Broadband electromagnetic wave absorption using pure carbon aerogel by synergistically modulating propagation path and carbonization degree
[Display omitted] Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effe...
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| Published in | Journal of colloid and interface science Vol. 652; no. Pt A; pp. 780 - 788 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
15.12.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effective absorption. Herein, a novel strategy using pure carbon aerogel with oriented structure was reported to enhance the EM wave absorption by synergistically modulating the wave propagation path and carbonization degree. The aerogel contained proposed modified carbon nanofibers (MCNF) derived from bacterial cellulose (BC), and core-shell carbon nanofibers @ reduced oxide graphene (CNF@RGO). The oriented structure was induced by the temperature field, which manifests anisotropic EM constitutive parameters (εx ≠ εz) at different directions of incident wave. The carbonization degree was adjusted by varying the carbonization temperature. At the carbonization temperature of 700 °C, the maximum reflection loss and effective absorption bandwidth reached −53.94 dB and 7.14 GHz, respectively, enabling the aerogel to outperform its previous counterparts. To clarify the EM wave mode-of-action in conjunction, physical models of the aerogel were established in addition to finite element simulation and theoretical analysis. Notably, the aerogel with a density of 3.6 mg/cm3 featured ultra-light weight, superhydrophobicity, superior compressibility, and thermal insulation. Our work offers an efficient strategy for designing broadband and multifunctional EM wave absorption materials (EWAMs), promising great potentials in complex stealth equipment. |
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| AbstractList | Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effective absorption. Herein, a novel strategy using pure carbon aerogel with oriented structure was reported to enhance the EM wave absorption by synergistically modulating the wave propagation path and carbonization degree. The aerogel contained proposed modified carbon nanofibers (MCNF) derived from bacterial cellulose (BC), and core-shell carbon nanofibers @ reduced oxide graphene (CNF@RGO). The oriented structure was induced by the temperature field, which manifests anisotropic EM constitutive parameters (εx ≠ εz) at different directions of incident wave. The carbonization degree was adjusted by varying the carbonization temperature. At the carbonization temperature of 700 °C, the maximum reflection loss and effective absorption bandwidth reached -53.94 dB and 7.14 GHz, respectively, enabling the aerogel to outperform its previous counterparts. To clarify the EM wave mode-of-action in conjunction, physical models of the aerogel were established in addition to finite element simulation and theoretical analysis. Notably, the aerogel with a density of 3.6 mg/cm3 featured ultra-light weight, superhydrophobicity, superior compressibility, and thermal insulation. Our work offers an efficient strategy for designing broadband and multifunctional EM wave absorption materials (EWAMs), promising great potentials in complex stealth equipment.Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effective absorption. Herein, a novel strategy using pure carbon aerogel with oriented structure was reported to enhance the EM wave absorption by synergistically modulating the wave propagation path and carbonization degree. The aerogel contained proposed modified carbon nanofibers (MCNF) derived from bacterial cellulose (BC), and core-shell carbon nanofibers @ reduced oxide graphene (CNF@RGO). The oriented structure was induced by the temperature field, which manifests anisotropic EM constitutive parameters (εx ≠ εz) at different directions of incident wave. The carbonization degree was adjusted by varying the carbonization temperature. At the carbonization temperature of 700 °C, the maximum reflection loss and effective absorption bandwidth reached -53.94 dB and 7.14 GHz, respectively, enabling the aerogel to outperform its previous counterparts. To clarify the EM wave mode-of-action in conjunction, physical models of the aerogel were established in addition to finite element simulation and theoretical analysis. Notably, the aerogel with a density of 3.6 mg/cm3 featured ultra-light weight, superhydrophobicity, superior compressibility, and thermal insulation. Our work offers an efficient strategy for designing broadband and multifunctional EM wave absorption materials (EWAMs), promising great potentials in complex stealth equipment. [Display omitted] Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effective absorption. Herein, a novel strategy using pure carbon aerogel with oriented structure was reported to enhance the EM wave absorption by synergistically modulating the wave propagation path and carbonization degree. The aerogel contained proposed modified carbon nanofibers (MCNF) derived from bacterial cellulose (BC), and core-shell carbon nanofibers @ reduced oxide graphene (CNF@RGO). The oriented structure was induced by the temperature field, which manifests anisotropic EM constitutive parameters (εx ≠ εz) at different directions of incident wave. The carbonization degree was adjusted by varying the carbonization temperature. At the carbonization temperature of 700 °C, the maximum reflection loss and effective absorption bandwidth reached −53.94 dB and 7.14 GHz, respectively, enabling the aerogel to outperform its previous counterparts. To clarify the EM wave mode-of-action in conjunction, physical models of the aerogel were established in addition to finite element simulation and theoretical analysis. Notably, the aerogel with a density of 3.6 mg/cm3 featured ultra-light weight, superhydrophobicity, superior compressibility, and thermal insulation. Our work offers an efficient strategy for designing broadband and multifunctional EM wave absorption materials (EWAMs), promising great potentials in complex stealth equipment. Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical conductivity. However, conventional means were typically available by combining carbon and other materials to achieve effective absorption. Herein, a novel strategy using pure carbon aerogel with oriented structure was reported to enhance the EM wave absorption by synergistically modulating the wave propagation path and carbonization degree. The aerogel contained proposed modified carbon nanofibers (MCNF) derived from bacterial cellulose (BC), and core-shell carbon nanofibers @ reduced oxide graphene (CNF@RGO). The oriented structure was induced by the temperature field, which manifests anisotropic EM constitutive parameters (εₓ ≠ εz) at different directions of incident wave. The carbonization degree was adjusted by varying the carbonization temperature. At the carbonization temperature of 700 °C, the maximum reflection loss and effective absorption bandwidth reached −53.94 dB and 7.14 GHz, respectively, enabling the aerogel to outperform its previous counterparts. To clarify the EM wave mode-of-action in conjunction, physical models of the aerogel were established in addition to finite element simulation and theoretical analysis. Notably, the aerogel with a density of 3.6 mg/cm³ featured ultra-light weight, superhydrophobicity, superior compressibility, and thermal insulation. Our work offers an efficient strategy for designing broadband and multifunctional EM wave absorption materials (EWAMs), promising great potentials in complex stealth equipment. |
| Author | Han, Mengjie Liu, Yaqing Xu, He-Xiu Wu, Qilei Zhang, Bin Su, Xiaogang Wang, Jun Liu, Yanan Huo, Siqi |
| Author_xml | – sequence: 1 givenname: Xiaogang orcidid: 0000-0002-9323-3916 surname: Su fullname: Su, Xiaogang email: sxgwhut@163.com organization: Key Laboratory of Functional Nanocomposites of Shanxi Province, School of Materials Science and Engineering, North University of China, Taiyuan 030051, China – sequence: 2 givenname: Jun surname: Wang fullname: Wang, Jun organization: Key Laboratory of Functional Nanocomposites of Shanxi Province, School of Materials Science and Engineering, North University of China, Taiyuan 030051, China – sequence: 3 givenname: Mengjie surname: Han fullname: Han, Mengjie organization: Key Laboratory of Functional Nanocomposites of Shanxi Province, School of Materials Science and Engineering, North University of China, Taiyuan 030051, China – sequence: 4 givenname: Yanan surname: Liu fullname: Liu, Yanan organization: Key Laboratory of Functional Nanocomposites of Shanxi Province, School of Materials Science and Engineering, North University of China, Taiyuan 030051, China – sequence: 5 givenname: Bin surname: Zhang fullname: Zhang, Bin organization: School of Materials Science and Engineering, Wuhan Textile University, Wuhan 430200, China – sequence: 6 givenname: Siqi orcidid: 0000-0002-6454-5208 surname: Huo fullname: Huo, Siqi organization: Center for Future Materials, University of Southern Queensland, Springfield 4300, Australia – sequence: 7 givenname: Qilei surname: Wu fullname: Wu, Qilei organization: Science and Technology on Electromagnetic Compatibility Laboratory, China Ship Development and Design Centre, Wuhan 430070, China – sequence: 8 givenname: Yaqing surname: Liu fullname: Liu, Yaqing email: lyq@nuc.edu.cn organization: Key Laboratory of Functional Nanocomposites of Shanxi Province, School of Materials Science and Engineering, North University of China, Taiyuan 030051, China – sequence: 9 givenname: He-Xiu surname: Xu fullname: Xu, He-Xiu email: hxxuellen@gmail.com organization: Air and Missile Defense College, Air Force Engineering University, Xi’an 710051, China |
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Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance... Carbon materials were widely used as electromagnetic (EM) wave absorption due to their advantages of light weight, environmental resistance and high electrical... |
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| SubjectTerms | absorption aerogels anisotropy Carbon aerogel carbon nanofibers carbonization Carbonization degree cellulose compressibility electrical conductivity electromagnetic radiation Electromagnetic wave absorption finite element analysis graphene hydrophobicity insulating materials Oriented structures Propagation path temperature |
| Title | Broadband electromagnetic wave absorption using pure carbon aerogel by synergistically modulating propagation path and carbonization degree |
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