Facile fabrication of conductive polyaniline nanoflower modified electrode and its application for microbial energy harvesting
[Display omitted] •Facile approach for synthesis of conductive polyaniline nanoflower was developed.•Modification of carbon cloth electrode with polyaniline nanoflower was achieved.•The application of the modified electrode for microbial fuel cells was demonstrated A facile strategy for fabrication...
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| Published in | Electrochimica acta Vol. 255; pp. 41 - 47 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
20.11.2017
Elsevier BV |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
•Facile approach for synthesis of conductive polyaniline nanoflower was developed.•Modification of carbon cloth electrode with polyaniline nanoflower was achieved.•The application of the modified electrode for microbial fuel cells was demonstrated
A facile strategy for fabrication of conductive polyaniline (PANI) nanoflower modified carbon cloth electrode was developed and its application for microbial energy harvesting was also demonstrated. By simply tuning the concentration of aniline monomer, uniformly distributed PANI nanoflowers assembled from PANI nanoflakes anchored on the surface of carbon cloth electrode were fabricated with in-situ polymerization. Electrochemical and spectral analyses indicated that the synthesized PANI nanoflower was in conductive emeraldine salt form. Electrochemical impedance spectroscopy (EIS) analysis revealed PANI nanoflower modification reduced the charge transfer resistance of carbon cloth electrode, indicating the PANI nanoflower had excellent electrochemical activity. Furthermore, the PANI nanoflower modified electrode was used as the anode of microbial fuel cells (MFC), which delivered 2.6 and 6.5 times higher voltage and power output than these of pristine carbon cloth electrode, respectively. This work provided a controllable synthesis strategy for PANI nanostructure and demonstrated its promise in microbial energy harvesting. |
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| AbstractList | A facile strategy for fabrication of conductive polyaniline (PANI) nanoflower modified carbon cloth electrode was developed and its application for microbial energy harvesting was also demonstrated. By simply tuning the concentration of aniline monomer, uniformly distributed PANI nanoflowers assembled from PANI nanoflakes anchored on the surface of carbon cloth electrode were fabricated with in-situ polymerization. Electrochemical and spectral analyses indicated that the synthesized PANI nanoflower was in conductive emeraldine salt form. Electrochemical impedance spectroscopy (EIS) analysis revealed PANI nanoflower modification reduced the charge transfer resistance of carbon cloth electrode, indicating the PANI nanoflower had excellent electrochemical activity. Furthermore, the PANI nanoflower modified electrode was used as the anode of microbial fuel cells (MFC), which delivered 2.6 and 6.5 times higher voltage and power output than these of pristine carbon cloth electrode, respectively. This work provided a controllable synthesis strategy for PANI nanostructure and demonstrated its promise in microbial energy harvesting. [Display omitted] •Facile approach for synthesis of conductive polyaniline nanoflower was developed.•Modification of carbon cloth electrode with polyaniline nanoflower was achieved.•The application of the modified electrode for microbial fuel cells was demonstrated A facile strategy for fabrication of conductive polyaniline (PANI) nanoflower modified carbon cloth electrode was developed and its application for microbial energy harvesting was also demonstrated. By simply tuning the concentration of aniline monomer, uniformly distributed PANI nanoflowers assembled from PANI nanoflakes anchored on the surface of carbon cloth electrode were fabricated with in-situ polymerization. Electrochemical and spectral analyses indicated that the synthesized PANI nanoflower was in conductive emeraldine salt form. Electrochemical impedance spectroscopy (EIS) analysis revealed PANI nanoflower modification reduced the charge transfer resistance of carbon cloth electrode, indicating the PANI nanoflower had excellent electrochemical activity. Furthermore, the PANI nanoflower modified electrode was used as the anode of microbial fuel cells (MFC), which delivered 2.6 and 6.5 times higher voltage and power output than these of pristine carbon cloth electrode, respectively. This work provided a controllable synthesis strategy for PANI nanostructure and demonstrated its promise in microbial energy harvesting. |
| Author | Shi, Yu-Tong Liu, Xiang Cheng, Qian-Wen Zhao, Xiaohua Yu, Yang-Yang Fang, Zhen Yong, Yang-Chun Wang, Yan-Zhai |
| Author_xml | – sequence: 1 givenname: Xiang surname: Liu fullname: Liu, Xiang organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 2 givenname: Xiaohua surname: Zhao fullname: Zhao, Xiaohua organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 3 givenname: Yang-Yang surname: Yu fullname: Yu, Yang-Yang organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 4 givenname: Yan-Zhai surname: Wang fullname: Wang, Yan-Zhai organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 5 givenname: Yu-Tong surname: Shi fullname: Shi, Yu-Tong organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 6 givenname: Qian-Wen surname: Cheng fullname: Cheng, Qian-Wen organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 7 givenname: Zhen surname: Fang fullname: Fang, Zhen organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 8 givenname: Yang-Chun surname: Yong fullname: Yong, Yang-Chun email: ycyong@ujs.edu.cn organization: Biofuels Institute, School of Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China |
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•Facile approach for synthesis of conductive polyaniline nanoflower was developed.•Modification of carbon cloth electrode with polyaniline... A facile strategy for fabrication of conductive polyaniline (PANI) nanoflower modified carbon cloth electrode was developed and its application for microbial... |
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| SubjectTerms | Aniline Biochemical fuel cells Bioenergy Carbon Charge transfer Chemical synthesis Cloth Conductivity Electrochemical impedance spectroscopy Electrodes Energy harvesting Fuel cells Heat conductivity Microbial fuel cells Microorganisms Nanoflower Polyaniline Polyanilines Polymerization Shewanella |
| Title | Facile fabrication of conductive polyaniline nanoflower modified electrode and its application for microbial energy harvesting |
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