Promoted ion conductivity of sodium salt–poly(ethylene oxide) polymer electrolyte induced by adding conductive beta-alumina and application in all-solid-state sodium batteries
Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid poly...
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| Published in | Journal of materials science Vol. 56; no. 16; pp. 9951 - 9960 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.06.2021
Springer Springer Nature B.V |
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| Abstract | Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid polymer electrolytes with enhanced ion conductivity are demonstrated by introducing inorganic solid electrolyte (beta-alumina) filler. With the presence of conductive beta-alumina filler, the ion conductivity of the resultant PEO polymer electrolyte is enhanced from 2.5*10
–4
to 3.95*10
–4
S cm
−1
. Applied in sodium-ion batteries (SIBs), the cell delivers an initial discharge capacity of 93.1 mAh g
−1
and acceptable cycling performance (77.8 mAh g
−1
after 100 cycles), which are significantly superior to that of the PEO solid polymer electrolyte without beta-alumina filler modification. The presented results prove that the ion conductivity of PEO polymer electrolyte can be enhanced by adding conductive beta-alumina, promoting its practical application in Na-ion all-solid-state batteries or other electrochemical energy storage systems. |
|---|---|
| AbstractList | Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid polymer electrolytes with enhanced ion conductivity are demonstrated by introducing inorganic solid electrolyte (beta-alumina) filler. With the presence of conductive beta-alumina filler, the ion conductivity of the resultant PEO polymer electrolyte is enhanced from 2.5*10–⁴ to 3.95*10–⁴ S cm⁻¹. Applied in sodium-ion batteries (SIBs), the cell delivers an initial discharge capacity of 93.1 mAh g⁻¹ and acceptable cycling performance (77.8 mAh g⁻¹ after 100 cycles), which are significantly superior to that of the PEO solid polymer electrolyte without beta-alumina filler modification. The presented results prove that the ion conductivity of PEO polymer electrolyte can be enhanced by adding conductive beta-alumina, promoting its practical application in Na-ion all-solid-state batteries or other electrochemical energy storage systems. Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid polymer electrolytes with enhanced ion conductivity are demonstrated by introducing inorganic solid electrolyte (beta-alumina) filler. With the presence of conductive beta-alumina filler, the ion conductivity of the resultant PEO polymer electrolyte is enhanced from 2.5*10.sup.-4 to 3.95*10.sup.-4 S cm.sup.-1. Applied in sodium-ion batteries (SIBs), the cell delivers an initial discharge capacity of 93.1 mAh g.sup.-1 and acceptable cycling performance (77.8 mAh g.sup.-1 after 100 cycles), which are significantly superior to that of the PEO solid polymer electrolyte without beta-alumina filler modification. The presented results prove that the ion conductivity of PEO polymer electrolyte can be enhanced by adding conductive beta-alumina, promoting its practical application in Na-ion all-solid-state batteries or other electrochemical energy storage systems. Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid polymer electrolytes with enhanced ion conductivity are demonstrated by introducing inorganic solid electrolyte (beta-alumina) filler. With the presence of conductive beta-alumina filler, the ion conductivity of the resultant PEO polymer electrolyte is enhanced from 2.5*10 –4 to 3.95*10 –4 S cm −1 . Applied in sodium-ion batteries (SIBs), the cell delivers an initial discharge capacity of 93.1 mAh g −1 and acceptable cycling performance (77.8 mAh g −1 after 100 cycles), which are significantly superior to that of the PEO solid polymer electrolyte without beta-alumina filler modification. The presented results prove that the ion conductivity of PEO polymer electrolyte can be enhanced by adding conductive beta-alumina, promoting its practical application in Na-ion all-solid-state batteries or other electrochemical energy storage systems. Solid polymer electrolytes can significantly improve the safety and energy density of sodium-ion batteries compared with the liquid electrolytes. However, the low ionic conductivity and poor mechanical properties inhibit the practical application. In this paper, poly(ethylene oxide) (PEO) solid polymer electrolytes with enhanced ion conductivity are demonstrated by introducing inorganic solid electrolyte (beta-alumina) filler. With the presence of conductive beta-alumina filler, the ion conductivity of the resultant PEO polymer electrolyte is enhanced from 2.5*10–4 to 3.95*10–4 S cm−1. Applied in sodium-ion batteries (SIBs), the cell delivers an initial discharge capacity of 93.1 mAh g−1 and acceptable cycling performance (77.8 mAh g−1 after 100 cycles), which are significantly superior to that of the PEO solid polymer electrolyte without beta-alumina filler modification. The presented results prove that the ion conductivity of PEO polymer electrolyte can be enhanced by adding conductive beta-alumina, promoting its practical application in Na-ion all-solid-state batteries or other electrochemical energy storage systems. |
