Supported Photocatalyst for Removal of Emerging Contaminants from Wastewater in a Continuous Packed-Bed Photoreactor Configuration

Water pollution from emerging contaminants (ECs) or emerging pollutants is an important environmental problem. Heterogeneous photocatalytic treatment, as advanced oxidation treatment of wastewater effluents, has been proposed to solve this problem. In this paper, a heterogeneous photocatalytic proce...

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Published inCatalysts Vol. 5; no. 1; pp. 77 - 87
Main Authors Borges, Ma Emma, Garcia, Dulce Maria, Hernandez, Tania, Ruiz-Morales, Juan Carlos, Esparza, Pedro
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 01.03.2015
Subjects
advanced oxidation technology (AOT)
Catalysts
Chemical reactions
Contaminants
emerging contaminants (ECs)
endocrine disrupting chemicals (EDCs)
glass spheres
heterogeneous photocatalysis
paracetamol
Photocatalysis
Scanning electron microscopy
Surface chemistry
Texture
TiO2
Titanium dioxide
Waste water
Wastewater treatment
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Abstract Water pollution from emerging contaminants (ECs) or emerging pollutants is an important environmental problem. Heterogeneous photocatalytic treatment, as advanced oxidation treatment of wastewater effluents, has been proposed to solve this problem. In this paper, a heterogeneous photocatalytic process was studied for emergent contaminants removal using paracetamol as a model contaminant molecule. TiO2 photocatalytic activity was evaluated using two photocatalytic reactor configurations: Photocatalyst solid suspension in wastewater in a stirred photoreactor and TiO2 supported on glass spheres (TGS) configuring a packed bed photoreactor. The surface morphology and texture of the TGS were monitored by scanning electron microscope (SEM). The influence of photocatalyst amount and wastewater pH were evaluated in the stirred photoreactor and the influence of wastewater flowrate was tested in the packed bed photoreactor, in order to obtain the optimal operation conditions. Moreover, results obtained were compared with those obtained from photolysis and adsorption studies, using the optimal operation conditions. Good photocatalytic activities have been observed and leads to the conclusion that the heterogeneous photocatalytic system in a packed bed is an effective method for removal of emerging pollutants.
AbstractList Water pollution from emerging contaminants (ECs) or emerging pollutants is an important environmental problem. Heterogeneous photocatalytic treatment, as advanced oxidation treatment of wastewater effluents, has been proposed to solve this problem. In this paper, a heterogeneous photocatalytic process was studied for emergent contaminants removal using paracetamol as a model contaminant molecule. TiO2 photocatalytic activity was evaluated using two photocatalytic reactor configurations: Photocatalyst solid suspension in wastewater in a stirred photoreactor and TiO2 supported on glass spheres (TGS) configuring a packed bed photoreactor. The surface morphology and texture of the TGS were monitored by scanning electron microscope (SEM). The influence of photocatalyst amount and wastewater pH were evaluated in the stirred photoreactor and the influence of wastewater flowrate was tested in the packed bed photoreactor, in order to obtain the optimal operation conditions. Moreover, results obtained were compared with those obtained from photolysis and adsorption studies, using the optimal operation conditions. Good photocatalytic activities have been observed and leads to the conclusion that the heterogeneous photocatalytic system in a packed bed is an effective method for removal of emerging pollutants.
Author Ruiz-Morales, Juan Carlos
Garcia, Dulce Maria
Hernandez, Tania
Esparza, Pedro
Borges, Ma Emma
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SubjectTerms advanced oxidation technology (AOT)
Catalysts
Chemical reactions
Contaminants
emerging contaminants (ECs)
endocrine disrupting chemicals (EDCs)
glass spheres
heterogeneous photocatalysis
paracetamol
Photocatalysis
Scanning electron microscopy
Surface chemistry
Texture
TiO2
Titanium dioxide
Waste water
Wastewater treatment
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Title Supported Photocatalyst for Removal of Emerging Contaminants from Wastewater in a Continuous Packed-Bed Photoreactor Configuration
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