Challenges in the ambient Raman spectroscopy characterization of methylammonium lead triiodide perovskite thin films
The importance triiodide （CH3NH3PbI3 or of methylammonium lead MAPbI3） organic-inorganic hybrid perovskites has shot up dramatically since their use in highly efficient thin-film perovskite solar cells （PSCs）. However, the basic structural characterization of these fascinating materials remains spar...
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| Published in | Frontiers of Optoelectronics (Online) Vol. 9; no. 1; pp. 81 - 86 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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Beijing
Higher Education Press
01.03.2016
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| Subjects | |
| Online Access | Get full text |
| ISSN | 2095-2759 2095-2767 |
| DOI | 10.1007/s12200-016-0573-8 |
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| Abstract | The importance triiodide （CH3NH3PbI3 or of methylammonium lead MAPbI3） organic-inorganic hybrid perovskites has shot up dramatically since their use in highly efficient thin-film perovskite solar cells （PSCs）. However, the basic structural characterization of these fascinating materials remains sparse. In particular, Raman spectroscopy, which is a powerful vibrational spectroscopy characterization tool and complements other characterization methods, of MAPbI3 under ambient conditions is plagued with difficulties. Here, a systematic ambient Raman spectroscopy characterization study of MAPbI3 thin films is conducted under different conditions （excitation laser wavelength, integration time, filter characteristic）. The results from this study help elucidate the possible sources of artifacts in the Raman spectra, and raise the awareness of the challenges in the ambient Raman spectroscopy of MAPbI3 perovskites. Approaches to overcome these challenges are suggested. |
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| AbstractList | The importance triiodide （CH3NH3PbI3 or of methylammonium lead MAPbI3） organic-inorganic hybrid perovskites has shot up dramatically since their use in highly efficient thin-film perovskite solar cells （PSCs）. However, the basic structural characterization of these fascinating materials remains sparse. In particular, Raman spectroscopy, which is a powerful vibrational spectroscopy characterization tool and complements other characterization methods, of MAPbI3 under ambient conditions is plagued with difficulties. Here, a systematic ambient Raman spectroscopy characterization study of MAPbI3 thin films is conducted under different conditions （excitation laser wavelength, integration time, filter characteristic）. The results from this study help elucidate the possible sources of artifacts in the Raman spectra, and raise the awareness of the challenges in the ambient Raman spectroscopy of MAPbI3 perovskites. Approaches to overcome these challenges are suggested. The importance of methylammonium lead triiodide (CH 3 NH 3 PbI 3 or MAPbI 3 ) organic-inorganic hybrid perovskites has shot up dramatically since their use in highly efficient thin-film perovskite solar cells (PSCs). However, the basic structural characterization of these fascinating materials remains sparse. In particular, Raman spectroscopy, which is a powerful vibrational spectroscopy characterization tool and complements other characterization methods, of MAPbI 3 under ambient conditions is plagued with difficulties. Here, a systematic ambient Raman spectroscopy characterization study of MAPbI 3 thin films is conducted under different conditions (excitation laser wavelength, integration time, filter characteristic). The results from this study help elucidate the possible sources of artifacts in the Raman spectra, and raise the awareness of the challenges in the ambient Raman spectroscopy of MAPbI 3 perovskites. Approaches to overcome these challenges are suggested. |
| Author | Yuanyuan ZHOU Hector F. GARCES Nitin P. PADTURE |
| AuthorAffiliation | School of Engineering, Brown University, Providence RI 02912, USA |
| Author_xml | – sequence: 1 givenname: Yuanyuan surname: Zhou fullname: Zhou, Yuanyuan email: yuanyuan_zhou@brown.edu organization: School of Engineering, Brown University – sequence: 2 givenname: Hector F. surname: Garces fullname: Garces, Hector F. organization: School of Engineering, Brown University – sequence: 3 givenname: Nitin P. surname: Padture fullname: Padture, Nitin P. email: nitin_padture@brown.edu organization: School of Engineering, Brown University |
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| Notes | The importance triiodide （CH3NH3PbI3 or of methylammonium lead MAPbI3） organic-inorganic hybrid perovskites has shot up dramatically since their use in highly efficient thin-film perovskite solar cells （PSCs）. However, the basic structural characterization of these fascinating materials remains sparse. In particular, Raman spectroscopy, which is a powerful vibrational spectroscopy characterization tool and complements other characterization methods, of MAPbI3 under ambient conditions is plagued with difficulties. Here, a systematic ambient Raman spectroscopy characterization study of MAPbI3 thin films is conducted under different conditions （excitation laser wavelength, integration time, filter characteristic）. The results from this study help elucidate the possible sources of artifacts in the Raman spectra, and raise the awareness of the challenges in the ambient Raman spectroscopy of MAPbI3 perovskites. Approaches to overcome these challenges are suggested. perovskite, solar cells, Raman spectroscopy,laser-degradation 11-5738/TN |
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| PublicationTitle | Frontiers of Optoelectronics (Online) |
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| Publisher | Higher Education Press |
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| Snippet | The importance triiodide （CH3NH3PbI3 or of methylammonium lead MAPbI3） organic-inorganic hybrid perovskites has shot up dramatically since their use in highly... The importance of methylammonium lead triiodide (CH 3 NH 3 PbI 3 or MAPbI 3 ) organic-inorganic hybrid perovskites has shot up dramatically since their use in... |
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| SubjectTerms | Biomedical Engineering and Bioengineering Electrical Engineering Engineering Physics Research Article 光谱表征 太阳能电池 拉曼光谱 有机-无机杂化 环境 碘化铅 薄膜 钙钛矿 |
| Title | Challenges in the ambient Raman spectroscopy characterization of methylammonium lead triiodide perovskite thin films |
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