Occurrence, distribution, air-seawater exchange and atmospheric deposition of organophosphate esters (OPEs) from the Northwestern Pacific to the Arctic Ocean

Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media....

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Published inMarine pollution bulletin Vol. 157; p. 111243
Main Authors Na, Guangshui, Hou, Chao, Li, Ruijing, Shi, Yali, Gao, Hui, Jin, Shuaichen, Gao, Yunze, Jiao, Liping, Cai, Yaqi
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.08.2020
Elsevier BV
Subjects
Air
Air-seawater exchange
Arctic Ocean
Arctic region
Asia
Atmospheric deposition
Atmospheric pollution deposition
Deposition
Dry deposition
Esters
Exchanging
Gas-particle partitioning
marine pollution
Oceans
Organophosphate esters
Organophosphates
organophosphorus compounds
Polar environments
Polar regions
Seawater
Temperature
Transport
transportation
Arctic Ocean
Asia
Arctic region
Organophosphate esters
Gas-particle partitioning
Atmospheric deposition
Air-seawater exchange
Polar regions
Online AccessGet full text
ISSN0025-326X
1879-3363
1879-3363
DOI10.1016/j.marpolbul.2020.111243

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Abstract Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from −792.68 to 590.29 pg/m2/day. The dry deposition flux ranged from 16.4 to 185 ng/m2/day with high value observed at the Bering Strait (64.70 ng/m2/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the “sink” in polar regions of OPEs atmospheric transportation. [Display omitted] •First reported gaseous OPEs from the Northwestern Pacific to the Arctic Ocean.•Air-seawater exchange, atmospheric dry deposition were estimated.•High deposition fluxes founded in the Bering Strait and high Arctic.•New evidence about the “sink” in polar regions of OPEs was exhibited.
AbstractList Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from −792.68 to 590.29 pg/m2/day. The dry deposition flux ranged from 16.4 to 185 ng/m2/day with high value observed at the Bering Strait (64.70 ng/m2/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the "sink" in polar regions of OPEs atmospheric transportation.
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from -792.68 to 590.29 pg/m /day. The dry deposition flux ranged from 13.64 to 94.17 ng/m /day with high value observed at the Bering Strait (64.70 ng/m /day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the "sink" in polar regions of OPEs atmospheric transportation.
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ₁₁OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m³ and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from −792.68 to 590.29 pg/m²/day. The dry deposition flux ranged from 16.4 to 185 ng/m²/day with high value observed at the Bering Strait (64.70 ng/m²/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the “sink” in polar regions of OPEs atmospheric transportation.
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from -792.68 to 590.29 pg/m2/day. The dry deposition flux ranged from 16.4 to 185 ng/m2/day with high value observed at the Bering Strait (64.70 ng/m2/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the "sink" in polar regions of OPEs atmospheric transportation.Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from -792.68 to 590.29 pg/m2/day. The dry deposition flux ranged from 16.4 to 185 ng/m2/day with high value observed at the Bering Strait (64.70 ng/m2/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the "sink" in polar regions of OPEs atmospheric transportation.
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in air and seawater ranged from 231.56 to 1884.25 pg/m3 and from 8.47 to 143.45 ng/L, respectively. Halogenated OPEs dominated in both two media. The slight decreasing trend was observed for OPEs in gaseous air, no obvious trend for particle-bound OPEs and in seawater. The net air-seawater exchange flux ranged from −792.68 to 590.29 pg/m2/day. The dry deposition flux ranged from 16.4 to 185 ng/m2/day with high value observed at the Bering Strait (64.70 ng/m2/day). The relationship between temperature and OPEs particle-bound fractions suggests that temperature might be a driving factor of OPEs long-range atmospheric transport (LRAT). This research highlighted that OPEs are subject to LRAT from the Asian continent to the northwestern Pacific and Arctic Oceans and demonstrated the “sink” in polar regions of OPEs atmospheric transportation. [Display omitted] •First reported gaseous OPEs from the Northwestern Pacific to the Arctic Ocean.•Air-seawater exchange, atmospheric dry deposition were estimated.•High deposition fluxes founded in the Bering Strait and high Arctic.•New evidence about the “sink” in polar regions of OPEs was exhibited.
ArticleNumber 111243
Author Na, Guangshui
Li, Ruijing
Cai, Yaqi
Gao, Hui
Hou, Chao
Shi, Yali
Jin, Shuaichen
Gao, Yunze
Jiao, Liping
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  surname: Na
  fullname: Na, Guangshui
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  organization: College of Marine Environment and Ecology, Shanghai Ocean University, Shanghai 201306, China
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  givenname: Chao
  surname: Hou
  fullname: Hou, Chao
  organization: College of Marine Environment and Ecology, Shanghai Ocean University, Shanghai 201306, China
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  givenname: Ruijing
  surname: Li
  fullname: Li, Ruijing
  organization: National Marine Environmental Monitoring Center, Dalian 116023, China
– sequence: 4
  givenname: Yali
  surname: Shi
  fullname: Shi, Yali
  organization: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
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  surname: Gao
  fullname: Gao, Hui
  organization: National Marine Environmental Monitoring Center, Dalian 116023, China
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  surname: Jin
  fullname: Jin, Shuaichen
  organization: National Marine Environmental Monitoring Center, Dalian 116023, China
– sequence: 7
  givenname: Yunze
  surname: Gao
  fullname: Gao, Yunze
  organization: College of Marine Environment and Ecology, Shanghai Ocean University, Shanghai 201306, China
– sequence: 8
  givenname: Liping
  surname: Jiao
  fullname: Jiao, Liping
  organization: Third Institute Of Oceanography, Ministry of Natural Resources, P.R.C, Xiamen 361005, China
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  givenname: Yaqi
  surname: Cai
  fullname: Cai, Yaqi
  email: caiyaqi@rcees.ac.cn
  organization: State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/32469743$$D View this record in MEDLINE/PubMed
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Keywords Organophosphate esters
Gas-particle partitioning
Atmospheric deposition
Air-seawater exchange
Polar regions
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  text: 2020-08-01
  day: 01
PublicationDecade 2020
PublicationPlace England
PublicationPlace_xml – name: England
– name: Oxford
PublicationTitle Marine pollution bulletin
PublicationTitleAlternate Mar Pollut Bull
PublicationYear 2020
Publisher Elsevier Ltd
Elsevier BV
Publisher_xml – name: Elsevier Ltd
– name: Elsevier BV
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SSID ssj0007271
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Snippet Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ11OPEs in...
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ OPEs in...
Eleven organophosphate esters (OPEs) in air and seawater were investigated from the Northwestern Pacific to the Arctic Ocean. The concentration of Σ₁₁OPEs in...
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StartPage 111243
SubjectTerms Air
Air-seawater exchange
Arctic Ocean
Arctic region
Asia
Atmospheric deposition
Atmospheric pollution deposition
Deposition
Dry deposition
Esters
Exchanging
Gas-particle partitioning
marine pollution
Oceans
Organophosphate esters
Organophosphates
organophosphorus compounds
Polar environments
Polar regions
Seawater
Temperature
Transport
transportation
Title Occurrence, distribution, air-seawater exchange and atmospheric deposition of organophosphate esters (OPEs) from the Northwestern Pacific to the Arctic Ocean
URI https://dx.doi.org/10.1016/j.marpolbul.2020.111243
https://www.ncbi.nlm.nih.gov/pubmed/32469743
https://www.proquest.com/docview/2444683400
https://www.proquest.com/docview/2408196051
https://www.proquest.com/docview/2552023950
Volume 157
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