Investigation of the impacts of ethyl lactate based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils
•Accumulation of oxy-PAHs was observed, with ATQ as the most abundant compound.•ATQ had lower accumulation in ethyl lactate based compared to ethanol based Fenton.•Both positive and negative impacts on soil physicochemical properties were recorded.•For revegetation, the treatment was most suitable f...
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| Published in | Journal of hazardous materials Vol. 262; pp. 691 - 700 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier B.V
15.11.2013
Elsevier |
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| Abstract | •Accumulation of oxy-PAHs was observed, with ATQ as the most abundant compound.•ATQ had lower accumulation in ethyl lactate based compared to ethanol based Fenton.•Both positive and negative impacts on soil physicochemical properties were recorded.•For revegetation, the treatment was most suitable for soil with native pH≳6.2.
This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH≳6.2 in order to obtain a final soil pH≳4.9 subject to the soil buffering capacity. |
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| AbstractList | This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH >/~ 6.2 in order to obtain a final soil pH >/~ 4.9 subject to the soil buffering capacity. This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH≳6.2 in order to obtain a final soil pH≳4.9 subject to the soil buffering capacity. This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH >/~ 6.2 in order to obtain a final soil pH >/~ 4.9 subject to the soil buffering capacity.This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH >/~ 6.2 in order to obtain a final soil pH >/~ 4.9 subject to the soil buffering capacity. •Accumulation of oxy-PAHs was observed, with ATQ as the most abundant compound.•ATQ had lower accumulation in ethyl lactate based compared to ethanol based Fenton.•Both positive and negative impacts on soil physicochemical properties were recorded.•For revegetation, the treatment was most suitable for soil with native pH≳6.2. This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils. Accumulation of oxygenated-polycyclic aromatic hydrocarbons (oxy-PAHs) was observed, but quantitative measurement on the most abundant compound 9,10-anthraquinone (ATQ) showed lower accumulation of the compound than that reported for ethanol (ET) based Fenton treatment. In general, as compared to conventional water (CW) based Fenton treatment, the EL based Fenton treatment exerted either a lower or higher negative impact on soil physicochemical properties depending on the property type and shared the main disadvantage of reduced soil pH. For revegetation, EL based Fenton treatment was most appropriately adopted for soil with native pH≳6.2 in order to obtain a final soil pH≳4.9 subject to the soil buffering capacity. |
| Author | Venny Ng, Hoon Kiat Yap, Chiew Lin Gan, Suyin |
| Author_xml | – sequence: 1 givenname: Suyin surname: Gan fullname: Gan, Suyin email: suyin.gan@nottingham.edu.my, suyingan@yahoo.co.uk organization: Department of Chemical and Environmental Engineering, The University of Nottingham Malaysia Campus, Jalan Broga, 43500 Semenyih, Selangor Darul Ehsan, Malaysia – sequence: 2 givenname: Chiew Lin surname: Yap fullname: Yap, Chiew Lin organization: Department of Chemical and Environmental Engineering, The University of Nottingham Malaysia Campus, Jalan Broga, 43500 Semenyih, Selangor Darul Ehsan, Malaysia – sequence: 3 givenname: Hoon Kiat surname: Ng fullname: Ng, Hoon Kiat organization: Department of Mechanical, Materials and Manufacturing Engineering, The University of Nottingham Malaysia Campus, Jalan Broga, 43500 Semenyih, Selangor Darul Ehsan, Malaysia – sequence: 4 surname: Venny fullname: Venny organization: Department of Chemical and Environmental Engineering, The University of Nottingham Malaysia Campus, Jalan Broga, 43500 Semenyih, Selangor Darul Ehsan, Malaysia |
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| Copyright | 2013 Elsevier B.V. 2015 INIST-CNRS Copyright © 2013 Elsevier B.V. All rights reserved. |
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| Keywords | Transformation products Soil quality Fenton Polycyclic aromatic hydrocarbons (PAHs) Ethyl lactate Soil physicochemical properties Hydrocarbon Property of soil Revegetation Polycyclic aromatic compound Soil pollution Buffering capacity Persistent organic pollutant pH Fenton reaction Oxidation Physicochemical properties Organic compounds |
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| Snippet | •Accumulation of oxy-PAHs was observed, with ATQ as the most abundant compound.•ATQ had lower accumulation in ethyl lactate based compared to ethanol based... This study aims to investigate the impacts of ethyl lactate (EL) based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons... |
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| SubjectTerms | Applied sciences buffering capacity Chemical engineering Decontamination. Miscellaneous Environmental Restoration and Remediation ethanol Ethyl lactate Exact sciences and technology Fenton Lactates - chemistry land restoration polluted soils Pollution polycyclic aromatic hydrocarbons Polycyclic aromatic hydrocarbons (PAHs) Polycyclic Aromatic Hydrocarbons - analysis Polycyclic Aromatic Hydrocarbons - chemistry quantitative analysis Reactors Soil - chemistry Soil and sediments pollution soil pH Soil physicochemical properties Soil Pollutants - analysis Soil Pollutants - chemistry soil pollution Soil quality soil remediation soil treatment Transformation products Water - chemistry |
| Title | Investigation of the impacts of ethyl lactate based Fenton treatment on soil quality for polycyclic aromatic hydrocarbons (PAHs)-contaminated soils |
| URI | https://dx.doi.org/10.1016/j.jhazmat.2013.09.023 https://www.ncbi.nlm.nih.gov/pubmed/24121640 https://www.proquest.com/docview/1459562043 https://www.proquest.com/docview/1705453798 |
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