISSN0378-3820
1873-7188
DOI10.1016/j.fuproc.2020.106485

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Abstract Due to the limitations on carbon emissions, many countries are seeking potential clean, renewable and sustainable energy and fuels. Conversion of lignocellulose biomass to liquid fuel is one of the research hotpots because biomass is a renewable and sustainable resource. This paper outlines an attractive strategy for the production of liquid transport fuels from lignocellulose biomass. Specifically, hemicellulose and cellulose are converted to C5 and C6 alkanes (bio-gasoline) and C8–C15 alkanes (aviation fuel) via C5/C6 platform molecules, and lignin is converted to arenes and cyclanes via phenolic monomers and dimers through hydrodeoxygenation. The focus is to review the state-of-the-art technologies for the preparation of platform molecules, the synthesis of light/heavy alkanes, lignin depolymerization and catalytic hydrodeoxygenation. In addition, major challenges and promising prospects are also pointed out for the future development of the conversion of lignocellulose biomass to liquid transport fuels. Integrated conversion is an attractive strategy for the production of hydrocarbon fuels from lignocellulose biomass. Hemicellulose and cellulose can be converted to bio-gasoline (C5 and C6 alkanes) and aviation fuel (C8–C15 alkanes) via C5/C6 platform molecules, and lignin can be converted to arenes and cyclanes via phenolic monomers and dimers through hydrodeoxygenation. This review provides a new perspective for utilization of lignocellulose biomass. [Display omitted] •Technologies for bio-gasoline production from hemicellulose and cellulose were summarized.•The state-of-the-art technologies for synthesis of aviation fuel were reviewed.•Lignin was proposed to be the feedstock of arenes and cyclanes.•Challenges and prospects of utilization of lignocellulose biomass were discussed.
AbstractList Due to the limitations on carbon emissions, many countries are seeking potential clean, renewable and sustainable energy and fuels. Conversion of lignocellulose biomass to liquid fuel is one of the research hotpots because biomass is a renewable and sustainable resource. This paper outlines an attractive strategy for the production of liquid transport fuels from lignocellulose biomass. Specifically, hemicellulose and cellulose are converted to C5 and C6 alkanes (bio-gasoline) and C8–C15 alkanes (aviation fuel) via C5/C6 platform molecules, and lignin is converted to arenes and cyclanes via phenolic monomers and dimers through hydrodeoxygenation. The focus is to review the state-of-the-art technologies for the preparation of platform molecules, the synthesis of light/heavy alkanes, lignin depolymerization and catalytic hydrodeoxygenation. In addition, major challenges and promising prospects are also pointed out for the future development of the conversion of lignocellulose biomass to liquid transport fuels.
Due to the limitations on carbon emissions, many countries are seeking potential clean, renewable and sustainable energy and fuels. Conversion of lignocellulose biomass to liquid fuel is one of the research hotpots because biomass is a renewable and sustainable resource. This paper outlines an attractive strategy for the production of liquid transport fuels from lignocellulose biomass. Specifically, hemicellulose and cellulose are converted to C5 and C6 alkanes (bio-gasoline) and C8–C15 alkanes (aviation fuel) via C5/C6 platform molecules, and lignin is converted to arenes and cyclanes via phenolic monomers and dimers through hydrodeoxygenation. The focus is to review the state-of-the-art technologies for the preparation of platform molecules, the synthesis of light/heavy alkanes, lignin depolymerization and catalytic hydrodeoxygenation. In addition, major challenges and promising prospects are also pointed out for the future development of the conversion of lignocellulose biomass to liquid transport fuels. Integrated conversion is an attractive strategy for the production of hydrocarbon fuels from lignocellulose biomass. Hemicellulose and cellulose can be converted to bio-gasoline (C5 and C6 alkanes) and aviation fuel (C8–C15 alkanes) via C5/C6 platform molecules, and lignin can be converted to arenes and cyclanes via phenolic monomers and dimers through hydrodeoxygenation. This review provides a new perspective for utilization of lignocellulose biomass. [Display omitted] •Technologies for bio-gasoline production from hemicellulose and cellulose were summarized.•The state-of-the-art technologies for synthesis of aviation fuel were reviewed.•Lignin was proposed to be the feedstock of arenes and cyclanes.•Challenges and prospects of utilization of lignocellulose biomass were discussed.
ArticleNumber 106485
Author Chen, Lungang
Zhang, Qi
Wang, Chenguang
Liu, Qiang
Ma, Longlong
Zhang, Xinghua
Author_xml – sequence: 1
  givenname: Chenguang
  surname: Wang
  fullname: Wang, Chenguang
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
– sequence: 2
  givenname: Xinghua
  surname: Zhang
  fullname: Zhang, Xinghua
  email: zhangxh@ms.giec.ac.cn
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
– sequence: 3
  givenname: Qiang
  surname: Liu
  fullname: Liu, Qiang
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
– sequence: 4
  givenname: Qi
  surname: Zhang
  fullname: Zhang, Qi
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
– sequence: 5
  givenname: Lungang
  surname: Chen
  fullname: Chen, Lungang
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
– sequence: 6
  givenname: Longlong
  surname: Ma
  fullname: Ma, Longlong
  email: mall@ms.giec.ac.cn
  organization: Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China
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Snippet Due to the limitations on carbon emissions, many countries are seeking potential clean, renewable and sustainable energy and fuels. Conversion of...
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SubjectTerms Alkanes
Aromatic compounds
aromatic hydrocarbons
Aviation fuel
Biomass
Biomass energy production
carbon
catalytic activity
cellulose
Chemical synthesis
Clean energy
Conversion
Depolymerization
Dimers
emissions
fuels
Gasoline
hemicellulose
Hydrocarbons
Hydrodeoxygenation
Lignin
Lignocellulose
Lignocellulosic biomass
Liquid fuels
liquids
Platform molecule
refining
renewable energy sources
State-of-the-art reviews
Title A review of conversion of lignocellulose biomass to liquid transport fuels by integrated refining strategies
URI https://dx.doi.org/10.1016/j.fuproc.2020.106485
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