In-situ construction of ternary Ti3C2 MXene@TiO2/ZnIn2S4 composites for highly efficient photocatalytic hydrogen evolution
[Display omitted] Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti3C2 MXene@TiO2/ZnIn2S4 photocatalyst with rapid charge...
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| Published in | Journal of colloid and interface science Vol. 580; pp. 669 - 680 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.11.2020
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0021-9797 1095-7103 1095-7103 |
| DOI | 10.1016/j.jcis.2020.07.044 |
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| Abstract | [Display omitted]
Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti3C2 MXene@TiO2/ZnIn2S4 photocatalyst with rapid charge transfer channels was constructed by two-step hydrothermal for efficient hydrogen production, adopting hydrothermal oxidation to in-situ synthesize Ti3C2 MXene embedded with TiO2 nanosheets (M@TiO2), which was applied to load ZnIn2S4 (ZIS). The hybridized photocatalyst with optimized ZIS amount had a hydrogen generation rate of 1185.8 μmol/g/h, which was higher than that of M@TiO2 and pure ZIS. That was originated from the outstanding light harvesting of ZIS and Ti3C2, sufficient active sites of Ti3C2, intimate interfacial contact, and efficient separation and transfer of photogenerated charges via heterojunction. The favorable and rapid charge transfer routes included type-II heterojunction between ZIS and TiO2 nanosheets, Schottky junction of Ti3C2/semiconductor, and metallic Ti3C2 with high conductivity. This work revealed the Schottky junction forming between ZIS and Ti3C2, and hierarchical M@TiO2 could be served as advantageous platform and efficient cocatalyst to construct MXene-based photocatalyst. |
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| AbstractList | Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti₃C₂ MXene@TiO₂/ZnIn₂S₄ photocatalyst with rapid charge transfer channels was constructed by two-step hydrothermal for efficient hydrogen production, adopting hydrothermal oxidation to in-situ synthesize Ti₃C₂ MXene embedded with TiO₂ nanosheets (M@TiO₂), which was applied to load ZnIn₂S₄ (ZIS). The hybridized photocatalyst with optimized ZIS amount had a hydrogen generation rate of 1185.8 μmol/g/h, which was higher than that of M@TiO₂ and pure ZIS. That was originated from the outstanding light harvesting of ZIS and Ti₃C₂, sufficient active sites of Ti₃C₂, intimate interfacial contact, and efficient separation and transfer of photogenerated charges via heterojunction. The favorable and rapid charge transfer routes included type-II heterojunction between ZIS and TiO₂ nanosheets, Schottky junction of Ti₃C₂/semiconductor, and metallic Ti₃C₂ with high conductivity. This work revealed the Schottky junction forming between ZIS and Ti₃C₂, and hierarchical M@TiO₂ could be served as advantageous platform and efficient cocatalyst to construct MXene-based photocatalyst. Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti3C2 MXene@TiO2/ZnIn2S4 photocatalyst with rapid charge transfer channels was constructed by two-step hydrothermal for efficient hydrogen production, adopting hydrothermal oxidation to in-situ synthesize Ti3C2 MXene embedded with TiO2 nanosheets (M@TiO2), which was applied to load ZnIn2S4 (ZIS). The hybridized photocatalyst with optimized ZIS amount had a hydrogen generation rate of 1185.8 μmol/g/h, which was higher than that of M@TiO2 and pure ZIS. That was originated from the outstanding light harvesting of ZIS and Ti3C2, sufficient active sites of Ti3C2, intimate interfacial contact, and efficient separation and transfer of photogenerated charges via heterojunction. The favorable and rapid charge transfer routes included type-II heterojunction between ZIS and TiO2 nanosheets, Schottky junction of Ti3C2/semiconductor, and metallic Ti3C2 with high conductivity. This work revealed the Schottky junction forming between ZIS and Ti3C2, and hierarchical M@TiO2 could be served as advantageous platform and efficient cocatalyst to construct MXene-based photocatalyst.Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti3C2 MXene@TiO2/ZnIn2S4 photocatalyst with rapid charge transfer channels was constructed by two-step hydrothermal for efficient hydrogen production, adopting hydrothermal oxidation to in-situ synthesize Ti3C2 MXene embedded with TiO2 nanosheets (M@TiO2), which was applied to load ZnIn2S4 (ZIS). The hybridized photocatalyst with optimized ZIS amount had a hydrogen generation rate of 1185.8 μmol/g/h, which was higher than that of M@TiO2 and pure ZIS. That was originated from the outstanding light harvesting of ZIS and Ti3C2, sufficient active sites of Ti3C2, intimate interfacial contact, and efficient separation and transfer of photogenerated charges via heterojunction. The favorable and rapid charge transfer routes included type-II heterojunction between ZIS and TiO2 nanosheets, Schottky junction of Ti3C2/semiconductor, and metallic Ti3C2 with high conductivity. This work revealed the Schottky junction forming between ZIS and Ti3C2, and hierarchical M@TiO2 could be served as advantageous platform and efficient cocatalyst to construct MXene-based photocatalyst. [Display omitted] Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy conversion for solving energy crisis. Hence, a novel hierarchical Ti3C2 MXene@TiO2/ZnIn2S4 photocatalyst with rapid charge transfer channels was constructed by two-step hydrothermal for efficient hydrogen production, adopting hydrothermal oxidation to in-situ synthesize Ti3C2 MXene embedded with TiO2 nanosheets (M@TiO2), which was applied to load ZnIn2S4 (ZIS). The hybridized photocatalyst with optimized ZIS amount had a hydrogen generation rate of 1185.8 μmol/g/h, which was higher than that of M@TiO2 and pure ZIS. That was originated from the outstanding light harvesting of ZIS and Ti3C2, sufficient active sites of Ti3C2, intimate interfacial contact, and efficient separation and transfer of photogenerated charges via heterojunction. The favorable and rapid charge transfer routes included type-II heterojunction between ZIS and TiO2 nanosheets, Schottky junction of Ti3C2/semiconductor, and metallic Ti3C2 with high conductivity. This work revealed the Schottky junction forming between ZIS and Ti3C2, and hierarchical M@TiO2 could be served as advantageous platform and efficient cocatalyst to construct MXene-based photocatalyst. |
| Author | Meng, Xiangchao Li, Chunhu Huang, Kelei |
| Author_xml | – sequence: 1 givenname: Kelei surname: Huang fullname: Huang, Kelei – sequence: 2 givenname: Chunhu orcidid: 0000-0001-7374-3719 surname: Li fullname: Li, Chunhu email: lichunhu@ouc.edu.cn – sequence: 3 givenname: Xiangchao orcidid: 0000-0001-9896-8690 surname: Meng fullname: Meng, Xiangchao email: mengxiangchao@ouc.edu.cn |
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Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize... Facing the demand of cleaning energy, the development of efficient photocatalysts for hydrogen evolution is a promising way to realize solar-to-chemical energy... |
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| SubjectTerms | active sites carbides energy conversion Hydrogen evolution hydrogen production indium nanosheets oxidation photocatalysis photocatalysts Schottky junction semiconductors sulfides Ti3C2 MXene TiO2 titanium titanium dioxide zinc ZnIn2S4 |
| Title | In-situ construction of ternary Ti3C2 MXene@TiO2/ZnIn2S4 composites for highly efficient photocatalytic hydrogen evolution |
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