| Audience | Academic |
| Author | Wang, Xiaotong Liu, Zehua Chen, Jingjing Wang, Xinxin Wang, Dajian Mao, Zhiyong Yao, Yiwei |
| Author_xml | – sequence: 1 givenname: Yiwei surname: Yao fullname: Yao, Yiwei organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology – sequence: 2 givenname: Zehua surname: Liu fullname: Liu, Zehua organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology – sequence: 3 givenname: Xinxin surname: Wang fullname: Wang, Xinxin organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology – sequence: 4 givenname: Jingjing surname: Chen fullname: Chen, Jingjing email: cj313313@email.tjut.edu.cn organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology – sequence: 5 givenname: Xiaotong surname: Wang fullname: Wang, Xiaotong organization: Key Laboratory of Display Materials and Photoelectric Devices, Ministry of Education, Tianjin University of Technology – sequence: 6 givenname: Dajian surname: Wang fullname: Wang, Dajian organization: Key Laboratory of Display Materials and Photoelectric Devices, Ministry of Education, Tianjin University of Technology – sequence: 7 givenname: Zhiyong orcidid: 0000-0003-0125-3408 surname: Mao fullname: Mao, Zhiyong email: mzhy1984@163.com organization: Tianjin Key Laboratory for Photoelectric Materials and Devices, School of Materials Science and Engineering, Tianjin University of Technology |
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| CitedBy_id | crossref_primary_10_1002_anie_202417778 crossref_primary_10_1002_ange_202417778 crossref_primary_10_1021_acsaem_4c02012 crossref_primary_10_1007_s10008_023_05523_9 crossref_primary_10_1002_cssc_202202152 crossref_primary_10_1002_anie_202318822 crossref_primary_10_1002_ange_202318822 crossref_primary_10_3390_batteries10030073 crossref_primary_10_1021_acs_langmuir_4c01845 crossref_primary_10_1149_1945_7111_ac4bf6 crossref_primary_10_1016_j_electacta_2022_139936 crossref_primary_10_1016_j_cej_2022_135816 crossref_primary_10_1002_smtd_202201032 crossref_primary_10_1039_D3EE02082G crossref_primary_10_1039_D4EE05966B crossref_primary_10_1002_admt_202200822 crossref_primary_10_1002_est2_636 crossref_primary_10_1021_acsaem_3c01170 crossref_primary_10_1007_s41918_023_00196_4 crossref_primary_10_1016_j_jallcom_2025_179544 crossref_primary_10_1016_j_colsurfa_2023_131704 crossref_primary_10_1016_j_optmat_2022_112815 |
| Cites_doi | 10.1021/ja407393y 10.1021/acs.nanolett.5b00600 10.1039/C6TA07590H 10.1016/j.electacta.2017.03.118 10.3390/en11102559 10.1016/j.ssi.2008.04.006 10.1016/j.nanoen.2017.12.037 10.1016/0167-2738(82)90072-8 10.1016/j.ensm.2018.03.016 10.1016/j.ensm.2019.08.019 10.1038/natrevmats.2016.103 10.1016/j.ceramint.2019.12.074 10.1038/s41928-018-0048-6 10.1166/jnn.2008.18257 10.1021/acsomega.9b00885 10.1016/0167-2738(90)90081-2 10.1002/anie.200701144 10.1016/j.jpowsour.2013.09.137 10.1021/acs.jpcb.7b03985 10.1039/C7TA00314E 10.1016/j.jpowsour.2014.10.078 10.1039/C7SE00441A 10.1016/j.ensm.2019.07.012 10.1021/acsmaterialslett.9b00103 10.1038/srep06272 10.1039/b514346b 10.1038/srep21771 10.1021/acsenergylett.8b00948 10.1007/BF02708607 |
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| SubjectTerms | Alumina Aluminum oxide Batteries Characterization and Evaluation of Materials Chemical compounds Chemistry and Materials Science Classical Mechanics Crystallography and Scattering Methods Electric properties Electrochemistry Electrolytes energy energy density Energy Materials Energy storage Ethylene oxide Fillers Flux density Ion currents liquids Lithium Materials Science Mechanical properties Molten salt electrolytes Polyelectrolytes Polyethylene oxide Polymer Sciences Polymers Rechargeable batteries Sodium Sodium salts Solid electrolytes Solid Mechanics Solid state Storage batteries Storage systems |
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| Title | Promoted ion conductivity of sodium salt–poly(ethylene oxide) polymer electrolyte induced by adding conductive beta-alumina and application in all-solid-state sodium batteries |
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