Size-controlled nitrogen-containing mesoporous carbon nanospheres by one-step aqueous self-assembly strategy
Nitrogen-containing mesoporous carbon nanospheres with tunable sizes have been prepared through an aqueous self-assembly process with F127 as a template and morphological control agent, and 3-aminophenol as carbon and nitrogen sources. The sphere sizes could be simply tuned by optimizing the concent...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 3; no. 5; pp. 2305 - 2313 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Nitrogen-containing mesoporous carbon nanospheres with tunable sizes have been prepared through an aqueous self-assembly process with F127 as a template and morphological control agent, and 3-aminophenol as carbon and nitrogen sources. The sphere sizes could be simply tuned by optimizing the concentration of F127 and ammonia. Compared with a traditional nanocasting method and a hydrothermal process, the present one-step method has the striking features of a simple synthesis process and easy introduction of the nitrogen atom into the carbon nanospheres. The feasibility of the fabrication method may open up a new way for the synthesis of heteroatom-containing carbon nanospheres with mesoporous structure. The prepared nitrogen-containing mesoporous carbon nanospheres exhibit good catalytic performance in the direct dehydrogenation of ethylbenzene due to their unique mesostructure and abundant oxygen and nitrogen functional groups. |
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| AbstractList | Nitrogen-containing mesoporous carbon nanospheres with tunable sizes have been prepared through an aqueous self-assembly process with F127 as a template and morphological control agent, and 3-aminophenol as carbon and nitrogen sources. The sphere sizes could be simply tuned by optimizing the concentration of F127 and ammonia. Compared with a traditional nanocasting method and a hydrothermal process, the present one-step method has the striking features of a simple synthesis process and easy introduction of the nitrogen atom into the carbon nanospheres. The feasibility of the fabrication method may open up a new way for the synthesis of heteroatom-containing carbon nanospheres with mesoporous structure. The prepared nitrogen-containing mesoporous carbon nanospheres exhibit good catalytic performance in the direct dehydrogenation of ethylbenzene due to their unique mesostructure and abundant oxygen and nitrogen functional groups. |
| Author | Zong, Baoning Diao, Jiangyong Gu, Xianmo Wang, Haihua Liu, Hongyang Wang, Jia Rong, Junfeng Su, Dang Sheng |
| Author_xml | – sequence: 1 givenname: Jia surname: Wang fullname: Wang, Jia organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China – sequence: 2 givenname: Hongyang surname: Liu fullname: Liu, Hongyang organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China – sequence: 3 givenname: Jiangyong surname: Diao fullname: Diao, Jiangyong organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China – sequence: 4 givenname: Xianmo surname: Gu fullname: Gu, Xianmo organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China – sequence: 5 givenname: Haihua surname: Wang fullname: Wang, Haihua organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China – sequence: 6 givenname: Junfeng surname: Rong fullname: Rong, Junfeng organization: Research Institute of Petroleum Processing, Beijing, P.R. China – sequence: 7 givenname: Baoning surname: Zong fullname: Zong, Baoning organization: Research Institute of Petroleum Processing, Beijing, P.R. China – sequence: 8 givenname: Dang Sheng surname: Su fullname: Su, Dang Sheng organization: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, P.R. China |
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| Snippet | Nitrogen-containing mesoporous carbon nanospheres with tunable sizes have been prepared through an aqueous self-assembly process with F127 as a template and... |
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| SubjectTerms | aminophenols ammonia Carbon catalytic activity dehydrogenation ethylbenzene Feasibility moieties Nanospheres nitrogen Optimization oxygen porous media Self assembly Strategy Sustainability Synthesis |
| Title | Size-controlled nitrogen-containing mesoporous carbon nanospheres by one-step aqueous self-assembly strategy |
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