Melamine as a single source for fabrication of mesoscopic 3D composites of N-doped carbon nanotubes on graphene
Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CV...
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Published in | RSC advances Vol. 8; no. 22; pp. 12157 - 12164 |
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Main Authors | , , , , , , , , |
Format | Journal Article |
Language | English |
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England
Royal Society of Chemistry
01.01.2018
The Royal Society of Chemistry |
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Abstract | Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G)
via
a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn-Ni-Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion.
Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. |
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AbstractList | Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G)
via
a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn-Ni-Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion.
Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G) a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn-Ni-Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion. Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G) via a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn-Ni-Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion.Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G) via a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn-Ni-Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion. Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G) via a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn–Ni–Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion. Integration of two-dimensional graphene and one-dimensional carbon nanotubes (CNTs) to create potentially useful 3D mesoscopic carbon structures with enhanced properties relative to the original materials is very desirable. Here, we report a novel and simple route using chemical vapor deposition (CVD) methods to fabricate bead-like nitrogen-doped CNT/graphene composites (NCNT/G) via a simple pyrolysis of the N-rich melamine in the presence of graphene oxide (GO) as a substrate using a Mn–Ni–Co ternary catalyst. We have characterized these structures by field-emission scanning electron microscopy, transmission electron microscopy, X-ray diffraction, Raman spectra, isothermal analyses, and X-ray photoelectron spectroscopy. The three dimensional NCNT/G hybrids have unique network structures, moderate graphitization, high specific surface area, good mesoporosity, and N doping, which makes them promising materials for applications in energy storage and conversion. |
Author | Li, Hua-Fei Yan, Xiao-Ling Dai, Gui-Ping Wu, Marvin H Hu, Hai-Yan Jiang, Bang-Bang Xie, Ning Vinodgopal, K Wang, Chen |
AuthorAffiliation | Dept. of Physics Institute for Advanced Study North Carolina Central University Dept. of Chemistry and Biochemistry School of Resources Environmental & Chemical Engineering Nanchang University |
AuthorAffiliation_xml | – name: Nanchang University – name: North Carolina Central University – name: Dept. of Physics – name: School of Resources Environmental & Chemical Engineering – name: Dept. of Chemistry and Biochemistry – name: Institute for Advanced Study |
Author_xml | – sequence: 1 givenname: Xiao-Ling surname: Yan fullname: Yan, Xiao-Ling – sequence: 2 givenname: Hua-Fei surname: Li fullname: Li, Hua-Fei – sequence: 3 givenname: Chen surname: Wang fullname: Wang, Chen – sequence: 4 givenname: Bang-Bang surname: Jiang fullname: Jiang, Bang-Bang – sequence: 5 givenname: Hai-Yan surname: Hu fullname: Hu, Hai-Yan – sequence: 6 givenname: Ning surname: Xie fullname: Xie, Ning – sequence: 7 givenname: Marvin H surname: Wu fullname: Wu, Marvin H – sequence: 8 givenname: K surname: Vinodgopal fullname: Vinodgopal, K – sequence: 9 givenname: Gui-Ping surname: Dai fullname: Dai, Gui-Ping |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35539379$$D View this record in MEDLINE/PubMed |
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SubjectTerms | Carbon Carbon nanotubes Chemical vapor deposition Chemistry Electron microscopy Energy storage Graphene Graphitization Manganese Melamine Microscopy Nanotubes Nickel Nitrogen Pyrolysis Raman spectra Spectrum analysis Substrates Three dimensional composites X-ray diffraction |
Title | Melamine as a single source for fabrication of mesoscopic 3D composites of N-doped carbon nanotubes on graphene |
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