Metal-organic framework derived carbon materials for electrocatalytic oxygen reactions: Recent progress and future perspectives
The electrocatalytic oxygen reactions, i.e. oxygen reduction/evolution reactions (ORR/OER), play a key role in electrochemical energy conversion and storage devices, including fuel cells, electrolyzers, and metal-air batteries, and have attracted significant attention in the past decades. Platinum-g...
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| Published in | Carbon (New York) Vol. 156; pp. 77 - 92 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Elsevier Ltd
01.01.2020
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0008-6223 1873-3891 |
| DOI | 10.1016/j.carbon.2019.09.029 |
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| Abstract | The electrocatalytic oxygen reactions, i.e. oxygen reduction/evolution reactions (ORR/OER), play a key role in electrochemical energy conversion and storage devices, including fuel cells, electrolyzers, and metal-air batteries, and have attracted significant attention in the past decades. Platinum-group metal (PGM)-free materials have been intensively investigated as alternatives to replace the well-accepted but costly PGM-based catalysts such as Pt for ORR and Ir/Ru (oxides) for OER. Particularly, metal-organic framework (MOF)-derived carbon materials are emerging PGM-free catalysts for ORR/OER. So far, excellent works have been achieved to enhance the activity and durability of the MOF-derived PGM-free catalysts. It is the occasion to promote the PGM-free catalysts to the next level of application, i.e. in real devices. However, ORR/OER in real devices are potentially subject to the porosity related challenges, e.g. electron/mass transfer issue and active site isolation in organic Li-air batteries. To address these challenges, the rational design of porous electrocatalyst for devices is required. In this review, we summarize the most recent progress of MOF-derived carbon materials for ORR/OER with the focus on not only the active site engineering but also the design of porous structure. We also provide perspectives on the rational design of PGM-free catalysts using MOF as precursors.
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| AbstractList | The electrocatalytic oxygen reactions, i.e. oxygen reduction/evolution reactions (ORR/OER), play a key role in electrochemical energy conversion and storage devices, including fuel cells, electrolyzers, and metal-air batteries, and have attracted significant attention in the past decades. Platinum-group metal (PGM)-free materials have been intensively investigated as alternatives to replace the well-accepted but costly PGM-based catalysts such as Pt for ORR and Ir/Ru (oxides) for OER. Particularly, metal-organic framework (MOF)-derived carbon materials are emerging PGM-free catalysts for ORR/OER. So far, excellent works have been achieved to enhance the activity and durability of the MOF-derived PGM-free catalysts. It is the occasion to promote the PGM-free catalysts to the next level of application, i.e. in real devices. However, ORR/OER in real devices are potentially subject to the porosity related challenges, e.g. electron/mass transfer issue and active site isolation in organic Li-air batteries. To address these challenges, the rational design of porous electrocatalyst for devices is required. In this review, we summarize the most recent progress of MOF-derived carbon materials for ORR/OER with the focus on not only the active site engineering but also the design of porous structure. We also provide perspectives on the rational design of PGM-free catalysts using MOF as precursors. The electrocatalytic oxygen reactions, i.e. oxygen reduction/evolution reactions (ORR/OER), play a key role in electrochemical energy conversion and storage devices, including fuel cells, electrolyzers, and metal-air batteries, and have attracted significant attention in the past decades. Platinum-group metal (PGM)-free materials have been intensively investigated as alternatives to replace the well-accepted but costly PGM-based catalysts such as Pt for ORR and Ir/Ru (oxides) for OER. Particularly, metal-organic framework (MOF)-derived carbon materials are emerging PGM-free catalysts for ORR/OER. So far, excellent works have been achieved to enhance the activity and durability of the MOF-derived PGM-free catalysts. It is the occasion to promote the PGM-free catalysts to the next level of application, i.e. in real devices. However, ORR/OER in real devices are potentially subject to the porosity related challenges, e.g. electron/mass transfer issue and active site isolation in organic Li-air batteries. To address these challenges, the rational design of porous electrocatalyst for devices is required. In this review, we summarize the most recent progress of MOF-derived carbon materials for ORR/OER with the focus on not only the active site engineering but also the design of porous structure. We also provide perspectives on the rational design of PGM-free catalysts using MOF as precursors. [Display omitted] |
| Author | Sun, Shuhui Du, Lei Xing, Lixin Zhang, Gaixia |
| Author_xml | – sequence: 1 givenname: Lei orcidid: 0000-0001-9584-4748 surname: Du fullname: Du, Lei organization: Institut National de la Recherche Scientifique-Énergie Matériaux et Télécommunications, Varennes, QC, J3X 1S2, Canada – sequence: 2 givenname: Lixin surname: Xing fullname: Xing, Lixin organization: Institut National de la Recherche Scientifique-Énergie Matériaux et Télécommunications, Varennes, QC, J3X 1S2, Canada – sequence: 3 givenname: Gaixia surname: Zhang fullname: Zhang, Gaixia email: gaixia.zhang@emt.inrs.ca organization: Institut National de la Recherche Scientifique-Énergie Matériaux et Télécommunications, Varennes, QC, J3X 1S2, Canada – sequence: 4 givenname: Shuhui surname: Sun fullname: Sun, Shuhui email: shuhui@emt.inrs.ca organization: Institut National de la Recherche Scientifique-Énergie Matériaux et Télécommunications, Varennes, QC, J3X 1S2, Canada |
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| PublicationYear | 2020 |
| Publisher | Elsevier Ltd Elsevier BV |
| Publisher_xml | – name: Elsevier Ltd – name: Elsevier BV |
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| SubjectTerms | active sites batteries Carbon Catalysts catalytic activity Chemical reactions coordination polymers Devices durability Electrocatalysis electrochemistry Electrolytic cells Energy conversion Energy management Energy storage engineering Fuel cells Iridium Mass transfer Metal air batteries Metal-organic frameworks oxides Oxygen Oxygen evolution Oxygen reduction Platinum Porosity Porous structure ruthenium Storage batteries |
| Title | Metal-organic framework derived carbon materials for electrocatalytic oxygen reactions: Recent progress and future perspectives |
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