Nanoparticle emissions from residential wood combustion: A critical literature review, characterization, and recommendations
The increased use of wood as a heating fuel in residential and small commercial buildings has increased concern about potential environmental and safety impacts, specifically particulate matter (PM) emissions in the nanometer range. Larger particles (> 2.5 µm) can be effectively removed from exha...
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Published in | Renewable & sustainable energy reviews Vol. 103; pp. 515 - 528 |
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Main Authors | , |
Format | Journal Article |
Language | English |
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United States
Elsevier Ltd
01.04.2019
Elsevier |
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Abstract | The increased use of wood as a heating fuel in residential and small commercial buildings has increased concern about potential environmental and safety impacts, specifically particulate matter (PM) emissions in the nanometer range. Larger particles (> 2.5 µm) can be effectively removed from exhaust streams by emission control devices. However, nanoparticles (NP), due to their size, are more difficult to capture in exhaust flue gases. In addition, NPs have a higher surface to volume ratio, allowing them to absorb organic compounds, causing them to be more reactive than their larger counterparts. This review focuses on the NPs produced from residential wood heating devices. Current emission regulations do not reflect the NP count or type produced from residential wood combustion, although most published studies show that a significant portion of the particles produced during combustion is in the nano-size range. Fuel type, device type and combustion periods have all shown to impact, at various degrees, the NPs produced. Contrary to common expectations, it appears that modern units may generate a higher count of NPs, although emitting less particulate mass than older units. This investigation supports arguments of needed particle type and count regulations in addition to the current mass based emission regulations. In addition to a critical review and analysis, recommendations are made regarding future testing, monitoring and environmental impact studies that address the significance of NP emissions.
•Heat from wood combustion may cause environmental impacts.•Large particles (>2.5 µm) are removed from exhaust streams by particulate control devices.•Nanoparticles (NPs) small size makes them more difficult to capture in exhaust gases.•Modern units may generate more NPs, but less particulate matter than older units.•Particle type and count should be added to current mass-based emission regulations. |
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AbstractList | The increased use of wood as a heating fuel in residential and small commercial buildings has increased concern about potential environmental and safety impacts, specifically particulate matter (PM) emissions in the nanometer range. Larger particles (> 2.5 µm) can be effectively removed from exhaust streams by emission control devices. However, nanoparticles (NP), due to their size, are more difficult to capture in exhaust flue gases. In addition, NPs have a higher surface to volume ratio, allowing them to absorb organic compounds, causing them to be more reactive than their larger counterparts. This review focuses here on the NPs produced from residential wood heating devices. Current emission regulations do not reflect the NP count or type produced from residential wood combustion, although most published studies show that a significant portion of the particles produced during combustion is in the nano-size range. Fuel type, device type and combustion periods have all shown to impact, at various degrees, the NPs produced. Contrary to common expectations, it appears that modern units may generate a higher count of NPs, although emitting less particulate mass than older units. This investigation supports arguments of needed particle type and count regulations in addition to the current mass based emission regulations. In addition to a critical review and analysis, recommendations are made regarding future testing, monitoring and environmental impact studies that address the significance of NP emissions. The increased use of wood as a heating fuel in residential and small commercial buildings has increased concern about potential environmental and safety impacts, specifically particulate matter (PM) emissions in the nanometer range. Larger particles (> 2.5 µm) can be effectively removed from exhaust streams by emission control devices. However, nanoparticles (NP), due to their size, are more difficult to capture in exhaust flue gases. In addition, NPs have a higher surface to volume ratio, allowing them to absorb organic compounds, causing them to be more reactive than their larger counterparts. This review focuses on the NPs produced from residential wood heating devices. Current emission regulations do not reflect the NP count or type produced from residential wood combustion, although most published studies show that a significant portion of the particles produced during combustion is in the nano-size range. Fuel type, device type and combustion periods have all shown to impact, at various degrees, the NPs produced. Contrary to common expectations, it appears that modern units may generate a higher count of NPs, although emitting less particulate mass than older units. This investigation supports arguments of needed particle type and count regulations in addition to the current mass based emission regulations. In addition to a critical review and analysis, recommendations are made regarding future testing, monitoring and environmental impact studies that address the significance of NP emissions. •Heat from wood combustion may cause environmental impacts.•Large particles (>2.5 µm) are removed from exhaust streams by particulate control devices.•Nanoparticles (NPs) small size makes them more difficult to capture in exhaust gases.•Modern units may generate more NPs, but less particulate matter than older units.•Particle type and count should be added to current mass-based emission regulations. |
Author | Trojanowski, Rebecca Fthenakis, Vasilis |
Author_xml | – sequence: 1 givenname: Rebecca surname: Trojanowski fullname: Trojanowski, Rebecca organization: Center for Life Cycle Analysis, Earth and Environmental Engineering, Columbia University, New York, NY, United States – sequence: 2 givenname: Vasilis surname: Fthenakis fullname: Fthenakis, Vasilis email: vmf5@columbia.edu organization: Center for Life Cycle Analysis, Earth and Environmental Engineering, Columbia University, New York, NY, United States |
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Title | Nanoparticle emissions from residential wood combustion: A critical literature review, characterization, and recommendations |
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